30 1001 Viggiano, A 781-377-4208, Ballenthin, J -3755, Hunton, D -4057, Miller, T -5031 Air Force Research Laboratory, AFRL/VSBP, 29 Randolph Rd, Hanscom AFB, MA 01731 Trace Gas Concentrations from Chemical Ionization Mass Spectrometer (CIMS) SONEX Campaign, Ames - Bangor, October, 1997 1 1 1997 10 13 1998 7 30 0 Elapsed Time in UT Seconds from 0 hours on day of flight 2 1 1 9999 9999 HNO3 concentration (pptv) SO2 concentration (pptv) 3 Comments for this flight: Calibration source: CIMS data normalized to UNH HNO3 data throughout flight Comparison to UNH HNO3: most trends agree; CIMS HNO3 increase at 66600 not seen in UNH data 11 Comments for entire CIMS Final Data Set: Time dependence of permeation tube emission rate has been included 5% correction of tube center flow to average flow rate has been included Deconvolution of adjacent ion peaks has been done using least squares peak fitting Instrumental background count rate ("dark" counts) has been subtracted No additional background subtraction (e.g. to correct wall outgassing) for HNO3 or SO2 has been done. Data are ten second averages - time listed is end of integration period One-second data can be provided as requested for specific times Calibrations have been replaced with missing data codes; altitude transitions are included SO2 sensitivity based on HNO3 permeation tube calibrations and k(HNO3) / k(SO2) = 1.7 UT(sec) HNO3 SO2 63471 63 0 63481 51 21 63491 69 0 63501 111 16 63511 44 0 63521 57 21 63531 35 21 63541 82 54 63551 85 38 63561 92 54 63571 79 21 63581 82 21 63591 88 38 63601 66 38 63611 63 38 63621 51 11 63631 22 81 63641 73 59 63651 85 54 63661 41 0 63671 117 97 63681 123 97 63691 155 54 63701 92 0 63711 114 11 63721 88 54 63731 92 0 63741 104 21 63751 133 59 63761 114 38 63771 117 38 63781 98 54 63791 107 21 63801 44 21 63811 85 54 63821 76 54 63831 107 38 63841 114 0 63851 51 81 63861 57 81 63871 44 27 63881 104 21 63891 60 70 63901 107 27 63911 66 38 63921 44 54 63931 13 38 63941 82 48 63951 117 0 63961 66 54 63971 41 38 63981 28 27 63991 73 81 64001 101 150 64011 47 70 64021 98 0 64031 9999 97 64041 9999 97 64051 9999 140 64061 9999 113 64071 9999 81 64081 9999 81 64091 9999 97 64101 9999 54 64111 9999 75 64121 9999 64 64131 9999 38 64141 9999 64 64151 9999 75 64161 9999 38 64171 9999 54 64181 9999 21 64191 9999 97 64201 9999 21 64211 9999 107 64221 9999 75 64231 9999 54 64241 9999 97 64251 9999 97 64261 9999 123 64271 9999 150 64281 9999 38 64291 9999 113 64301 9999 54 64311 9999 54 64321 9999 54 64331 9999 54 64341 9999 38 64351 9999 54 64361 9999 21 64371 9999 123 64381 9999 0 64391 9999 27 64401 9999 54 64411 9999 107 64421 9999 91 64431 9999 64 64441 9999 81 64451 9999 54 64461 9999 -5 64471 9999 16 64481 9999 21 64491 9999 21 64501 9999 27 64511 9999 38 64521 9999 134 64531 9999 11 64541 9999 75 64551 9999 54 64561 9999 113 64571 9999 64 64581 9999 0 64591 9999 -5 64601 9999 59 64611 9999 70 64621 9999 64 64631 9999 113 64641 9999 81 64651 9999 38 64661 9999 64 64671 9999 150 64681 158 54 64691 234 97 64701 161 48 64711 174 64 64721 183 21 64731 111 54 64741 139 75 64751 123 64 64761 224 59 64771 189 107 64781 167 86 64791 196 102 64801 199 107 64811 177 86 64821 142 134 64831 186 91 64841 186 150 64851 183 75 64861 180 161 64871 152 107 64881 180 59 64891 202 107 64901 161 161 64911 234 54 64921 142 38 64931 221 54 64941 262 59 64951 231 38 64961 253 75 64971 360 11 64981 243 54 64991 335 21 65001 319 54 65011 357 38 65021 338 27 65031 313 59 65050 213 36 65060 276 36 65070 213 14 65080 280 25 65090 295 25 65100 251 36 65110 272 25 65120 301 25 65130 286 18 65140 160 75 65150 135 64 65160 101 75 65170 99 9999 65180 126 9999 65190 82 9999 65200 120 9999 65210 187 9999 65220 242 9999 65230 204 9999 65240 168 9999 65250 154 9999 65260 152 9999 65270 61 311 65280 141 222 65290 9999 125 65300 9999 183 65310 9999 222 65320 9999 75 65330 9999 233 65340 9999 186 65350 9999 147 65360 9999 9999 65370 9999 9999 65380 9999 9999 65390 9999 9999 65400 9999 9999 65410 9999 9999 65420 9999 9999 65430 9999 9999 65440 9999 9999 65450 9999 9999 65460 9999 9999 65470 9999 9999 65480 9999 9999 65490 9999 9999 65500 9999 9999 65510 9999 9999 65520 9999 9999 65530 9999 9999 65540 175 9999 65550 141 9999 65560 149 9999 65570 149 9999 65580 181 9999 65590 137 9999 65600 156 9999 65610 116 186 65620 194 193 65630 192 225 65640 152 222 65650 179 111 65660 185 147 65670 147 183 65680 137 175 65690 143 200 65700 152 225 65710 97 222 65720 118 211 65730 143 54 65740 154 89 65750 99 140 65760 105 240 65770 147 150 65780 120 268 65790 143 111 65800 139 175 65810 204 150 65820 135 136 65830 149 186 65840 74 136 65850 141 143 65860 116 125 65870 120 193 65880 103 261 65890 120 229 65900 189 276 65910 131 268 65920 128 286 65930 126 276 65940 133 157 65950 131 512 65960 141 304 65970 135 100 65980 93 193 65990 171 211 66000 133 147 66010 173 211 66020 164 211 66030 133 9999 66040 6 9999 66050 2 9999 66060 0 9999 66070 15 9999 66080 32 9999 66090 116 9999 66100 147 9999 66110 131 9999 66120 133 9999 66130 76 9999 66140 85 9999 66150 68 9999 66160 73 9999 66170 90 9999 66180 104 9999 66190 122 9999 66200 99 9999 66210 73 9999 66220 74 9999 66230 98 9999 66240 69 9999 66250 99 9999 66260 101 9999 66270 65 9999 66280 66 9999 66290 63 9999 66300 55 9999 66310 109 9999 66320 118 9999 66330 88 9999 66340 43 9999 66350 44 9999 66360 68 9999 66370 153 9999 66380 175 9999 66390 155 9999 66400 202 9999 66410 193 9999 66420 253 9999 66430 245 9999 66440 294 9999 66450 235 9999 66460 309 9999 66470 322 9999 66480 330 9999 66490 237 9999 66500 279 9999 66510 336 9999 66520 292 9999 66530 347 9999 66540 321 9999 66550 336 9999 66560 261 9999 66570 330 9999 66580 281 9999 66590 308 9999 66600 287 9999 66610 237 9999 66620 9999 9999 66630 9999 9999 66640 9999 9999 66650 9999 9999 66660 9999 9999 66670 9999 9999 66680 9999 9999 66690 9999 9999 66700 9999 9999 66710 9999 9999 66720 9999 9999 66730 9999 9999 66740 9999 9999 66750 9999 9999 66760 9999 9999 66770 9999 9999 66780 9999 9999 66790 9999 9999 66800 9999 9999 66810 9999 9999 66820 9999 9999 66830 9999 9999 66840 9999 9999 66850 9999 9999 66860 9999 9999 66870 9999 9999 66880 9999 9999 66890 9999 9999 66900 9999 9999 66910 9999 9999 66920 9999 9999 66930 9999 9999 66940 9999 9999 66950 9999 9999 66960 9999 9999 66970 9999 9999 66980 9999 9999 66990 9999 9999 67000 9999 9999 67010 9999 9999 67020 9999 9999 67030 212 258 67040 303 376 67050 248 207 67060 242 357 67070 246 357 67080 273 346 67090 259 381 67100 262 349 67110 283 250 67120 229 199 67130 215 282 67140 313 314 67150 253 268 67160 221 201 67170 216 266 67180 188 150 67190 215 255 67200 189 129 67210 194 161 67220 169 140 67230 117 142 67240 125 134 67250 169 169 67260 172 153 67270 208 115 67280 164 150 67290 189 185 67300 156 180 67310 183 193 67320 185 156 67330 196 113 67340 155 123 67350 171 148 67360 137 129 67370 125 177 67380 166 250 67390 182 172 67400 166 142 67410 117 129 67420 224 137 67430 166 188 67440 164 140 67450 210 158 67460 153 150 67470 174 113 67480 152 129 67490 153 158 67500 126 145 67510 123 145 67520 76 70 67530 98 83 67540 84 46 67550 128 51 67560 85 86 67570 98 72 67580 134 72 67590 111 78 67600 114 70 67610 79 97 67620 129 46 67630 71 102 67640 118 115 67650 98 89 67660 65 115 67670 117 75 67680 73 91 67690 95 137 67700 106 59 67710 77 78 67720 111 107 67730 118 64 67740 103 89 67750 99 102 67760 66 105 67770 79 62 67780 9999 81 67790 9999 115 67800 9999 75 67810 9999 46 67820 9999 140 67830 9999 242 67840 9999 341 67850 9999 298 67860 9999 336 67870 9999 255 67880 9999 129 67890 9999 89 67900 9999 153 67910 99 134 67920 122 145 67930 169 252 67940 129 250 67950 147 255 67960 141 166 67970 199 183 67980 182 188 67990 178 81 68000 164 145 68010 148 153 68020 120 94 68030 126 145 68040 141 94 68050 136 94 68060 9999 164 68070 9999 209 68080 9999 89 68090 9999 134 68100 9999 148 68110 9999 137 68120 9999 9999 68130 9999 9999 68140 9999 9999 68150 9999 9999 68160 9999 9999 68170 9999 9999 68180 9999 9999 68190 9999 9999 68200 9999 9999 68210 9999 9999 68220 9999 9999 68230 9999 9999 68240 9999 9999 68250 9999 9999 68260 9999 9999 68270 9999 9999 68280 9999 9999 68290 9999 9999 68300 9999 9999 68310 9999 9999 68320 9999 9999 68330 9999 9999 68340 9999 9999 68350 9999 9999 68360 9999 9999 68370 185 9999 68380 156 9999 68390 148 9999 68400 175 9999 68410 148 9999 68420 167 9999 68430 171 9999 68440 118 9999 68450 166 9999 68460 133 161 68470 148 180 68480 117 153 68490 148 105 68500 96 156 68510 131 180 68520 123 145 68530 104 110 68540 150 177 68550 101 121 68560 118 180 68570 159 118 68580 118 169 68590 129 132 68600 122 193 68610 133 172 68620 111 148 68630 147 105 68640 139 150 68650 118 72 68660 106 156 68670 114 115 68680 77 123 68690 134 99 68700 84 123 68710 144 158 68720 123 134 68730 85 94 68740 109 102 68750 131 94 68760 137 126 68770 122 129 68780 126 89 68790 131 132 68800 96 161 68810 112 121 68820 87 94 68830 99 115 68840 93 134 68850 125 115 68860 120 86 68870 144 110 68880 137 59 68890 88 56 68900 98 81 68910 125 83 68920 92 158 68930 76 123 68940 148 110 68950 120 137 68960 148 121 68970 134 105 68980 148 81 68990 136 140 69000 81 121 69010 103 185 69020 111 134 69030 131 142 69040 106 89 69050 126 148 69060 107 86 69070 123 110 69080 106 97 69090 85 132 69100 81 113 69110 88 118 69120 103 123 69130 81 89 69140 112 123 69150 104 115 69160 76 107 69170 69 123 69180 9999 132 69190 9999 121 69200 9999 9999 69210 9999 9999 69220 9999 9999 69230 9999 9999 69240 9999 9999 69250 9999 9999 69260 9999 9999 69270 9999 9999 69280 9999 9999 69290 9999 9999 69300 9999 9999 69310 9999 9999 69320 9999 9999 69330 9999 9999 69340 9999 9999 69350 9999 9999 69360 9999 9999 69370 9999 9999 69380 9999 9999 69390 9999 9999 69400 9999 9999 69410 9999 9999 69420 9999 9999 69430 9999 9999 69440 9999 9999 69450 9999 9999 69460 9999 9999 69470 9999 9999 69480 9999 9999 69490 9999 9999 69500 9999 9999 69510 9999 9999 69520 9999 9999 69530 9999 9999 69540 9999 9999 69550 9999 9999 69560 9999 9999 69570 9999 9999 69580 9999 9999 69590 9999 9999 69600 9999 9999 69610 9999 9999 69620 9999 9999 69630 9999 9999 69640 9999 9999 69650 9999 9999 69660 9999 9999 69670 9999 9999 69680 9999 9999 69690 9999 9999 69700 9999 9999 69710 9999 9999 69720 9999 9999 69730 9999 9999 69740 9999 9999 69750 9999 9999 69760 9999 9999 69770 9999 9999 69780 9999 9999 69790 9999 9999 69800 9999 9999 69810 9999 9999 69820 9999 9999 69830 9999 9999 69840 9999 9999 69850 188 9999 69860 161 9999 69870 161 9999 69880 161 9999 69890 112 9999 69900 103 150 69910 139 110 69920 128 134 69930 90 62 69940 112 91 69950 139 105 69960 107 59 69970 96 75 69980 107 89 69990 104 91 70000 112 91 70010 92 83 70020 93 115 70030 125 51 70040 93 64 70050 88 67 70060 69 102 70070 90 102 70080 76 46 70090 104 81 70100 77 48 70110 79 94 70120 84 64 70130 104 70 70140 112 56 70150 84 43 70160 115 51 70170 96 70 70180 103 121 70190 104 64 70200 71 51 70210 92 24 70220 79 56 70230 77 70 70240 123 48 70250 107 59 70260 120 59 70270 104 78 70280 77 83 70290 76 64 70300 87 91 70310 114 78 70320 84 62 70330 99 70 70340 68 81 70350 85 62 70360 77 51 70370 60 102 70380 87 99 70390 77 83 70400 88 62 70410 81 72 70420 77 91 70430 82 48 70440 79 70 70450 77 86 70460 103 70 70470 58 78 70480 103 56 70490 81 137 70500 77 91 70510 98 78 70520 112 48 70530 92 118 70540 92 70 70550 58 72 70560 96 51 70570 88 46 70580 122 56 70590 87 64 70600 88 81 70610 85 48 70620 62 91 70630 73 64 70640 106 97 70650 88 81 70660 74 121 70670 101 75 70680 76 72 70690 74 59 70700 73 99 70710 92 59 70720 87 70 70730 69 59 70740 115 126 70750 95 91 70760 95 89 70770 109 86 70780 90 115 70790 98 67 70800 122 56 70810 109 137 70820 68 102 70830 66 59 70840 101 62 70850 68 40 70860 74 59 70870 69 94 70880 81 81 70890 93 102 70900 101 78 70910 84 64 70920 99 40 70930 68 110 70940 92 123 70950 79 91 70960 109 86 70970 92 89 70980 71 9999 70990 9999 9999 71000 9999 9999 71010 9999 9999 71020 9999 9999 71030 9999 9999 71040 9999 9999 71050 9999 9999 71060 9999 9999 71070 9999 9999 71080 9999 9999 71090 9999 9999 71100 9999 9999 71110 9999 9999 71120 9999 9999 71130 9999 9999 71140 9999 9999 71150 9999 9999 71160 9999 9999 71170 9999 9999 71180 9999 9999 71190 9999 9999 71200 9999 9999 71210 9999 9999 71220 9999 9999 71230 9999 9999 71240 9999 9999 71250 9999 9999 71260 9999 9999 71270 9999 9999 71280 9999 9999 71290 9999 9999 71300 9999 9999 71310 9999 9999 71320 9999 9999 71330 9999 9999 71340 9999 9999 71350 9999 9999 71360 9999 9999 71370 9999 9999 71380 9999 9999 71390 9999 9999 71400 9999 9999 71410 9999 9999 71420 9999 9999 71430 9999 9999 71440 9999 9999 71450 9999 9999 71460 9999 9999 71470 9999 9999 71480 164 9999 71490 169 9999 71500 111 9999 71510 129 9999 71520 122 9999 71530 122 9999 71540 104 126 71550 131 43 71560 106 99 71570 99 78 71580 96 64 71590 92 81 71600 74 64 71610 87 38 71620 106 46 71630 57 51 71640 82 43 71650 77 40 71660 95 78 71670 115 62 71680 85 51 71690 103 94 71700 112 30 71710 71 19 71720 114 62 71730 123 48 71740 77 35 71750 71 62 71760 84 46 71770 98 48 71780 93 38 71790 60 40 71800 99 43 71810 109 46 71820 92 27 71830 68 46 71840 115 30 71850 90 38 71860 87 51 71870 104 48 71880 118 48 71890 81 78 71900 65 67 71910 117 105 71920 115 48 71930 62 64 71940 55 59 71950 68 40 71960 66 40 71970 88 46 71980 77 81 71990 60 54 72000 88 38 72010 71 62 72020 73 75 72030 98 35 72040 81 59 72050 96 48 72060 74 56 72070 71 70 72080 63 70 72090 74 48 72100 79 51 72110 93 75 72120 82 62 72130 82 40 72140 71 89 72150 60 81 72160 65 81 72170 90 51 72180 74 43 72190 122 83 72200 74 43 72210 73 97 72220 57 43 72230 79 46 72240 81 67 72250 63 56 72260 74 64 72270 46 67 72280 69 48 72290 76 54 72300 74 70 72310 82 72 72320 65 102 72330 73 27 72340 96 64 72350 47 81 72360 68 70 72370 65 89 72380 63 54 72390 90 81 72400 93 46 72410 120 107 72420 109 54 72430 92 72 72440 79 72 72450 81 72 72460 98 75 72470 103 43 72480 77 83 72490 109 89 72500 74 62 72510 52 59 72520 87 64 72530 81 51 72540 133 102 72550 51 137 72560 68 91 72570 62 83 72580 55 86 72590 81 75 72600 84 72 72610 74 81 72620 93 67 72630 112 123 72640 76 142 72650 90 64 72660 60 70 72670 93 89 72680 58 86 72690 58 59 72700 57 54 72710 65 91 72720 58 99 72730 74 89 72740 71 67 72750 66 72 72760 85 70 72770 55 94 72780 79 51 72790 77 83 72800 82 110 72810 92 78 72820 93 67 72830 87 153 72840 81 78 72850 109 83 72860 82 75 72870 76 113 72880 65 46 72890 101 107 72900 90 70 72910 98 9999 72920 106 9999 72930 92 9999 72940 79 9999 72950 69 9999 72960 65 9999 72970 84 9999 72980 74 9999 72990 88 9999 73000 73 9999 73010 74 9999 73020 57 9999 73030 90 9999 73040 101 9999 73050 88 9999 73060 90 9999 73070 71 9999 73080 96 9999 73090 65 9999 73100 81 9999 73110 60 9999 73120 46 9999 73130 77 9999 73140 57 9999 73150 9999 9999 73160 9999 9999 73170 9999 9999 73180 9999 9999 73190 9999 9999 73200 9999 9999 73210 9999 9999 73220 9999 9999 73230 9999 9999 73240 9999 9999 73250 9999 9999 73260 9999 9999 73270 9999 9999 73280 9999 9999 73290 9999 9999 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125 9999 73950 71 9999 73960 79 9999 73970 133 9999 73980 55 105 73990 115 115 74000 98 64 74010 57 75 74020 81 140 74030 95 38 74040 79 62 74050 90 121 74060 69 75 74070 71 64 74080 55 81 74090 55 83 74100 87 81 74110 84 78 74120 58 72 74130 57 56 74140 85 48 74150 47 86 74160 85 78 74170 96 62 74180 81 70 74190 69 75 74200 82 83 74210 82 91 74220 111 94 74230 93 35 74240 128 62 74250 74 102 74260 57 51 74270 96 62 74280 63 62 74290 62 75 74300 71 9999 74310 66 9999 74320 79 9999 74330 81 9999 74340 60 9999 74350 68 9999 74360 71 9999 74370 88 9999 74380 82 9999 74390 66 9999 74400 114 9999 74410 9999 9999 74420 9999 9999 74430 9999 9999 74440 9999 9999 74450 9999 9999 74460 9999 9999 74470 9999 9999 74480 9999 9999 74490 9999 9999 74500 9999 9999 74510 9999 9999 74520 9999 9999 74530 9999 9999 74540 9999 9999 74550 9999 9999 74560 9999 9999 74570 9999 9999 74580 9999 9999 74590 9999 9999 74600 9999 9999 74610 9999 9999 74620 9999 9999 74630 9999 9999 74640 9999 9999 74650 9999 9999 74660 9999 9999 74670 9999 9999 74680 9999 9999 74690 9999 9999 74700 9999 9999 74710 9999 9999 74720 9999 9999 74730 9999 9999 74740 9999 9999 74750 9999 9999 74760 9999 9999 74770 9999 9999 74780 9999 9999 74790 9999 9999 74800 9999 9999 74810 9999 9999 74820 9999 9999 74830 9999 9999 74840 9999 9999 74850 9999 9999 74860 9999 9999 74870 9999 9999 74880 9999 9999 74890 9999 9999 74900 9999 9999 74910 9999 9999 74920 9999 9999 74930 9999 9999 74940 9999 9999 74950 9999 9999 74960 9999 9999 74970 9999 9999 74980 9999 9999 74990 9999 9999 75000 9999 9999 75010 9999 9999 75020 9999 9999 75030 9999 9999 75040 9999 9999 75050 9999 9999 75060 9999 9999 75070 9999 9999 75080 152 9999 75090 114 9999 75100 152 9999 75110 152 9999 75120 171 9999 75130 131 9999 75140 133 9999 75150 109 9999 75160 66 9999 75170 68 9999 75180 122 9999 75190 123 9999 75200 88 9999 75210 115 89 75220 164 72 75230 120 91 75240 114 70 75250 88 102 75260 115 38 75270 93 78 75280 68 70 75290 103 78 75300 74 67 75310 92 113 75320 92 86 75330 66 78 75340 107 97 75350 96 48 75360 87 56 75370 84 97 75380 79 56 75390 88 67 75400 95 35 75410 71 62 75420 126 94 75430 95 123 75440 88 54 75450 81 72 75460 88 72 75470 112 107 75480 92 97 75490 101 97 75500 77 67 75510 62 40 75520 60 70 75530 55 62 75540 52 75 75550 58 56 75560 69 59 75570 57 46 75580 62 62 75590 92 64 75600 92 51 75610 52 64 75620 81 70 75630 41 78 75640 73 46 75650 84 72 75660 85 83 75670 65 99 75680 69 81 75690 81 56 75700 82 62 75710 58 67 75720 96 72 75730 55 24 75740 60 70 75750 79 56 75760 71 70 75770 82 99 75780 58 67 75790 76 56 75800 77 54 75810 63 54 75820 58 70 75830 71 72 75840 90 105 75850 60 59 75860 41 94 75870 58 110 75880 62 97 75890 92 43 75900 77 89 75910 71 78 75920 41 59 75930 62 48 75940 57 59 75950 77 48 75960 65 72 75970 74 56 75980 111 59 75990 92 54 76000 69 48 76010 60 46 76020 65 48 76030 55 105 76040 60 83 76050 60 62 76060 85 94 76070 95 62 76080 62 43 76090 46 64 76100 49 59 76110 103 70 76120 54 54 76130 47 91 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