173 1001 Lloyd, Steven; Kusterer, Thomas; Swartz, William H.; Anderson, Donald The Johns Hopkins University Applied Physics Laboratory Photodissociation rate coefficients for the ER-2 flight track POLARIS 1 1 1997 09 14 1999 04 05 0 Time in seconds (UT) 92 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 1. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. 9999. Flight Altitude (km) Flight Latitude (km) Flight Longitude (km) Solar Zenith Angle (degrees) Temperature (degrees K) Reflectivity (0.0 - 1.0) Cloud Pressure (mbar) Cloud Height (km) Cloud Fraction Terrain Pressure (mbar) Terrain Height (km) Total Column Ozone above terrain (Dobsons) Total Column Ozone above cloud (Dobsons) Total Ozone above ER-2 (Dobsons) Slant O3 Column (integrated along refracted path, DU) O2 --hv(partial)--> O(3P) + O(3P) Partial J-value, 175-204 nm, DeMajistre/Minschwaner: recalculated parameters O2 --hv(partial)--> O(3P) + O(3P) JPL 97, Partial J-value, Herzberg cont., 205-240 nm O2 --hv--> O(3P) + O(3P) Total J-value O3 --hv--> O2 + O(3P) JPL 94 WMO/Molina&Molina temp-dep CS, JPL 97 t-d QY O3 --hv--> O2 + O(1D) JPL 94 WMO/Molina&Molina t-d CS, JPL 97 t-d QY HO2 --hv--> OH + H JPL 97 H2O --hv--> H + OH JPL 97 H2O2 --hv--> OH + OH JPL 97, analytic t-d CS, 190-350 nm NO2 --hv--> NO + O(3P) JPL 97, temp-dep CS and QY NO3 --hv(partial)--> Products Graham and Johnston 1978 CS, 370-645 nm only NO3 --hv(partial)--> Products JPL 97, 600-670 nm only NO3 --hv--> Products Combined CS 370-670 nm N2O --hv--> N2 + O(1D) JPL 97, analytic temp-dep CS N2O5 --hv--> NO2 + NO3 JPL 97, analytic CS for 285-380 HONO --hv--> OH + NO JPL 97 HONO2 --hv--> OH + NO2 JPL 94, Burkholder & Ravishankara temperature-dependent cross sections HO2NO2 --hv--> HO2 + NO2 JPL 97 CH2O --hv--> H + CHO JPL 97 CH2O --hv--> H2 + CO JPL 97 CH3O2 --hv--> Products JPL 97 C2H5O2 --hv--> Products JPL97 CH3OOH --hv--> Products JPL 97 CH3C(O)O2NO2 --hv--> Products JPL 97 temp-dep Cross Sections Cl2 --hv--> Cl + Cl JPL 97 temp-dep Cross Sections ClO --hv--> Cl + O(3P) JPL 97 derived analytic CS, 220-330 nm ClO --hv--> Cl + O(3P) JPL 94, above 250 nm only ClOO --hv--> ClO + O(3P) JPL 97 OClO --hv--> ClO + O(3P) JPL 94, data digitized and binned from Ravishankara Cl2O --hv--> Products JPL97 ClOOCl --hv--> Products JPL 97 **(ClO)2 --hv--> Cl + ClOO Burkholder, 210-425 nm Cl2O3 --hv--> Products JPL97 Cl2O4 --hv--> Products JPL97 Cl2O6 --hv--> Products JPL97 HCl --hv--> H + Cl JPL 97 HOCl --hv--> OH + Cl JPL 97 FNO --hv--> F + NO JPL 97 ClNO --hv--> Cl + NO JPL 97 ClNO2 --hv--> Products JPL 97 ClONO --hv--> Products JPL97 ClONO2 --hv--> Cl + NO3 JPL 97, Analytic Temp-Dep CS, QY ClONO2 --hv--> ClO + NO2 JPL 97, Analytic Temp-Dep CS, QY CCl4 --hv--> Products JPL97 CCl3F --hv--> Products JPL97 Temp-Dep Cross Sections CCl2F2 --hv--> Products JPL97 Temp-Dep Cross Sections CF2ClCFCl2 --hv--> Products JPL97 Temp-Dep Cross Sections CF2ClCF2Cl --hv--> Products JPL97 Temp-Dep Cross Sections CF3CF2Cl --hv--> Products JPL97 CCl2O --hv--> Products JPL97 CClFO --hv--> Products JPL97 CF2O --hv--> Products JPL97 CH3Cl --hv--> Products JPL97 Temp-Dep Cross Sections CH3CCl3 --hv--> Products JPL97 Temp-Dep Cross Sections CHClF2 --hv--> Products JPL97 Temp-Dep Cross Sections CH3CF2Cl --hv--> Products JPL97 CF3CHCl2 --hv--> Products JPL97 CF3CHFCl --hv--> Products JPL97 CH3CFCl2 --hv--> Products JPL97 CF3CF2CHCl2 --hv--> Products JPL97 CF2ClCF2CHFCl --hv--> Products JPL97 CH3OCl --hv--> Products JPL 97 BrO --hv--> Br + O(3P) JPL 97 HOBr --hv--> Products JPL97 BrONO2 --hv--> BrO + NO2 JPL 97 CS and QY BrONO2 --hv--> Br + NO3 JPL 97 CS and QY **BrONO2 --hv--> Br + NO3 JPL 94 BrCl --hv--> Br + Cl JPL 97 analytic cross section CH3Br --hv--> Products JPL97 CHBr3 --hv--> Products JPL97 analytic cross section CF3Br --hv--> Products JPL97 CF2Br2 --hv--> Products JPL97 CF2BrCF2Br --hv--> Products JPL97 CF2ClBr --hv--> Products JPL97 CF3I --hv--> CF3 + I JPL97 OCS --hv--> CO + S JPL97 Temp-Dep Cross Sections NO2 --hv--> NO2* Excited state NO2 (no photolysis), t-d CS/QY below 425 nm SO2 --hv--> Products MODTRAN3 1 *** Final Data *** 60 This file tabulates photolysis rate coefficients (J-values) along the ER-2 flight track, based on the radiative transfer codes developed by Anderson, DeMajistre, Lloyd and Kusterer, and discussed in Anderson and Meier (1982), Anderson (1983), Anderson and Lloyd (1990), Gao et al. (1997) and Swartz et al. (submitted 1999). The direct solar deposition and single scattering from the surface are calculated in a spherical refracting atmosphere, and the multiple scattering component is calculated using a plane parallel model. Extensive comparisons have shown that this algorithm provides reliable estimates of the radiation field for solar zenith angles of up to 95 degrees for all but extreme volcanic conditions. Aerosol climatologies are taken from the Air Force Geophysics Laboratory (now Phillips Lab) Handbook of Geophysics, as used in MODTRAN, LOWTRAN, etc. Observations of the volcanically quiescent period during POLARIS indicate the use of background aerosol distributions is appropriate for the troposphere, stratosphere, and above. The climatology for pressure, temperature, and ozone is compiled from balloon ozonesondes taken at Fairbanks, Alaska during the POLARIS campaigns (Jaffe, Simpson and Kelley, see "Related Measurements" under the POLARIS Web homepage), and is available from the APL group upon request. The temperature at the ER-2 altitude is taken from the ER-2's MMS (MM) file. One composite profile consisting of six ozonesonde measurements has been compiled for each deployment. Ozone profiles are scaled to Earth Probe TOMS total ozone along the ER-2 flight track contained in the EP97mmdd.EA1 files, using the profile itself as a weighting function (i.e., most changes in ozone occur near the ozone peak, and the troposphere and upper stratosphere do not vary significantly). In an effort to most accurately apply the TOMS ozone and reflectivity algorithm in our radiative transfer code, we have adopted the following approach to handling surface albedo/reflectivity and cloud top/terrain heights. If the TOMS UV effective reflectivity at 360 nm is less than 0.08, this albedo is used and applied to the terrain height (converted from pressure to geometric altitude from the EP97mmdd.EA1 files). If the reflectivity is above 0.80, this albedo is used and applied to the cloud top height (the ISSCP climatological cloud height used in the TOMS version 7 retrieval algorithm, also from the EP97mmdd.EA1 file, converted from pressure to geometric altitude). If the reflectivity is between 0.08 and 0.80, two calculations are performed, one at the terrain height with an albedo of 0.08 (slightly larger than for open ocean, but typical for terrain in the near UV) and another at the cloud top height with an albedo of 0.80, and the TOMS cloud fraction from the EP97mmdd.EA1 file is used to provided a weighted average of the two calculations, yielding the total J-values. If the surface climatology used in the TOMS retrieval indicates that there is a greater than 50/50 chance of snow or ice on the ground, the reflectivities are re-calculated accordingly (see NASA/TP-1998-206895, Earth Probe TOMS Data Product User's Guide for more details). Preliminary comparisons with CPFM partial column ozone above the flight altitude and the CPFM 600-nm "albedo" channel show good general agreement. The Earth Probe TOMS footprint in the nadir is approximately 24 km on the ground. As expected, the CPFM data shown finer spatial variability not seen in the TOMS data. Cross sections are taken from the JPL97 compilation of cross sections used in photochemical modeling, unless otherwise indicated. A parameterization of the solar transmittance through the Schumann-Runge bands (175-204 nm) was developed by DeMajistre, based on the work of Minschwaner. This code calculates the radiation field over the wavelength range 175-850 nm. Each radiation field calculation generates the actinic flux for each altitude layer (0-120 km) at every wavelength (50-wavenumber bins 175-298 nm, 0.5-nm bins 298-320 nm, and 5-nm bins 320-850 nm). The results are interpolated to the exact altitude and solar zenith angle of the ER-2 along the flight track. Another calculation is generated each time the total ozone changes by more than 5 Dobson Units, the effective cloud height changes by more than 0.5 km, or the UV effective reflectivity changes by more than 2 percent, and the results are interpolated between points. The sometimes "boxy" appearance of the results arises from the sparse TOMS observations along the flight track, and the occasional oscillation between adjacent TOMS observations. 4.71400e+04 2.6687e-01 6.4840e+01 -1.4760e+02 1.0280e+02 2.8025e+02 1.600e-02 5.066e+02 5.476e+00 0.000e+00 9.829e+02 2.020e-01 2.6340e+02 2.6340e+02 2.6332e+02 0.0000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 0.00000e+00 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