44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 03 05 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 32788.25 -8.8 999999.9 999999.9 32823.25 0.8 999999.9 999999.9 32858.25 10.3 999999.9 999999.9 32893.25 2.8 999999.9 999999.9 32928.25 10.6 999999.9 999999.9 32963.25 -2.8 999999.9 999999.9 32998.25 2.2 999999.9 999999.9 33033.25 14.8 999999.9 999999.9 33068.25 14.2 999999.9 999999.9 33103.25 12.7 999999.9 999999.9 33138.25 8.8 999999.9 999999.9 33173.25 25.7 999999.9 999999.9 33208.25 18.3 999999.9 999999.9 33243.25 12.6 999999.9 999999.9 33278.25 26.4 999999.9 999999.9 33313.25 33.7 999999.9 999999.9 33348.25 25.5 999999.9 999999.9 33383.25 23.3 999999.9 999999.9 33418.25 26.8 999999.9 999999.9 33453.25 52.8 999999.9 999999.9 33488.25 106.8 999999.9 999999.9 33523.25 141.9 999999.9 999999.9 33558.25 156.3 999999.9 999999.9 33593.25 199.9 999999.9 999999.9 33628.25 204.8 999999.9 999999.9 33663.25 224.8 999999.9 999999.9 33698.25 253.5 999999.9 999999.9 33733.25 313.5 999999.9 999999.9 33768.25 347.9 999999.9 387.0 33803.25 360.1 999999.9 289.2 33838.25 385.5 999999.9 343.1 33873.25 396.3 99.4 999999.9 33908.25 396.4 83.9 999999.9 33943.25 495.9 999999.9 999999.9 33978.25 569.9 999999.9 999999.9 34013.25 614.4 999999.9 999999.9 34048.25 605.4 999999.9 999999.9 34083.25 589.7 194.1 999999.9 34118.25 999999.9 999999.9 999999.9 34153.25 614.4 155.6 999999.9 34188.25 679.9 999999.9 376.5 34223.25 707.9 999999.9 354.1 34258.25 758.3 999999.9 350.6 34293.25 763.7 182.3 999999.9 34328.25 776.1 203.4 999999.9 34363.25 835.2 999999.9 999999.9 34398.25 801.8 999999.9 999999.9 34433.25 820.6 999999.9 999999.9 34468.25 845.1 999999.9 999999.9 34503.25 912.5 999999.9 999999.9 34538.25 873.9 999999.9 999999.9 34573.25 925.8 999999.9 999999.9 34608.25 924.0 999999.9 999999.9 34643.25 888.5 999999.9 999999.9 34678.25 915.7 999999.9 999999.9 34713.25 846.0 999999.9 999999.9 34748.25 914.3 209.0 999999.9 34783.25 863.7 211.6 999999.9 34818.25 747.9 190.8 999999.9 34853.25 705.8 999999.9 428.3 34888.25 821.8 999999.9 424.4 34923.25 778.5 999999.9 999999.9 34958.25 799.4 137.4 999999.9 34993.25 820.4 173.5 999999.9 35028.25 1010.2 999999.9 999999.9 35063.25 977.6 999999.9 999999.9 35098.25 998.3 999999.9 999999.9 35133.25 954.3 999999.9 999999.9 35168.25 956.5 219.0 999999.9 35203.25 983.7 226.9 999999.9 35238.25 980.9 202.8 999999.9 35273.25 915.4 999999.9 431.3 35308.25 896.7 999999.9 494.3 35343.25 904.7 999999.9 999999.9 35378.25 929.7 162.5 999999.9 35413.25 880.9 174.8 999999.9 35448.25 936.8 999999.9 999999.9 35483.25 912.8 999999.9 999999.9 35518.25 911.0 999999.9 999999.9 35553.25 1008.2 999999.9 999999.9 35588.25 1018.1 197.8 999999.9 35623.25 953.1 193.4 999999.9 35658.25 917.2 202.5 999999.9 35693.25 907.4 999999.9 448.9 35728.25 984.7 999999.9 406.9 35763.25 979.8 999999.9 999999.9 35798.25 1070.2 198.6 999999.9 35833.25 1054.4 208.1 999999.9 35868.25 1065.1 999999.9 999999.9 35903.25 1069.0 999999.9 999999.9 35938.25 988.1 999999.9 999999.9 35973.25 1011.3 999999.9 999999.9 36008.25 1104.6 999999.9 999999.9 36043.25 1107.9 999999.9 999999.9 36078.25 1072.2 999999.9 999999.9 36113.25 1128.7 999999.9 999999.9 36148.25 1085.0 999999.9 999999.9 36183.25 1110.2 999999.9 999999.9 36218.25 1067.7 999999.9 999999.9 36253.25 1124.6 277.2 999999.9 36288.25 1163.1 264.3 999999.9 36323.25 1162.3 247.7 999999.9 36358.25 1139.8 999999.9 342.1 36393.25 1108.3 999999.9 346.7 36428.25 1076.5 999999.9 999999.9 36463.25 1080.2 999999.9 999999.9 36498.25 924.9 188.8 999999.9 36533.25 1025.7 999999.9 999999.9 36568.25 1035.9 999999.9 999999.9 36603.25 991.0 999999.9 999999.9 36638.25 982.0 999999.9 999999.9 36673.25 961.3 217.8 999999.9 36708.25 848.8 186.0 999999.9 36743.25 965.8 175.5 999999.9 36778.25 929.0 999999.9 556.7 36813.25 746.2 999999.9 769.3 36848.25 682.6 999999.9 999999.9 36883.25 664.4 84.8 999999.9 36918.25 632.3 77.0 999999.9 36953.25 646.2 999999.9 999999.9 36988.25 660.0 999999.9 999999.9 37023.25 583.7 999999.9 999999.9 37058.25 569.7 999999.9 999999.9 37093.25 539.4 84.2 999999.9 37128.25 515.7 66.6 999999.9 37163.25 529.1 62.8 999999.9 37198.25 526.1 999999.9 998.0 37233.25 431.8 999999.9 1052.4 37268.25 438.4 999999.9 999999.9 37303.25 764.8 999999.9 999999.9 37338.25 656.4 90.4 999999.9 37373.25 799.7 999999.9 999999.9 37408.25 762.1 999999.9 999999.9 37443.25 606.9 999999.9 999999.9 37478.25 516.4 999999.9 999999.9 37513.25 679.1 999999.9 999999.9 37548.25 731.8 999999.9 999999.9 37583.25 779.7 999999.9 999999.9 37618.25 894.7 999999.9 999999.9 37653.25 945.5 999999.9 999999.9 37688.25 898.9 999999.9 999999.9 37723.25 987.3 999999.9 999999.9 37758.25 983.4 207.7 999999.9 37793.25 1076.7 228.6 999999.9 37828.25 1184.4 265.9 999999.9 37863.25 1123.8 999999.9 250.5 37898.25 1091.3 999999.9 275.5 37933.25 1092.1 999999.9 999999.9 37968.25 1064.7 999999.9 999999.9 38003.25 1009.3 207.8 999999.9 38038.25 1051.6 999999.9 999999.9 38073.25 1133.8 999999.9 999999.9 38108.25 1030.3 999999.9 999999.9 38143.25 1037.6 999999.9 999999.9 38178.25 1038.4 239.0 999999.9 38213.25 1113.2 217.1 999999.9 38248.25 1087.7 210.3 999999.9 38283.25 966.0 999999.9 514.4 38318.25 964.8 999999.9 468.0 38353.25 1057.5 999999.9 999999.9 38388.25 1006.8 999999.9 999999.9 38423.25 1004.3 208.0 999999.9 38458.25 1010.2 999999.9 999999.9 38493.25 913.2 999999.9 999999.9 38528.25 965.4 999999.9 999999.9 38563.25 930.9 999999.9 999999.9 38598.25 1010.7 196.0 999999.9 38633.25 974.0 190.5 999999.9 38668.25 878.8 158.4 999999.9 38703.25 866.0 999999.9 638.3 38738.25 872.1 999999.9 645.5 38773.25 869.8 999999.9 999999.9 38808.25 904.5 999999.9 999999.9 38843.25 877.5 148.7 999999.9 38878.25 838.4 999999.9 999999.9 38913.25 840.9 999999.9 999999.9 38948.25 817.6 999999.9 999999.9 38983.25 758.9 999999.9 999999.9 39018.25 820.9 999999.9 999999.9 39053.25 817.7 999999.9 999999.9 39088.25 805.0 999999.9 999999.9 39123.25 788.2 999999.9 999999.9 39158.25 749.3 999999.9 999999.9 39193.25 777.4 999999.9 999999.9 39228.25 882.0 999999.9 999999.9 39263.25 704.6 138.5 999999.9 39298.25 710.2 118.9 999999.9 39333.25 694.2 123.1 999999.9 39368.25 695.9 999999.9 850.1 39403.25 646.2 999999.9 896.5 39438.25 636.3 999999.9 999999.9 39473.25 592.4 999999.9 999999.9 39508.25 541.9 70.2 999999.9 39543.25 457.0 999999.9 999999.9 39578.25 524.4 999999.9 999999.9 39613.25 493.3 999999.9 999999.9 39648.25 455.8 999999.9 999999.9 39683.25 567.9 101.5 999999.9 39718.25 477.0 105.2 999999.9 39753.25 638.1 154.0 999999.9 39788.25 585.2 999999.9 439.9 39823.25 570.3 999999.9 522.7 39858.25 565.4 999999.9 999999.9 39893.25 502.6 106.8 999999.9 39928.25 441.5 114.4 999999.9 39963.25 489.9 999999.9 999999.9 39998.25 337.7 999999.9 999999.9 40033.25 232.4 999999.9 999999.9 40068.25 197.4 999999.9 999999.9 40103.25 179.8 39.6 999999.9 40138.25 111.0 32.8 999999.9 40173.25 130.5 37.2 999999.9 40208.25 83.8 999999.9 261.2 40243.25 66.0 999999.9 274.1 40278.25 78.3 999999.9 535.6 40313.25 106.6 -6.0 999999.9 40348.25 104.8 -7.6 999999.9 40383.25 138.9 999999.9 999999.9 40418.25 200.3 999999.9 999999.9 40453.25 217.1 999999.9 999999.9 40488.25 273.1 999999.9 999999.9 40523.25 327.6 999999.9 999999.9 40558.25 516.4 999999.9 999999.9 40593.25 525.1 999999.9 999999.9 40628.25 490.4 999999.9 999999.9 40663.25 540.5 999999.9 999999.9 40698.25 642.6 999999.9 999999.9 40733.25 693.8 999999.9 999999.9 40768.25 647.2 203.4 999999.9 40803.25 655.6 175.1 999999.9 40838.25 679.7 170.7 999999.9 40873.25 605.1 999999.9 477.9 40908.25 526.2 999999.9 539.0 40943.25 469.0 999999.9 999999.9 40978.25 520.6 72.2 999999.9 41013.25 533.3 91.2 999999.9 41048.25 477.6 999999.9 999999.9 41083.25 559.2 999999.9 999999.9 41118.25 561.2 999999.9 999999.9 41153.25 557.1 999999.9 999999.9 41188.25 534.7 107.0 999999.9 41223.25 540.8 117.0 999999.9 41258.25 533.7 99.8 999999.9 41293.25 531.9 999999.9 735.5 41328.25 519.5 999999.9 736.9 41363.25 447.5 999999.9 999999.9 41398.25 451.6 69.2 999999.9 41433.25 490.7 78.7 999999.9 41468.25 497.7 999999.9 999999.9 41503.25 521.5 999999.9 999999.9 41538.25 498.2 999999.9 999999.9 41573.25 516.5 999999.9 999999.9 41608.25 521.5 102.0 999999.9 41643.25 489.5 86.9 999999.9 41678.25 577.3 79.9 999999.9 41713.25 524.6 999999.9 754.5 41748.25 525.3 999999.9 816.9 41783.25 497.5 999999.9 999999.9 41818.25 562.0 999999.9 999999.9 41853.25 595.1 97.4 999999.9 41888.25 595.0 999999.9 999999.9 41923.25 612.5 999999.9 999999.9 41958.25 602.0 999999.9 999999.9 41993.25 617.7 999999.9 999999.9 42028.25 637.6 999999.9 999999.9 42063.25 639.3 999999.9 999999.9 42098.25 659.4 999999.9 999999.9 42133.25 673.8 999999.9 999999.9 42168.25 669.8 999999.9 999999.9 42203.25 677.9 999999.9 999999.9 42238.25 665.9 999999.9 999999.9 42273.25 660.9 151.7 999999.9 42308.25 656.8 138.8 999999.9 42343.25 611.7 147.0 999999.9 42378.25 668.2 999999.9 656.3 42413.25 579.6 999999.9 715.2 42448.25 550.7 999999.9 999999.9 42483.25 585.1 124.9 999999.9 42518.25 638.3 152.3 999999.9 42553.25 708.9 999999.9 999999.9 42588.25 768.8 999999.9 999999.9 42623.25 728.6 999999.9 999999.9 42658.25 719.8 999999.9 999999.9 42693.25 664.4 201.5 999999.9 42728.25 676.7 166.7 999999.9 42763.25 667.9 149.8 999999.9 42798.25 693.1 999999.9 740.7 42833.25 769.3 999999.9 729.6 42868.25 813.2 999999.9 999999.9 42903.25 860.6 999999.9 999999.9 42938.25 828.6 233.8 999999.9 42973.25 862.2 999999.9 999999.9 43008.25 819.4 999999.9 999999.9 43043.25 815.1 999999.9 999999.9 43078.25 862.8 999999.9 999999.9 43113.25 773.9 225.7 999999.9 43148.25 759.6 216.1 999999.9 43183.25 730.2 203.1 999999.9 43218.25 626.5 999999.9 727.0 43253.25 574.0 999999.9 819.8 43288.25 529.1 999999.9 999999.9 43323.25 750.7 999999.9 999999.9 43358.25 697.1 203.9 999999.9 43393.25 721.6 999999.9 999999.9 43428.25 688.6 999999.9 999999.9 43463.25 717.0 999999.9 999999.9 43498.25 672.2 999999.9 999999.9 43533.25 681.8 999999.9 999999.9 43568.25 636.0 999999.9 999999.9 43603.25 619.6 999999.9 999999.9 43638.25 654.1 999999.9 999999.9 43673.25 604.2 999999.9 999999.9 43708.25 600.2 999999.9 999999.9 43743.25 625.3 999999.9 999999.9 43778.25 579.7 161.6 999999.9 43813.25 571.6 138.3 999999.9 43848.25 599.4 130.0 999999.9 43883.25 597.0 999999.9 1122.1 43918.25 565.6 999999.9 1085.6 43953.25 576.5 999999.9 999999.9 43988.25 585.4 999999.9 999999.9 44023.25 560.5 134.9 999999.9 44058.25 603.9 999999.9 999999.9 44093.25 643.2 999999.9 999999.9 44128.25 615.5 999999.9 999999.9 44163.25 620.4 999999.9 999999.9 44198.25 596.4 146.7 999999.9 44233.25 592.7 119.4 999999.9 44268.25 614.9 149.1 999999.9 44303.25 604.3 999999.9 999.3 44338.25 598.6 999999.9 1084.0 44373.25 599.1 999999.9 999999.9 44408.25 614.8 999999.9 999999.9 44443.25 620.8 120.4 999999.9 44478.25 614.2 999999.9 999999.9 44513.25 643.6 999999.9 999999.9 44548.25 636.4 999999.9 999999.9 44583.25 581.5 999999.9 999999.9 44618.25 568.8 144.2 999999.9 44653.25 590.8 121.2 999999.9 44688.25 601.4 156.8 999999.9 44723.25 584.5 999999.9 992.4 44758.25 602.3 999999.9 1030.6 44793.25 650.1 999999.9 999999.9 44828.25 749.2 999999.9 999999.9 44863.25 814.1 238.6 999999.9 44898.25 956.5 999999.9 999999.9 44933.25 933.7 999999.9 999999.9 44968.25 1019.4 999999.9 999999.9 45003.25 1020.1 999999.9 999999.9 45038.25 1067.2 999999.9 999999.9 45073.25 1051.5 999999.9 999999.9 45108.25 1050.8 999999.9 999999.9 45143.25 1036.7 999999.9 999999.9 45178.25 993.7 999999.9 999999.9 45213.25 996.8 999999.9 999999.9 45248.25 1050.2 999999.9 999999.9 45283.25 961.9 410.3 999999.9 45318.25 1046.0 399.7 999999.9 45353.25 1038.5 414.3 999999.9 45388.25 1040.0 999999.9 154.7 45423.25 1038.6 999999.9 127.5 45458.25 1018.1 999999.9 999999.9 45493.25 1023.4 999999.9 999999.9 45528.25 1012.4 387.8 999999.9 45563.25 1107.7 999999.9 999999.9 45598.25 1085.0 999999.9 999999.9 45633.25 1063.6 999999.9 999999.9 45668.25 1123.4 999999.9 999999.9 45703.25 1035.6 377.6 999999.9 45738.25 970.7 382.9 999999.9 45773.25 1030.0 370.2 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999999.9 46893.25 963.3 999999.9 503.9 46928.25 977.0 999999.9 462.2 46963.25 947.4 999999.9 999999.9 46998.25 1006.9 999999.9 999999.9 47033.25 1020.8 321.2 999999.9 47068.25 1034.3 999999.9 999999.9 47103.25 1053.0 999999.9 999999.9 47138.25 1051.1 999999.9 999999.9 47173.25 1036.5 999999.9 999999.9 47208.25 981.7 327.2 999999.9 47243.25 993.7 338.6 999999.9 47278.25 1045.7 315.3 999999.9 47313.25 1031.6 999999.9 560.3 47348.25 992.0 999999.9 516.6 47383.25 977.7 999999.9 999999.9 47418.25 984.3 999999.9 999999.9 47453.25 1009.8 318.0 999999.9 47488.25 1041.7 999999.9 999999.9 47523.25 1147.7 999999.9 999999.9 47558.25 1164.2 999999.9 999999.9 47593.25 1134.3 999999.9 999999.9 47628.25 1082.5 423.3 999999.9 47663.25 1146.5 432.8 999999.9 47698.25 1181.2 421.8 999999.9 47733.25 1180.6 999999.9 252.8 47768.25 1135.2 999999.9 122.4 47803.25 1219.9 999999.9 999999.9 47838.25 1176.4 999999.9 999999.9 47873.25 1189.8 413.8 999999.9 47908.25 1164.7 999999.9 999999.9 47943.25 1119.8 999999.9 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