NASA - National Aeronautics and Space Administration

AATS-14 measures direct solar beam transmission at 14 wavelengths between 354 and 2139 nm in narrow channels with bandwidths between 2 and 5.6 nm for the wavelengths less than 1640 nm and 17.3 nm for the 2139 nm channel. The transmission measurements at all channels except 940 nm are used to retrieve spectra of aerosol optical depth (AOD). In addition, the transmission at 940 nm and surrounding channels is used to derive columnar water vapor (CWV) [Livingston et al., 2008]. Methods for AATS-14 data reduction, calibration, and error analysis have been described extensively, for example, by Russell et al. [2007] and Shinozuka et al. [2011]. AATS-14 measurements of spectral AOD and CWV obtained during aircraft vertical profiles can be differentiated to determine corresponding vertical profiles of spectral aerosol extinction and water vapor density. Such measurements have been used extensively in the characterization of the horizontal and vertical distribution of aerosol optical properties and in the validation of satellite aerosol sensors. For example, in the Aerosol Characterization Experiment-Asia (ACE-Asia), AATS measurements were used for closure (consistency) studies with in situ aerosol samplers aboard the NCAR C-130 and the CIRPAS Twin-Otter aircraft, and with ground-based lidar systems. In ACE-Asia, CLAMS (Chesapeake Lighthouse & Aircraft Measurements for Satellites, 2001), the Extended-MODIS-λ Validation Experiment (EVE), INTEX-A, INTEX-B, and ARCTAS, AATS results have been used in the validation of satellite sensors aboard various EOS platforms, providing important aerosol information used in the improvement of retrieval algorithms for the MISR and MODIS sensors among others.

Aerosols (particulate matter) have a dramatic effect on radiative forcing of the climate, in some cases cooling and in other cases warming. The Fourth Assessment Report of the IPCC estimates that direct radiative forcing due to all aerosols is a cooling of -0.50 W m-2 with absorbing aerosol (black carbon) responsible for a warming of +0.22 W m-2, but the uncertainties associated with these numbers are very large. Better measurements of the optical properties of aerosols, especially absorption coefficient and asymmetry parameter, and their spatial and temporal distribution are required to reduce these uncertainties and improve the ability of models to predict climate change. Aero3X was designed to provide such measurements. It is a light weight (11 kg), compact (0.25 x 0.30 x 0.6 m), and fast (1 Hz sample rate) instrument intended for use on an Unmanned Aerial System (UAS) but suitable for flight on other aircraft and for surface measurements. Aero3X uses an off-axis cavity ring-down technique to measure extinction coefficient and a reciprocal nephelometry technique for measurement of total-, forward- and back-scatter coefficients at wavelengths of 405 nm and 675 nm. Its outstanding precision (0.1 Mm-1) and sensitivity (0.2 Mm- 1) allow the determination of absorption coefficient, single-scattering albedo, estimates of backscatter to extinction ratio and asymmetry parameter at both wavelengths, and Angstrom exponent. Together with its humidification system for measurement of the dependence of aerosol optical properties on relative humidity, these represent a complete set of the aerosol optical properties important to climate and air quality. Aero3X was designed to operate in pollution plumes where NO2 may cause interference with the measurement, therefore, a measurement of NO2 mixing ratio is also made.

ATHOS uses laser-induced fluorescence (LIF) to measure OH and HO2 simultaneously. OH is both excited and detected with the A2Σ+ (v’=0) → X2π (v”=0) transition near 308 nm. HO2 is reacted with reagent NO to form OH and is then detected with LIF. The laser is tuned on and off the OH wavelength to determine the fluorescence and background signals. ATHOS can detect OH and HO2 in clear air and light clouds from Earth's surface to the lower stratosphere. The ambient air is slowed from the aircraft speed of 240 m/s to 8-40 m/s in an aerodynamic nacelle. It is then pulled by a vacuum pump through a small inlet, up a sampling tube, and into two low-pressure detection cells - the first for OH and the second for HO2. Detection occurs in each cell at the intersection of the airflow, the laser beam, and the detector field-of-view.