44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 03 11 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 29166.25 -19.4 999999.9 999999.9 29201.25 -10.3 999999.9 999999.9 29236.25 1.3 999999.9 999999.9 29271.25 -1.2 999999.9 999999.9 29306.25 1.8 999999.9 999999.9 29341.25 -5.1 999999.9 999999.9 29376.25 2.0 999999.9 999999.9 29411.25 -1.7 999999.9 999999.9 29446.25 10.6 999999.9 999999.9 29481.25 19.8 999999.9 999999.9 29516.25 7.8 999999.9 999999.9 29551.25 15.7 999999.9 999999.9 29586.25 34.7 999999.9 999999.9 29621.25 60.1 999999.9 999999.9 29656.25 35.2 999999.9 999999.9 29691.25 54.6 999999.9 999999.9 29726.25 51.4 999999.9 999999.9 29761.25 999999.9 999999.9 999999.9 29796.25 86.4 999999.9 999999.9 29831.25 92.9 999999.9 999999.9 29866.25 142.7 999999.9 999999.9 29901.25 147.5 999999.9 999999.9 29936.25 155.9 999999.9 999999.9 29971.25 222.7 999999.9 999999.9 30006.25 234.2 999999.9 999999.9 30041.25 244.0 999999.9 999999.9 30076.25 269.8 999999.9 999999.9 30111.25 306.7 999999.9 999999.9 30146.25 360.0 999999.9 999999.9 30181.25 333.3 999999.9 439.2 30216.25 349.0 999999.9 999999.9 30251.25 330.6 81.6 999999.9 30286.25 361.2 86.2 999999.9 30321.25 414.3 999999.9 999999.9 30356.25 390.6 999999.9 999999.9 30391.25 453.7 999999.9 999999.9 30426.25 446.0 999999.9 999999.9 30461.25 444.4 134.7 999999.9 30496.25 419.8 103.9 999999.9 30531.25 482.5 104.5 999999.9 30566.25 511.6 999999.9 626.2 30601.25 546.3 999999.9 522.5 30636.25 583.2 999999.9 999999.9 30671.25 687.5 146.4 999999.9 30706.25 763.6 180.2 999999.9 30741.25 766.7 999999.9 999999.9 30776.25 830.6 999999.9 999999.9 30811.25 820.5 999999.9 999999.9 30846.25 819.1 999999.9 999999.9 30881.25 960.2 999999.9 999999.9 30916.25 916.7 999999.9 999999.9 30951.25 950.7 999999.9 999999.9 30986.25 1022.9 999999.9 999999.9 31021.25 966.1 999999.9 999999.9 31056.25 980.4 999999.9 999999.9 31091.25 1012.2 999999.9 999999.9 31126.25 936.6 263.1 999999.9 31161.25 973.8 258.6 999999.9 31196.25 992.5 237.3 999999.9 31231.25 1012.3 999999.9 314.5 31266.25 1005.2 999999.9 999999.9 31301.25 998.2 999999.9 999999.9 31336.25 1027.9 248.7 999999.9 31371.25 1000.9 229.8 999999.9 31406.25 1034.0 999999.9 999999.9 31441.25 1076.1 999999.9 999999.9 31476.25 1121.8 999999.9 999999.9 31511.25 1096.8 999999.9 999999.9 31546.25 1048.2 243.5 999999.9 31581.25 1091.2 224.5 999999.9 31616.25 1024.5 236.3 999999.9 31651.25 1034.5 999999.9 282.2 31686.25 1081.2 999999.9 268.1 31721.25 1088.1 999999.9 999999.9 31756.25 1041.0 228.7 999999.9 31791.25 1044.0 221.3 999999.9 31826.25 1076.5 999999.9 999999.9 31861.25 1047.8 999999.9 999999.9 31896.25 1177.3 999999.9 999999.9 31931.25 963.5 999999.9 999999.9 31966.25 1066.5 220.9 999999.9 32001.25 992.7 229.4 999999.9 32036.25 991.4 211.7 999999.9 32071.25 956.9 999999.9 341.0 32106.25 1026.9 999999.9 442.4 32141.25 1056.8 999999.9 999999.9 32176.25 1009.7 190.2 999999.9 32211.25 1056.2 183.2 999999.9 32246.25 1124.4 999999.9 999999.9 32281.25 1115.2 999999.9 999999.9 32316.25 1106.3 999999.9 999999.9 32351.25 993.0 999999.9 999999.9 32386.25 1133.3 999999.9 999999.9 32421.25 1094.9 999999.9 999999.9 32456.25 1031.2 999999.9 999999.9 32491.25 1173.0 999999.9 999999.9 32526.25 1005.4 999999.9 999999.9 32561.25 989.9 999999.9 999999.9 32596.25 887.5 999999.9 999999.9 32631.25 879.0 164.0 999999.9 32666.25 470.6 114.2 999999.9 32701.25 451.3 53.8 999999.9 32736.25 606.0 999999.9 846.5 32771.25 669.7 999999.9 916.0 32806.25 737.7 999999.9 999999.9 32841.25 816.6 999999.9 999999.9 32876.25 805.4 89.4 999999.9 32911.25 869.1 999999.9 999999.9 32946.25 696.0 999999.9 999999.9 32981.25 654.6 999999.9 999999.9 33016.25 626.3 999999.9 999999.9 33051.25 502.1 73.6 999999.9 33086.25 264.9 42.6 999999.9 33121.25 269.4 21.3 999999.9 33156.25 285.9 999999.9 1102.6 33191.25 247.8 999999.9 1138.0 33226.25 185.8 999999.9 999999.9 33261.25 207.9 -6.2 999999.9 33296.25 192.7 16.5 999999.9 33331.25 142.9 999999.9 999999.9 33366.25 127.8 999999.9 999999.9 33401.25 155.5 999999.9 999999.9 33436.25 126.2 999999.9 999999.9 33471.25 125.3 34.4 999999.9 33506.25 124.0 17.9 999999.9 33541.25 108.1 2.4 999999.9 33576.25 121.4 999999.9 965.7 33611.25 108.8 999999.9 736.1 33646.25 100.5 999999.9 999999.9 33681.25 98.7 999999.9 999999.9 33716.25 80.9 -27.0 999999.9 33751.25 93.0 999999.9 999999.9 33786.25 79.3 999999.9 999999.9 33821.25 86.0 999999.9 999999.9 33856.25 116.3 999999.9 999999.9 33891.25 117.0 999999.9 999999.9 33926.25 155.4 999999.9 999999.9 33961.25 145.0 999999.9 999999.9 33996.25 138.6 999999.9 999999.9 34031.25 140.4 999999.9 999999.9 34066.25 128.3 999999.9 999999.9 34101.25 119.2 999999.9 999999.9 34136.25 127.4 34.2 999999.9 34171.25 139.5 14.7 999999.9 34206.25 151.2 10.0 999999.9 34241.25 89.8 999999.9 1062.3 34276.25 108.6 999999.9 957.2 34311.25 129.1 999999.9 999999.9 34346.25 120.2 999999.9 999999.9 34381.25 119.5 -21.6 999999.9 34416.25 121.2 999999.9 999999.9 34451.25 107.8 999999.9 999999.9 34486.25 99.9 999999.9 999999.9 34521.25 95.1 999999.9 999999.9 34556.25 93.2 5.5 999999.9 34591.25 115.8 -4.4 999999.9 34626.25 116.7 -12.4 999999.9 34661.25 129.0 999999.9 794.3 34696.25 156.5 999999.9 1188.1 34731.25 224.5 999999.9 999999.9 34766.25 267.2 -18.9 999999.9 34801.25 253.1 -20.4 999999.9 34836.25 295.3 999999.9 999999.9 34871.25 304.7 999999.9 999999.9 34906.25 305.9 999999.9 999999.9 34941.25 290.5 999999.9 999999.9 34976.25 296.0 40.6 999999.9 35011.25 258.0 7.9 999999.9 35046.25 295.4 17.0 999999.9 35081.25 257.5 999999.9 1063.9 35116.25 222.4 999999.9 1127.6 35151.25 185.2 999999.9 999999.9 35186.25 182.3 -46.3 999999.9 35221.25 156.5 -11.1 999999.9 35256.25 130.5 999999.9 999999.9 35291.25 102.8 999999.9 999999.9 35326.25 89.8 999999.9 999999.9 35361.25 103.5 999999.9 999999.9 35396.25 83.8 999999.9 999999.9 35431.25 76.5 999999.9 999999.9 35466.25 78.7 999999.9 999999.9 35501.25 79.1 999999.9 999999.9 35536.25 67.8 999999.9 999999.9 35571.25 79.6 999999.9 999999.9 35606.25 94.1 999999.9 999999.9 35641.25 60.1 28.4 999999.9 35676.25 79.8 2.9 999999.9 35711.25 63.8 12.0 999999.9 35746.25 64.1 999999.9 395.0 35781.25 59.3 999999.9 999999.9 35816.25 54.4 999999.9 999999.9 35851.25 23.8 -11.6 999999.9 35886.25 20.4 -15.7 999999.9 35921.25 35.0 999999.9 999999.9 35956.25 28.2 999999.9 999999.9 35991.25 21.3 999999.9 999999.9 36026.25 30.2 999999.9 999999.9 36061.25 26.7 8.1 999999.9 36096.25 26.2 2.0 999999.9 36131.25 30.7 -10.9 999999.9 36166.25 22.7 999999.9 150.8 36201.25 22.9 999999.9 154.8 36236.25 29.8 999999.9 999999.9 36271.25 26.7 999999.9 999999.9 36306.25 41.9 -2.9 999999.9 36341.25 21.9 999999.9 999999.9 36376.25 40.9 999999.9 999999.9 36411.25 19.1 999999.9 999999.9 36446.25 49.7 999999.9 999999.9 36481.25 22.6 7.4 999999.9 36516.25 37.4 8.6 999999.9 36551.25 32.0 -14.2 999999.9 36586.25 39.2 999999.9 239.9 36621.25 38.9 999999.9 218.3 36656.25 36.4 999999.9 999999.9 36691.25 40.9 -7.6 999999.9 36726.25 40.2 8.7 999999.9 36761.25 51.8 999999.9 999999.9 36796.25 30.7 999999.9 999999.9 36831.25 24.8 999999.9 999999.9 36866.25 45.0 999999.9 999999.9 36901.25 36.0 999999.9 999999.9 36936.25 59.3 999999.9 999999.9 36971.25 62.6 999999.9 999999.9 37006.25 59.8 999999.9 999999.9 37041.25 30.9 999999.9 999999.9 37076.25 29.0 999999.9 999999.9 37111.25 40.8 999999.9 999999.9 37146.25 40.3 21.4 999999.9 37181.25 36.9 9.7 999999.9 37216.25 53.5 12.7 999999.9 37251.25 37.1 999999.9 166.2 37286.25 28.6 999999.9 194.9 37321.25 41.7 999999.9 999999.9 37356.25 29.8 999999.9 999999.9 37391.25 34.2 2.9 999999.9 37426.25 21.1 999999.9 999999.9 37461.25 39.2 999999.9 999999.9 37496.25 34.2 999999.9 999999.9 37531.25 32.5 999999.9 999999.9 37566.25 26.7 10.4 999999.9 37601.25 20.1 13.7 999999.9 37636.25 16.7 3.9 999999.9 37671.25 26.6 999999.9 101.9 37706.25 7.3 999999.9 45.6 37741.25 34.0 999999.9 999999.9 37776.25 27.4 999999.9 999999.9 37811.25 30.9 -2.1 999999.9 37846.25 25.2 999999.9 999999.9 37881.25 21.6 999999.9 999999.9 37916.25 12.8 999999.9 999999.9 37951.25 25.9 999999.9 999999.9 37986.25 26.2 4.7 999999.9 38021.25 46.1 -2.4 999999.9 38056.25 40.9 -7.1 999999.9 38091.25 41.2 999999.9 156.8 38126.25 30.7 999999.9 170.7 38161.25 37.4 999999.9 999999.9 38196.25 47.3 999999.9 999999.9 38231.25 47.6 -7.3 999999.9 38266.25 55.3 999999.9 999999.9 38301.25 30.4 999999.9 999999.9 38336.25 41.7 999999.9 999999.9 38371.25 44.9 999999.9 999999.9 38406.25 46.1 999999.9 999999.9 38441.25 36.6 999999.9 999999.9 38476.25 54.1 999999.9 999999.9 38511.25 46.3 999999.9 999999.9 38546.25 32.4 999999.9 999999.9 38581.25 41.2 999999.9 999999.9 38616.25 58.1 999999.9 999999.9 38651.25 38.6 7.6 999999.9 38686.25 41.0 3.6 999999.9 38721.25 31.9 -0.8 999999.9 38756.25 40.6 999999.9 137.0 38791.25 36.1 999999.9 158.9 38826.25 52.4 999999.9 999999.9 38861.25 41.8 999999.9 999999.9 38896.25 59.2 6.3 999999.9 38931.25 52.9 999999.9 999999.9 38966.25 47.1 999999.9 999999.9 39001.25 53.0 999999.9 999999.9 39036.25 48.6 999999.9 999999.9 39071.25 67.6 8.7 999999.9 39106.25 86.6 1.1 999999.9 39141.25 81.5 -11.6 999999.9 39176.25 60.2 999999.9 354.5 39211.25 91.0 999999.9 293.9 39246.25 76.7 999999.9 999999.9 39281.25 60.1 999999.9 999999.9 39316.25 99.3 10.9 999999.9 39351.25 119.1 999999.9 999999.9 39386.25 87.5 999999.9 999999.9 39421.25 75.6 999999.9 999999.9 39456.25 78.9 999999.9 999999.9 39491.25 65.9 14.0 999999.9 39526.25 68.5 -10.5 999999.9 39561.25 68.8 8.3 999999.9 39596.25 81.4 999999.9 335.3 39631.25 33.6 999999.9 225.0 39666.25 39.6 999999.9 999999.9 39701.25 22.8 -2.4 999999.9 39736.25 12.8 -13.8 999999.9 39771.25 21.3 999999.9 999999.9 39806.25 4.6 999999.9 999999.9 39841.25 5.5 999999.9 999999.9 39876.25 3.3 999999.9 999999.9 39911.25 -1.8 999999.9 999999.9 39946.25 2.1 999999.9 999999.9 39981.25 15.3 999999.9 999999.9 40016.25 16.4 999999.9 999999.9 40051.25 3.3 999999.9 999999.9 40086.25 26.6 999999.9 999999.9 40121.25 4.8 999999.9 999999.9 40156.25 -17.8 -6.6 999999.9 40191.25 3.7 5.3 999999.9 40226.25 6.0 -2.6 999999.9 40261.25 -5.2 999999.9 999999.9 40296.25 7.7 999999.9 999999.9 40331.25 -0.9 999999.9 999999.9 40366.25 10.5 -4.2 999999.9 40401.25 8.6 8.4 999999.9 40436.25 17.4 999999.9 999999.9 40471.25 6.1 999999.9 999999.9 40506.25 13.2 999999.9 999999.9 40541.25 6.1 999999.9 999999.9 40576.25 23.7 19.6 999999.9 40611.25 24.6 13.5 999999.9 40646.25 23.8 25.9 999999.9 40681.25 8.4 999999.9 -21.9 40716.25 21.1 999999.9 18.3 40751.25 42.7 999999.9 999999.9 40786.25 56.4 22.8 999999.9 40821.25 77.2 14.3 999999.9 40856.25 73.5 999999.9 999999.9 40891.25 40.3 999999.9 999999.9 40926.25 33.2 999999.9 999999.9 40961.25 48.3 999999.9 999999.9 40996.25 45.4 11.3 999999.9 41031.25 36.2 5.6 999999.9 41066.25 39.8 0.0 999999.9 41101.25 38.2 999999.9 163.4 41136.25 31.0 999999.9 175.9 41171.25 23.7 999999.9 999999.9 41206.25 42.0 5.0 999999.9 41241.25 33.0 6.1 999999.9 41276.25 25.7 999999.9 999999.9 41311.25 39.2 999999.9 999999.9 41346.25 24.2 999999.9 999999.9 41381.25 37.7 999999.9 999999.9 41416.25 61.5 999999.9 999999.9 41451.25 48.0 999999.9 999999.9 41486.25 50.3 999999.9 999999.9 41521.25 65.7 999999.9 999999.9 41556.25 33.3 999999.9 999999.9 41591.25 42.4 999999.9 999999.9 41626.25 37.8 999999.9 999999.9 41661.25 30.4 15.5 999999.9 41696.25 45.0 -3.9 999999.9 41731.25 44.6 -6.8 999999.9 41766.25 39.9 999999.9 291.4 41801.25 52.2 999999.9 214.4 41836.25 45.0 999999.9 999999.9 41871.25 30.4 999999.9 999999.9 41906.25 42.8 0.3 999999.9 41941.25 28.0 999999.9 999999.9 41976.25 60.5 999999.9 999999.9 42011.25 49.5 999999.9 999999.9 42046.25 40.1 999999.9 999999.9 42081.25 45.4 4.1 999999.9 42116.25 40.6 3.2 999999.9 42151.25 23.0 10.9 999999.9 42186.25 49.6 999999.9 194.5 42221.25 44.7 999999.9 193.6 42256.25 34.0 999999.9 999999.9 42291.25 38.1 999999.9 999999.9 42326.25 52.4 1.5 999999.9 42361.25 41.1 999999.9 999999.9 42396.25 60.7 999999.9 999999.9 42431.25 86.7 999999.9 999999.9 42466.25 59.8 999999.9 999999.9 42501.25 69.3 18.2 999999.9 42536.25 89.5 4.9 999999.9 42571.25 63.2 1.9 999999.9 42606.25 59.7 999999.9 311.7 42641.25 63.3 999999.9 530.4 42676.25 54.3 999999.9 999999.9 42711.25 69.2 999999.9 999999.9 42746.25 80.3 -22.6 999999.9 42781.25 102.9 999999.9 999999.9 42816.25 102.8 999999.9 999999.9 42851.25 115.4 999999.9 999999.9 42886.25 124.3 999999.9 999999.9 42921.25 111.9 999999.9 999999.9 42956.25 109.9 999999.9 999999.9 42991.25 153.4 999999.9 999999.9 43026.25 147.1 999999.9 999999.9 43061.25 111.4 999999.9 999999.9 43096.25 142.0 999999.9 999999.9 43131.25 130.4 999999.9 999999.9 43166.25 113.6 18.1 999999.9 43201.25 120.0 -7.8 999999.9 43236.25 116.9 -2.6 999999.9 43271.25 117.6 999999.9 977.2 43306.25 93.4 999999.9 926.3 43341.25 117.0 999999.9 999999.9 43376.25 81.1 999999.9 999999.9 43411.25 95.6 -12.5 999999.9 43446.25 100.8 999999.9 999999.9 43481.25 106.0 999999.9 999999.9 43516.25 87.9 999999.9 999999.9 43551.25 87.3 999999.9 999999.9 43586.25 86.9 0.9 999999.9 43621.25 91.8 -13.4 999999.9 43656.25 100.2 -9.1 999999.9 43691.25 102.2 999999.9 826.7 43726.25 107.3 999999.9 833.3 43761.25 98.5 999999.9 999999.9 43796.25 92.2 999999.9 999999.9 43831.25 107.1 -23.1 999999.9 43866.25 97.8 999999.9 999999.9 43901.25 113.1 999999.9 999999.9 43936.25 86.7 999999.9 999999.9 43971.25 79.3 999999.9 999999.9 44006.25 74.2 -5.1 999999.9 44041.25 78.3 -6.3 999999.9 44076.25 103.7 11.8 999999.9 44111.25 86.3 999999.9 669.4 44146.25 75.2 999999.9 678.7 44181.25 92.9 999999.9 999999.9 44216.25 84.8 999999.9 999999.9 44251.25 97.2 -13.5 999999.9 44286.25 74.4 999999.9 999999.9 44321.25 71.5 999999.9 999999.9 44356.25 68.5 999999.9 999999.9 44391.25 92.3 999999.9 999999.9 44426.25 99.1 999999.9 999999.9 44461.25 106.3 999999.9 999999.9 44496.25 103.8 999999.9 999999.9 44531.25 97.3 999999.9 999999.9 44566.25 97.6 999999.9 999999.9 44601.25 107.7 999999.9 999999.9 44636.25 78.9 999999.9 999999.9 44671.25 64.7 40.9 999999.9 44706.25 58.9 -2.1 999999.9 44741.25 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