25 1001 K.K. Perkins (kathy@huarp.harvard.edu), E.J. Lanzendorf, and J.G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 Harvard NO2 SOLVE 1 1 2000 03 11 2001 07 27 0 Elapsed time (sec) from 0 GMT on flight day 1 1.0 999999.9 NO2 Volume Mixing Ratio (pptv) 8 FINAL DATA Estimated Accuracy (2 sigma): +/- 20 percent Estimated Zero Offset error (2 sigma): + 35 /- 10 ppt NO2 measurements during deep vortex flights with high ClO concentrations suggest a systematic offset of ~10 to 15 ppt ppt. We recommend accounting for this offset in the analysis of SOLVE data. For more information on flight-specific errors or instrument specifics, please contact the investigators. 2 ********** FINAL DATA ********** Time NO2 29765.25 37.3 29780.25 62.0 29800.25 35.5 29815.25 45.4 29825.25 20.7 29835.25 44.2 29850.25 50.2 29870.25 22.4 29885.25 11.1 29895.25 21.9 29905.25 39.4 29920.25 29.2 29940.25 34.8 29955.25 39.4 29965.25 34.1 29975.25 36.9 29990.25 31.2 30010.25 32.0 30025.25 19.6 30035.25 29.7 30045.25 28.4 30176.25 23.1 30191.25 7.5 30211.25 21.1 30226.25 35.4 30236.25 27.5 30246.25 30.1 30261.25 24.6 30281.25 21.8 30296.25 28.9 30306.25 15.5 30316.25 22.8 30331.25 16.4 30351.25 22.7 30366.25 17.9 30376.25 31.7 30386.25 21.4 30401.25 17.9 30421.25 9.5 30436.25 25.5 30446.25 25.4 30456.25 17.6 30587.25 9.5 30602.25 22.6 30622.25 14.8 30637.25 18.6 30647.25 10.6 30657.25 17.0 30672.25 8.3 30692.25 23.6 30707.25 12.8 30717.25 14.2 30727.25 17.7 30742.25 12.1 30762.25 4.4 30777.25 23.0 30787.25 17.9 30797.25 15.7 30812.25 11.1 30832.25 19.5 30847.25 15.7 30857.25 14.4 30867.25 16.0 30882.25 16.9 30902.25 6.2 30927.25 21.7 30937.25 18.5 30952.25 20.8 30972.25 14.0 30987.25 21.6 30997.25 9.2 31007.25 17.2 31022.25 10.6 31042.25 10.7 31057.25 13.6 31067.25 4.6 31077.25 14.2 31092.25 13.3 31112.25 7.8 31127.25 24.0 31137.25 16.9 31147.25 8.1 31162.25 18.7 31182.25 16.8 31197.25 10.0 31207.25 12.6 31217.25 14.5 31232.25 12.5 31252.25 14.9 31267.25 15.5 31277.25 6.2 31287.25 13.0 31302.25 10.4 31322.25 18.2 31337.25 8.5 31347.25 10.4 31357.25 6.7 31372.25 5.3 31392.25 11.1 31407.25 11.7 31417.25 3.4 31427.25 15.1 31442.25 7.0 31462.25 7.4 31477.25 13.4 31487.25 5.9 31497.25 0.3 31512.25 9.4 31532.25 18.9 31547.25 15.3 31557.25 14.9 31567.25 16.1 31582.25 21.9 31602.25 19.4 31617.25 11.3 31627.25 11.7 31637.25 16.3 31652.25 17.2 31672.25 16.2 31687.25 9.5 31697.25 18.7 31707.25 19.8 31722.25 15.5 31742.25 17.8 31757.25 11.4 31767.25 17.0 31777.25 10.3 31792.25 19.9 31812.25 15.8 31827.25 18.9 31837.25 18.0 31847.25 11.4 31862.25 7.3 31882.25 10.7 31897.25 14.1 31907.25 7.5 31917.25 14.2 31932.25 8.4 31952.25 4.9 31967.25 14.9 31977.25 5.7 31987.25 2.9 32002.25 12.5 32022.25 9.0 32037.25 2.2 32047.25 14.9 32057.25 10.9 32072.25 12.0 32092.25 16.0 32107.25 10.1 32117.25 22.8 32127.25 14.5 32142.25 16.7 32162.25 13.7 32177.25 12.3 32187.25 12.6 32197.25 19.1 32212.25 19.9 32232.25 22.6 32247.25 20.0 32257.25 16.7 32267.25 7.0 32282.25 15.6 32302.25 17.5 32317.25 15.3 32327.25 18.0 32337.25 21.6 32352.25 20.3 32372.25 11.6 32387.25 20.8 32397.25 10.8 32407.25 21.8 32422.25 27.8 32442.25 20.1 32457.25 19.3 32467.25 22.0 32477.25 22.8 32492.25 16.9 32628.25 28.0 32643.25 30.9 32663.25 39.6 32678.25 57.3 32688.25 86.0 32698.25 93.9 32713.25 64.7 32733.25 44.4 32748.25 39.2 32758.25 37.2 32768.25 28.3 32783.25 24.6 32803.25 29.3 32818.25 29.1 32828.25 28.6 32838.25 28.6 32853.25 22.5 32873.25 22.5 32888.25 11.5 32898.25 20.0 32908.25 16.7 32923.25 16.9 32943.25 18.3 32958.25 25.1 32968.25 23.8 32978.25 25.8 32993.25 22.4 33013.25 31.6 33028.25 36.6 33038.25 35.3 33048.25 36.6 33063.25 49.4 33083.25 40.7 33098.25 78.6 33108.25 76.5 33118.25 88.3 33133.25 75.4 33153.25 80.6 33168.25 75.4 33178.25 83.0 33188.25 76.6 33203.25 75.9 33223.25 80.0 33238.25 106.5 33248.25 97.9 33258.25 112.8 33273.25 115.7 33293.25 121.1 33308.25 116.0 33318.25 110.6 33328.25 102.8 33343.25 128.1 33363.25 120.0 33378.25 113.3 33388.25 109.7 33398.25 119.0 33413.25 121.0 33433.25 119.3 33448.25 131.1 33458.25 133.1 33468.25 125.3 33483.25 126.7 33503.25 116.0 33518.25 126.7 33528.25 132.4 33538.25 131.6 33553.25 125.8 33573.25 147.1 33588.25 145.8 33598.25 136.1 33608.25 156.6 33623.25 134.3 33643.25 143.0 33658.25 131.1 33668.25 140.9 33678.25 148.4 33693.25 141.9 33713.25 151.4 33728.25 143.2 33738.25 140.4 33748.25 145.4 33763.25 139.0 33783.25 146.1 33798.25 144.9 33808.25 142.1 33818.25 136.0 33833.25 164.0 33853.25 148.8 33868.25 152.2 33878.25 153.3 33888.25 152.6 33903.25 140.0 33923.25 143.8 33938.25 152.5 33948.25 142.3 33958.25 140.6 33973.25 154.4 33993.25 150.6 34008.25 132.7 34018.25 140.3 34028.25 150.2 34043.25 141.0 34063.25 139.8 34078.25 152.5 34088.25 142.2 34098.25 141.4 34113.25 140.6 34133.25 157.9 34148.25 145.2 34158.25 164.2 34168.25 152.3 34183.25 152.5 34203.25 154.1 34218.25 143.2 34228.25 153.6 34238.25 156.9 34253.25 143.5 34273.25 169.6 34288.25 169.4 34298.25 162.5 34308.25 147.0 34323.25 158.8 34343.25 152.0 34358.25 160.4 34368.25 172.0 34378.25 164.9 34393.25 146.4 34413.25 163.5 34428.25 150.4 34438.25 147.4 34448.25 149.5 34463.25 164.2 34483.25 148.1 34498.25 160.6 34508.25 151.0 34518.25 165.4 34533.25 162.4 34553.25 162.7 34568.25 157.9 34578.25 159.6 34588.25 161.2 34603.25 153.2 34623.25 160.6 34638.25 170.3 34648.25 157.8 34658.25 184.1 34673.25 168.4 34693.25 131.1 34708.25 131.4 34718.25 123.1 34728.25 102.2 34743.25 85.3 34879.25 78.0 34894.25 69.3 34914.25 68.0 34929.25 68.1 34939.25 72.1 34949.25 71.9 34984.25 75.8 34999.25 66.7 35009.25 78.8 35019.25 81.6 35034.25 70.7 35054.25 73.5 35069.25 61.7 35079.25 76.3 35089.25 79.0 35104.25 87.8 35124.25 100.8 35139.25 88.8 35149.25 95.8 35159.25 105.8 35174.25 104.1 35194.25 114.7 35209.25 99.6 35219.25 111.1 35229.25 111.4 35244.25 116.6 35264.25 121.1 35279.25 132.6 35289.25 122.8 35299.25 142.0 35314.25 142.0 35334.25 136.2 35349.25 130.1 35359.25 132.6 35369.25 142.3 35384.25 126.7 35404.25 133.3 35419.25 117.3 35429.25 131.3 35439.25 137.3 35454.25 112.1 35474.25 129.6 35489.25 121.5 35499.25 120.7 35509.25 120.7 35524.25 114.8 35544.25 119.6 35559.25 123.3 35569.25 118.7 35579.25 124.2 35594.25 118.4 35614.25 116.4 35629.25 142.8 35639.25 137.2 35649.25 138.6 35664.25 135.1 35684.25 122.9 35700.25 132.5 35709.25 134.1 35719.25 114.7 35734.25 124.3 35754.25 135.3 35769.25 145.0 35779.25 125.9 35790.25 133.4 35805.25 127.8 35824.25 133.0 35839.25 127.4 35850.25 114.9 35860.25 111.2 35875.25 108.1 35894.25 100.9 35910.25 107.8 35920.25 104.7 35930.25 101.2 35945.25 107.6 35965.25 84.4 35980.25 105.7 35990.25 99.2 36000.25 112.1 36015.25 102.2 36035.25 98.6 36050.25 101.5 36060.25 103.4 36070.25 97.9 36085.25 114.9 36105.25 101.3 36120.25 95.8 36130.25 102.9 36140.25 102.3 36155.25 102.2 36175.25 96.7 36190.25 102.0 36200.25 100.7 36210.25 98.9 36225.25 95.0 36245.25 99.3 36260.25 114.1 36270.25 109.5 36280.25 100.6 36295.25 103.0 36315.25 114.4 36330.25 111.2 36340.25 98.3 36350.25 107.8 36365.25 112.5 36385.25 120.1 36400.25 115.5 36410.25 125.7 36420.25 125.2 36435.25 116.1 36455.25 118.2 36470.25 124.2 36480.25 146.0 36490.25 115.5 36505.25 123.1 36525.25 124.2 36540.25 125.7 36550.25 121.0 36560.25 129.6 36575.25 113.4 36595.25 114.0 36610.25 124.6 36620.25 108.9 36630.25 103.6 36645.25 125.3 36665.25 120.9 36680.25 122.7 36690.25 112.9 36700.25 112.2 36715.25 125.6 36735.25 116.3 36750.25 102.1 36760.25 106.2 36770.25 111.9 36785.25 123.5 36921.25 131.0 36936.25 130.8 36956.25 130.4 36971.25 126.4 36981.25 121.9 36991.25 122.2 37006.25 117.9 37026.25 123.1 37041.25 132.1 37051.25 122.1 37061.25 120.3 37076.25 117.8 37096.25 133.7 37111.25 133.5 37121.25 128.1 37131.25 130.8 37146.25 124.1 37166.25 124.9 37181.25 129.2 37191.25 124.8 37201.25 109.3 37216.25 119.1 37236.25 124.3 37251.25 140.3 37261.25 115.1 37271.25 127.3 37286.25 117.9 37306.25 102.7 37321.25 118.8 37331.25 120.8 37341.25 132.1 37356.25 119.9 37376.25 113.8 37391.25 109.8 37401.25 108.8 37411.25 111.7 37426.25 117.3 37446.25 98.3 37461.25 104.3 37471.25 105.0 37481.25 117.6 37496.25 92.8 37516.25 96.9 37531.25 105.0 37541.25 91.2 37551.25 109.2 37566.25 108.3 37586.25 107.5 37601.25 103.0 37611.25 114.7 37621.25 98.6 37636.25 119.0 37656.25 109.0 37671.25 94.4 37681.25 93.1 37691.25 95.7 37706.25 90.8 37726.25 107.9 37741.25 85.9 37751.25 107.2 37761.25 101.0 37776.25 111.5 37796.25 110.3 37811.25 109.8 37821.25 107.1 37831.25 109.9 37846.25 114.2 37866.25 93.8 37881.25 115.5 37891.25 125.5 37901.25 117.5 37916.25 120.7 37936.25 111.1 37951.25 127.8 37961.25 101.9 37971.25 109.6 37986.25 118.1 38006.25 111.8 38021.25 113.3 38031.25 120.9 38041.25 110.0 38056.25 125.8 38076.25 112.4 38091.25 114.5 38101.25 110.5 38111.25 125.9 38126.25 114.3 38146.25 111.5 38161.25 99.9 38171.25 110.3 38181.25 123.0 38196.25 121.6 38216.25 130.4 38231.25 114.5 38241.25 111.8 38251.25 110.2 38266.25 108.9 38286.25 104.6 38301.25 113.6 38311.25 118.1 38321.25 111.6 38336.25 106.3 38356.25 117.0 38371.25 117.0 38381.25 124.6 38391.25 108.6 38406.25 102.6 38426.25 101.7 38441.25 118.6 38451.25 122.9 38461.25 123.3 38476.25 118.3 38496.25 138.2 38511.25 126.0 38521.25 113.1 38531.25 126.8 38546.25 104.4 38581.25 132.2 38591.25 112.9 38601.25 122.2 38616.25 129.6 38636.25 116.5 38651.25 106.1 38661.25 112.1 38671.25 122.6 38686.25 113.2 38706.25 106.6 38721.25 95.7 38731.25 113.1 38741.25 106.6 38756.25 103.0 38776.25 119.7 38791.25 121.8 38801.25 124.2 38811.25 116.2 38826.25 111.0 38846.25 120.0 38861.25 122.0 38871.25 115.1 38881.25 125.9 38896.25 113.7 38916.25 124.3 38931.25 106.4 38941.25 103.2 38951.25 116.3 38966.25 124.7 38986.25 115.5 39001.25 111.5 39011.25 98.3 39021.25 111.4 39036.25 113.0 39172.25 128.8 39187.25 140.6 39207.25 145.6 39222.25 125.4 39232.25 132.0 39242.25 161.1 39257.25 156.1 39277.25 139.3 39292.25 135.2 39302.25 152.5 39312.25 156.2 39327.25 144.4 39347.25 153.2 39362.25 161.8 39372.25 159.9 39382.25 165.3 39397.25 156.7 39417.25 167.1 39432.25 146.1 39442.25 152.2 39452.25 140.4 39467.25 150.8 39487.25 146.6 39502.25 131.5 39512.25 145.5 39522.25 132.8 39537.25 144.2 39557.25 155.8 39572.25 155.4 39582.25 159.8 39592.25 154.0 39607.25 146.4 39627.25 146.6 39642.25 108.7 39652.25 117.8 39662.25 98.8 39677.25 108.5 39697.25 95.5 39712.25 100.5 39722.25 78.9 39732.25 87.8 39747.25 64.5 39767.25 64.6 39782.25 45.0 39792.25 64.1 39802.25 71.3 39817.25 61.2 39837.25 62.1 39852.25 64.3 39862.25 64.1 39872.25 54.9 39887.25 72.3 39907.25 77.5 39922.25 94.6 39932.25 75.7 39942.25 79.7 39957.25 63.4 39977.25 64.0 39992.25 81.2 40002.25 73.0 40012.25 72.4 40027.25 71.8 40047.25 83.9 40062.25 62.7 40072.25 72.7 40082.25 65.2 40097.25 60.4 40117.25 39.5 40132.25 38.7 40142.25 54.1 40152.25 43.2 40167.25 52.0 40187.25 62.6 40202.25 65.0 40212.25 47.2 40222.25 49.5 40237.25 55.5 40257.25 64.3 40272.25 46.5 40282.25 51.6 40292.25 37.9 40307.25 51.7 40327.25 51.2 40342.25 55.2 40352.25 42.5 40362.25 42.0 40377.25 57.5 40397.25 59.4 40412.25 49.6 40422.25 53.3 40432.25 49.2 40447.25 75.7 40467.25 55.2 40482.25 70.2 40492.25 67.3 40502.25 69.9 40517.25 59.3 40537.25 65.7 40552.25 78.6 40562.25 69.0 40572.25 68.5 40587.25 73.3 40607.25 81.1 40622.25 80.8 40632.25 79.0 40642.25 64.8 40657.25 86.1 40677.25 67.7 40692.25 57.3 40702.25 59.1 40712.25 66.0 40727.25 64.1 40747.25 74.2 40762.25 93.5 40772.25 86.3 40782.25 99.8 40797.25 131.2 40817.25 124.9 40832.25 121.5 40842.25 130.6 40852.25 138.1 40867.25 133.6 40887.25 123.0 40912.25 116.4 40922.25 104.7 40937.25 112.7 40957.25 104.9 40972.25 111.1 40982.25 108.7 40992.25 96.7 41007.25 82.9 41027.25 86.4 41042.25 95.8 41052.25 124.6 41062.25 107.9 41077.25 124.5 41213.25 124.5 41228.25 117.4 41248.25 125.7 41263.25 118.1 41273.25 101.7 41283.25 117.6 41298.25 101.8 41318.25 111.6 41333.25 117.2 41343.25 109.8 41353.25 108.6 41368.25 116.3 41388.25 123.9 41403.25 125.9 41413.25 122.7 41423.25 110.4 41438.25 114.0 41458.25 127.0 41473.25 117.4 41483.25 135.3 41493.25 132.1 41508.25 132.9 41528.25 115.5 41543.25 135.1 41553.25 127.1 41563.25 136.7 41578.25 139.4 41598.25 122.2 41613.25 152.1 41623.25 139.3 41633.25 142.7 41648.25 143.0 41668.25 130.8 41683.25 123.3 41693.25 150.5 41703.25 134.5 41718.25 133.1 41738.25 128.7 41753.25 135.1 41763.25 153.4 41773.25 133.8 41788.25 128.3 41808.25 142.4 41823.25 155.2 41833.25 136.2 41843.25 149.0 41858.25 132.8 41878.25 127.1 41893.25 151.3 41903.25 145.9 41913.25 141.4 41928.25 136.4 41948.25 133.7 41963.25 137.1 41973.25 128.2 41983.25 155.4 41998.25 134.5 42018.25 143.7 42033.25 148.2 42043.25 141.6 42053.25 129.5 42068.25 134.1 42088.25 135.2 42103.25 137.2 42113.25 138.2 42123.25 142.7 42138.25 152.4 42158.25 127.0 42173.25 137.5 42183.25 121.7 42193.25 140.3 42208.25 131.3 42228.25 138.7 42243.25 131.8 42253.25 138.7 42263.25 129.4 42278.25 141.7 42298.25 145.1 42313.25 145.3 42323.25 122.2 42333.25 146.8 42348.25 143.1 42368.25 135.9 42383.25 164.8 42393.25 149.5 42403.25 139.1 42418.25 149.0 42438.25 160.1 42453.25 163.4 42463.25 169.5 42488.25 150.1 42508.25 159.6 42523.25 151.3 42533.25 158.5 42543.25 180.2 42558.25 182.3 42578.25 182.4 42593.25 165.7 42603.25 171.8 42613.25 166.8 42628.25 170.1 42648.25 166.4 42663.25 181.7 42673.25 184.5 42683.25 166.2 42698.25 150.8 42718.25 181.3 42733.25 178.7 42743.25 168.2 42753.25 173.0 42768.25 182.1 42788.25 189.7 42803.25 200.6 42813.25 203.2 42823.25 204.3 42838.25 203.8 42858.25 197.7 42873.25 207.1 42883.25 211.5 42893.25 207.3 42908.25 215.5 42928.25 215.4 42943.25 224.8 42953.25 209.6 42963.25 215.0 42978.25 207.1 42998.25 207.6 43013.25 190.9 43023.25 190.5 43033.25 193.1 43048.25 191.6 43068.25 195.1 43083.25 203.1 43093.25 204.1 43103.25 201.0 43118.25 193.1 43138.25 196.4 43153.25 190.4 43163.25 210.9 43173.25 201.8 43188.25 204.0 43208.25 211.2 43223.25 197.7 43233.25 213.2 43243.25 213.1 43258.25 200.5 43278.25 185.0 43293.25 217.8 43303.25 204.4 43313.25 192.4 43328.25 198.6 43464.25 209.0 43479.25 223.3 43499.25 215.3 43514.25 224.3 43524.25 215.6 43534.25 201.1 43549.25 208.6 43569.25 210.8 43584.25 218.5 43594.25 218.7 43604.25 201.7 43619.25 213.6 43639.25 198.9 43654.25 205.1 43664.25 204.9 43674.25 205.6 43689.25 208.4 43709.25 202.3 43724.25 209.5 43734.25 192.1 43744.25 221.4 43759.25 208.2 43779.25 213.9 43794.25 210.8 43804.25 202.5 43814.25 214.7 43829.25 200.2 43849.25 201.6 43864.25 198.8 43874.25 212.2 43884.25 211.4 43899.25 188.8 43919.25 215.0 43934.25 192.8 43944.25 200.8 43954.25 203.5 43969.25 194.9 43989.25 209.1 44004.25 207.9 44014.25 210.0 44024.25 201.3 44039.25 219.4 44059.25 209.2 44074.25 199.7 44084.25 207.0 44094.25 211.9 44109.25 205.7 44129.25 212.6 44144.25 217.0 44154.25 182.4 44164.25 187.1 44179.25 193.6 44199.25 205.2 44214.25 196.1 44224.25 206.3 44234.25 206.3 44249.25 204.5 44269.25 218.5 44284.25 226.7 44294.25 229.2 44304.25 208.2 44319.25 189.2 44339.25 203.0 44354.25 208.2 44364.25 197.1 44374.25 201.9 44389.25 210.1 44409.25 202.4 44424.25 217.3 44434.25 213.2 44444.25 212.4 44459.25 215.1 44479.25 225.4 44494.25 231.9 44504.25 226.8 44514.25 231.2 44529.25 221.7 44549.25 206.4 44564.25 232.7 44574.25 219.2 44584.25 221.2 44599.25 220.2 44619.25 233.0 44634.25 212.5 44644.25 192.3 44654.25 184.0 44669.25 203.8 44689.25 180.3 44704.25 176.4 44714.25 165.0 44724.25 159.2 44739.25 161.3 44759.25 182.4 44774.25 171.2 44784.25 156.8 44794.25 164.8 44809.25 172.5 44829.25 144.4 44844.25 158.2 44854.25 158.0 44864.25 162.0 44879.25 155.2 44899.25 160.0 44914.25 162.3 44924.25 165.2 44934.25 157.8 44949.25 169.1 44969.25 180.3 44984.25 193.0 44994.25 169.3 45004.25 171.6 45019.25 182.8 45039.25 176.4 45054.25 179.4 45064.25 188.0 45074.25 183.3 45089.25 203.5 45109.25 209.5 45124.25 216.2 45134.25 192.7 45144.25 196.1 45159.25 212.0 45179.25 176.5 45194.25 181.7 45204.25 200.6 45214.25 188.2 45229.25 204.3 45249.25 178.4 45264.25 206.1 45274.25 194.3 45284.25 187.4 45299.25 184.3 45319.25 202.6 45334.25 160.9 45344.25 162.1 45354.25 155.6 45370.25 127.3 45506.25 86.9 45521.25 103.0 45541.25 131.4 45556.25 140.4 45566.25 168.8 45576.25 168.2 45591.25 184.4 45610.25 192.0 45626.25 136.4 45636.25 121.4 45645.25 105.4 45660.25 51.3 45681.25 49.1 45696.25 70.8 45706.25 60.5 45716.25 65.4 45731.25 57.4 45751.25 45.9 45766.25 48.5 45776.25 51.3 45786.25 44.1 45801.25 41.1 45821.25 35.1 45836.25 28.3 45846.25 37.7 45856.25 38.3 45871.25 37.8 45891.25 32.2 45906.25 42.0 45916.25 23.4 45926.25 27.2 45941.25 33.1 45961.25 29.2 45976.25 33.7 45986.25 26.9 45996.25 23.5 46011.25 25.5 46031.25 18.0 46046.25 27.6 46056.25 23.8 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