44 1001 R. M. Stimpfle, D. M. Wilmouth and J. G. Anderson Harvard University, Cambridge, MA 02138; Tel (617) 495-5922 ClONO2 SOLVE 1 1 1 1 2000 02 26 2002 9 19 0 Elapsed time (sec) from 0 GMT on flight day 3 1.0 1.0 1.0 999999.9 999999.9 999999.9 ClO Volume Mixing Ratio (pptv) ClOOCl Volume Mixing Ratio (pptv) ClONO2 Volume Mixing Ratio (pptv) 25 Estimated accuracy for ClO: +/- 30 percent, 2 sigma. Estimated accuracy for ClOOCl and ClONO2: +/- 40 percent, 2 sigma. Contact investigators for more information. This version of the inorganic chlorine data differs from the preceding version in that the ClO measurements have been increased on average by up to 25 per cent. This pressure and temperature dependent revision results from the inclusion of the ClOO+NO reaction in the calculation of the yield of Cl atoms from the titration of ClO with NO. The ClOOCl and ClONO2 results are unaffected. In addition we are reporting zero values for those flights where our instrument was operating properly but ClOOCl and/or ClONO2 were demonstrably below the detection limit (approx. 20 ppt for each) for the entire flight. Previously we reported nan values for these flights. Thus the ClOOCl measurements for the flights of 20000106, 20000109, 20000111, and 20000316 are zero values. The flight of 20000123 reports nans because we had an instrument operation failure on that flight. For ClONO2 the flights of 20000120, 20000123, 20000131, 20000202, 20000203 now are zero values. 2 ******************** Data ***************** Time ClO ClOOCl ClONO2 27426.25 -2.2 999999.9 999999.9 27461.25 -9.2 999999.9 999999.9 27496.25 3.2 999999.9 999999.9 27531.25 -17.5 999999.9 999999.9 27566.25 3.1 999999.9 999999.9 27601.25 -14.6 999999.9 999999.9 27636.25 9.9 999999.9 999999.9 27671.25 -9.0 999999.9 999999.9 27706.25 12.9 999999.9 999999.9 27741.25 18.7 999999.9 999999.9 27776.25 8.8 999999.9 999999.9 27811.25 8.7 999999.9 999999.9 27846.25 44.8 999999.9 999999.9 27881.25 27.8 999999.9 999999.9 27916.25 88.5 999999.9 999999.9 27951.25 133.8 999999.9 999999.9 27986.25 132.9 999999.9 999999.9 28021.25 83.3 999999.9 999999.9 28056.25 54.6 999999.9 999999.9 28091.25 78.1 999999.9 999999.9 28126.25 85.9 999999.9 999999.9 28161.25 63.8 999999.9 999999.9 28196.25 79.5 999999.9 999999.9 28231.25 58.1 999999.9 999999.9 28266.25 54.3 999999.9 999999.9 28301.25 91.1 999999.9 999999.9 28336.25 92.8 999999.9 999999.9 28371.25 79.3 999999.9 999999.9 28406.25 90.0 999999.9 396.3 28441.25 118.7 999999.9 429.2 28476.25 136.4 999999.9 999999.9 28511.25 109.8 51.4 999999.9 28546.25 143.6 47.0 999999.9 28581.25 130.9 999999.9 999999.9 28616.25 127.1 999999.9 999999.9 28651.25 140.0 999999.9 999999.9 28686.25 296.3 999999.9 999999.9 28721.25 439.6 66.5 999999.9 28756.25 557.9 149.5 999999.9 28791.25 522.9 115.4 999999.9 28826.25 414.0 999999.9 438.0 28861.25 600.3 999999.9 497.4 28896.25 656.1 999999.9 999999.9 28931.25 706.3 164.2 999999.9 28966.25 763.8 172.2 999999.9 29001.25 737.5 999999.9 999999.9 29036.25 665.6 999999.9 999999.9 29071.25 718.0 999999.9 999999.9 29106.25 765.5 999999.9 999999.9 29141.25 810.0 999999.9 999999.9 29176.25 742.0 999999.9 999999.9 29211.25 827.8 999999.9 999999.9 29246.25 830.6 999999.9 999999.9 29281.25 746.1 999999.9 999999.9 29316.25 799.8 999999.9 999999.9 29351.25 808.7 999999.9 999999.9 29386.25 817.9 196.2 999999.9 29421.25 728.4 175.0 999999.9 29456.25 694.0 157.3 999999.9 29491.25 631.8 999999.9 451.5 29526.25 403.2 999999.9 642.6 29561.25 218.6 999999.9 598.3 29596.25 182.1 -14.5 999999.9 29631.25 211.8 1.4 999999.9 29666.25 140.8 999999.9 999999.9 29701.25 483.4 999999.9 999999.9 29736.25 649.1 999999.9 999999.9 29771.25 604.2 999999.9 999999.9 29806.25 422.3 102.9 999999.9 29841.25 189.8 66.4 999999.9 29876.25 391.1 18.3 999999.9 29911.25 384.0 999999.9 856.3 29946.25 274.6 999999.9 827.0 29981.25 417.3 999999.9 999999.9 30016.25 363.0 999999.9 999999.9 30051.25 189.9 26.2 999999.9 30086.25 729.3 999999.9 999999.9 30121.25 740.7 999999.9 999999.9 30156.25 412.5 999999.9 999999.9 30191.25 528.8 999999.9 999999.9 30226.25 427.0 99.0 999999.9 30261.25 535.7 67.4 999999.9 30296.25 800.0 125.3 999999.9 30331.25 714.7 999999.9 599.9 30366.25 730.2 999999.9 758.4 30401.25 813.1 999999.9 999999.9 30436.25 636.7 96.3 999999.9 30471.25 729.1 86.5 999999.9 30506.25 742.7 999999.9 999999.9 30541.25 794.8 999999.9 999999.9 30576.25 761.0 999999.9 999999.9 30611.25 592.1 999999.9 999999.9 30646.25 355.3 999999.9 999999.9 30681.25 391.5 999999.9 999999.9 30716.25 570.4 999999.9 999999.9 30751.25 449.9 999999.9 999999.9 30786.25 511.5 999999.9 999999.9 30821.25 676.6 999999.9 999999.9 30856.25 628.6 999999.9 999999.9 30891.25 444.3 110.9 999999.9 30926.25 305.9 49.1 999999.9 30961.25 370.1 53.2 999999.9 30996.25 448.6 999999.9 987.7 31031.25 637.9 999999.9 848.5 31066.25 682.8 999999.9 999999.9 31101.25 742.6 91.4 999999.9 31136.25 677.4 107.1 999999.9 31171.25 624.0 999999.9 999999.9 31206.25 624.7 999999.9 999999.9 31241.25 615.9 999999.9 999999.9 31276.25 610.4 999999.9 999999.9 31311.25 728.0 116.7 999999.9 31346.25 637.8 104.3 999999.9 31381.25 632.5 76.9 999999.9 31416.25 651.1 999999.9 898.9 31451.25 656.5 999999.9 930.8 31486.25 653.1 999999.9 999999.9 31521.25 603.3 44.9 999999.9 31556.25 710.7 75.2 999999.9 31591.25 832.0 999999.9 999999.9 31626.25 827.6 999999.9 999999.9 31661.25 835.9 999999.9 999999.9 31696.25 852.1 999999.9 999999.9 31731.25 837.0 152.0 999999.9 31766.25 819.5 167.2 999999.9 31801.25 883.3 151.7 999999.9 31836.25 808.1 999999.9 620.7 31871.25 685.8 999999.9 741.5 31906.25 765.2 999999.9 999999.9 31941.25 767.2 999999.9 999999.9 31976.25 769.3 137.8 999999.9 32011.25 787.5 999999.9 999999.9 32046.25 828.3 999999.9 999999.9 32081.25 984.8 999999.9 999999.9 32116.25 933.4 999999.9 999999.9 32151.25 1026.2 999999.9 999999.9 32186.25 1025.6 999999.9 999999.9 32221.25 974.8 999999.9 999999.9 32256.25 1051.4 999999.9 999999.9 32291.25 1032.3 999999.9 999999.9 32326.25 1008.9 999999.9 999999.9 32361.25 956.5 999999.9 999999.9 32396.25 917.5 185.6 999999.9 32431.25 850.5 156.0 999999.9 32466.25 808.4 174.9 999999.9 32501.25 832.0 999999.9 641.8 32536.25 820.9 999999.9 617.3 32571.25 809.0 999999.9 600.8 32606.25 873.5 999999.9 999999.9 32641.25 863.0 163.3 999999.9 32676.25 919.9 999999.9 999999.9 32711.25 924.1 999999.9 999999.9 32746.25 926.9 999999.9 999999.9 32781.25 899.4 999999.9 999999.9 32816.25 950.8 215.6 999999.9 32851.25 990.4 239.9 999999.9 32886.25 995.6 214.4 999999.9 32921.25 969.7 999999.9 379.0 32956.25 1067.9 999999.9 319.3 32991.25 1080.7 999999.9 999999.9 33026.25 1067.7 999999.9 999999.9 33061.25 1119.0 265.8 999999.9 33096.25 1174.6 999999.9 999999.9 33131.25 1127.0 999999.9 999999.9 33166.25 1149.6 999999.9 999999.9 33201.25 1180.9 999999.9 999999.9 33236.25 1119.4 304.6 999999.9 33271.25 1139.9 299.9 999999.9 33306.25 1162.3 304.0 999999.9 33341.25 1161.3 999999.9 114.7 33376.25 1108.7 999999.9 140.8 33411.25 1163.5 999999.9 999999.9 33446.25 1118.7 307.8 999999.9 33481.25 1180.2 303.0 999999.9 33516.25 1237.1 999999.9 999999.9 33551.25 1167.4 999999.9 999999.9 33586.25 1144.8 999999.9 999999.9 33621.25 1182.2 999999.9 999999.9 33656.25 1311.0 999999.9 999999.9 33691.25 1269.9 999999.9 999999.9 33726.25 1278.4 999999.9 999999.9 33761.25 1282.5 999999.9 999999.9 33796.25 1189.5 999999.9 999999.9 33831.25 1210.7 999999.9 999999.9 33866.25 1191.3 999999.9 999999.9 33901.25 1142.0 333.6 999999.9 33936.25 1140.4 302.4 999999.9 33971.25 1166.9 290.2 999999.9 34006.25 1198.7 999999.9 199.8 34041.25 1160.3 999999.9 191.2 34076.25 1167.0 999999.9 999999.9 34111.25 1197.4 999999.9 999999.9 34146.25 1149.4 306.0 999999.9 34181.25 1179.7 999999.9 999999.9 34216.25 1173.1 999999.9 999999.9 34251.25 1219.3 999999.9 999999.9 34286.25 1162.3 999999.9 999999.9 34321.25 1239.1 352.2 999999.9 34356.25 1203.2 343.1 999999.9 34391.25 1172.8 305.4 999999.9 34426.25 1097.9 999999.9 167.3 34461.25 1146.7 999999.9 248.5 34496.25 1108.6 999999.9 999999.9 34531.25 1128.6 999999.9 999999.9 34566.25 1174.3 314.5 999999.9 34601.25 1172.4 999999.9 999999.9 34636.25 1179.3 999999.9 999999.9 34671.25 1222.3 999999.9 999999.9 34706.25 1159.6 999999.9 999999.9 34741.25 1109.6 302.1 999999.9 34776.25 1124.6 332.4 999999.9 34811.25 1221.0 299.6 999999.9 34846.25 1209.3 999999.9 98.1 34881.25 1184.6 999999.9 115.7 34916.25 1142.0 999999.9 999999.9 34951.25 1154.9 999999.9 999999.9 34986.25 1192.9 336.5 999999.9 35021.25 1107.4 999999.9 999999.9 35056.25 1126.1 999999.9 999999.9 35091.25 1106.3 999999.9 999999.9 35126.25 1121.2 999999.9 999999.9 35161.25 1170.4 999999.9 999999.9 35196.25 1194.8 999999.9 999999.9 35231.25 1131.5 999999.9 999999.9 35266.25 1182.5 999999.9 999999.9 35301.25 1200.1 999999.9 999999.9 35336.25 1195.2 999999.9 999999.9 35371.25 1097.1 999999.9 999999.9 35406.25 1055.9 319.4 999999.9 35441.25 1086.3 316.1 999999.9 35476.25 1118.0 305.5 999999.9 35511.25 1116.9 999999.9 206.2 35546.25 1041.4 999999.9 193.4 35581.25 1114.7 999999.9 999999.9 35616.25 1092.2 999999.9 999999.9 35651.25 1125.7 333.1 999999.9 35686.25 1153.5 999999.9 999999.9 35721.25 1068.2 999999.9 999999.9 35756.25 1011.2 999999.9 999999.9 35791.25 1020.9 999999.9 999999.9 35826.25 1034.5 262.2 999999.9 35861.25 1003.5 261.1 999999.9 35896.25 951.2 213.4 999999.9 35931.25 915.7 999999.9 563.0 35966.25 893.2 999999.9 518.3 36001.25 840.9 999999.9 999999.9 36036.25 915.4 999999.9 999999.9 36071.25 910.9 228.5 999999.9 36106.25 925.6 999999.9 999999.9 36141.25 911.0 999999.9 999999.9 36176.25 950.7 999999.9 999999.9 36211.25 950.9 999999.9 999999.9 36246.25 886.9 231.6 999999.9 36281.25 863.3 201.3 999999.9 36316.25 873.1 209.6 999999.9 36351.25 853.9 999999.9 601.1 36386.25 857.2 999999.9 578.7 36421.25 863.1 999999.9 999999.9 36456.25 826.8 999999.9 999999.9 36491.25 834.8 200.0 999999.9 36526.25 911.6 999999.9 999999.9 36561.25 947.5 999999.9 999999.9 36596.25 967.3 999999.9 999999.9 36631.25 876.9 999999.9 999999.9 36666.25 949.9 999999.9 999999.9 36701.25 947.4 999999.9 999999.9 36736.25 904.8 999999.9 999999.9 36771.25 913.0 999999.9 999999.9 36806.25 900.9 999999.9 999999.9 36841.25 924.2 999999.9 999999.9 36876.25 914.8 999999.9 999999.9 36911.25 850.3 228.7 999999.9 36946.25 849.2 228.2 999999.9 36981.25 935.5 212.2 999999.9 37016.25 935.2 999999.9 504.3 37051.25 849.5 999999.9 485.1 37086.25 842.1 999999.9 999999.9 37121.25 858.4 999999.9 999999.9 37156.25 900.1 266.9 999999.9 37191.25 991.5 999999.9 999999.9 37226.25 994.4 999999.9 999999.9 37261.25 1036.5 999999.9 999999.9 37296.25 1160.2 999999.9 999999.9 37331.25 1098.4 373.4 999999.9 37366.25 1179.5 342.1 999999.9 37401.25 1064.3 357.0 999999.9 37436.25 1008.1 999999.9 232.3 37471.25 913.7 999999.9 324.5 37506.25 915.5 999999.9 999999.9 37541.25 904.8 999999.9 999999.9 37576.25 879.3 241.9 999999.9 37611.25 891.8 999999.9 999999.9 37646.25 872.8 999999.9 999999.9 37681.25 938.5 999999.9 999999.9 37716.25 922.6 999999.9 999999.9 37751.25 888.5 280.1 999999.9 37786.25 909.0 232.9 999999.9 37821.25 974.8 270.2 999999.9 37856.25 935.8 999999.9 363.5 37891.25 977.9 999999.9 319.7 37926.25 890.1 999999.9 999999.9 37961.25 959.8 999999.9 999999.9 37996.25 976.5 296.0 999999.9 38031.25 968.8 999999.9 999999.9 38066.25 965.2 999999.9 999999.9 38101.25 915.6 999999.9 999999.9 38136.25 941.3 999999.9 999999.9 38171.25 937.3 999999.9 999999.9 38206.25 923.5 999999.9 999999.9 38241.25 931.3 999999.9 999999.9 38276.25 935.4 999999.9 999999.9 38311.25 894.4 999999.9 999999.9 38346.25 883.4 999999.9 999999.9 38381.25 953.3 999999.9 999999.9 38416.25 908.6 313.7 999999.9 38451.25 957.0 307.6 999999.9 38486.25 981.4 301.3 999999.9 38521.25 948.0 999999.9 380.5 38556.25 924.8 999999.9 473.9 38591.25 958.4 999999.9 999999.9 38626.25 961.2 999999.9 999999.9 38661.25 965.2 333.2 999999.9 38696.25 971.0 999999.9 999999.9 38731.25 911.3 999999.9 999999.9 38766.25 937.9 999999.9 999999.9 38801.25 969.5 999999.9 999999.9 38836.25 938.8 355.0 999999.9 38871.25 895.2 327.4 999999.9 38906.25 939.6 311.3 999999.9 38941.25 923.0 999999.9 446.4 38976.25 901.4 999999.9 452.5 39011.25 875.1 999999.9 999999.9 39046.25 853.9 999999.9 999999.9 39081.25 888.3 293.3 999999.9 39116.25 929.7 999999.9 999999.9 39151.25 904.1 999999.9 999999.9 39186.25 883.3 999999.9 999999.9 39221.25 861.3 999999.9 999999.9 39256.25 875.9 318.8 999999.9 39291.25 910.3 324.3 999999.9 39326.25 929.7 299.0 999999.9 39361.25 902.1 999999.9 465.5 39396.25 918.5 999999.9 324.2 39431.25 911.6 999999.9 999999.9 39466.25 953.9 999999.9 999999.9 39501.25 941.0 409.5 999999.9 39536.25 993.7 999999.9 999999.9 39571.25 983.6 999999.9 999999.9 39606.25 1024.8 999999.9 999999.9 39641.25 1002.6 999999.9 999999.9 39676.25 1031.6 999999.9 999999.9 39711.25 984.7 999999.9 999999.9 39746.25 1004.9 999999.9 999999.9 39781.25 1057.9 999999.9 999999.9 39816.25 964.1 999999.9 999999.9 39851.25 998.8 999999.9 999999.9 39886.25 990.8 999999.9 999999.9 39921.25 923.6 434.3 999999.9 39956.25 925.0 405.3 999999.9 39991.25 990.7 384.7 999999.9 40026.25 944.7 999999.9 218.0 40061.25 905.8 999999.9 240.8 40096.25 931.4 999999.9 999999.9 40131.25 907.3 999999.9 999999.9 40166.25 949.8 469.4 999999.9 40201.25 896.0 999999.9 999999.9 40236.25 927.9 999999.9 999999.9 40271.25 945.3 999999.9 999999.9 40306.25 957.7 999999.9 999999.9 40341.25 902.1 531.7 999999.9 40376.25 928.4 527.8 999999.9 40411.25 923.4 508.9 999999.9 40446.25 880.6 999999.9 151.7 40481.25 898.1 999999.9 183.7 40516.25 845.6 999999.9 999999.9 40551.25 895.2 999999.9 999999.9 40586.25 855.2 516.1 999999.9 40621.25 865.1 999999.9 999999.9 40656.25 874.3 999999.9 999999.9 40691.25 807.2 999999.9 999999.9 40726.25 835.5 999999.9 999999.9 40761.25 758.4 516.9 999999.9 40796.25 802.3 536.0 999999.9 40831.25 792.0 538.1 999999.9 40866.25 761.2 999999.9 114.9 40901.25 767.5 999999.9 127.6 40936.25 706.4 999999.9 999999.9 40971.25 737.0 999999.9 999999.9 41006.25 738.6 582.8 999999.9 41041.25 759.1 999999.9 999999.9 41076.25 697.7 999999.9 999999.9 41111.25 733.7 999999.9 999999.9 41146.25 656.0 999999.9 999999.9 41181.25 679.0 999999.9 999999.9 41216.25 667.1 999999.9 999999.9 41251.25 675.0 999999.9 999999.9 41286.25 608.2 999999.9 999999.9 41321.25 632.5 999999.9 999999.9 41356.25 579.7 999999.9 999999.9 41391.25 625.5 999999.9 999999.9 41426.25 591.6 625.8 999999.9 41461.25 553.6 649.7 999999.9 41496.25 553.2 619.4 999999.9 41531.25 543.5 999999.9 17.1 41566.25 547.6 999999.9 139.5 41601.25 472.7 999999.9 999999.9 41636.25 470.3 999999.9 999999.9 41671.25 474.0 620.0 999999.9 41706.25 460.7 999999.9 999999.9 41741.25 472.6 999999.9 999999.9 41776.25 423.9 999999.9 999999.9 41811.25 424.9 999999.9 999999.9 41846.25 395.7 689.1 999999.9 41881.25 388.0 668.4 999999.9 41916.25 370.7 678.1 999999.9 41951.25 344.5 999999.9 121.9 41986.25 327.8 999999.9 172.5 42021.25 343.6 999999.9 999999.9 42056.25 307.5 999999.9 999999.9 42091.25 318.5 680.2 999999.9 42126.25 318.6 999999.9 999999.9 42161.25 306.1 999999.9 999999.9 42196.25 261.6 999999.9 999999.9 42231.25 258.7 999999.9 999999.9 42266.25 258.1 650.0 999999.9 42301.25 255.9 651.9 999999.9 42336.25 273.4 640.5 999999.9 42371.25 258.5 999999.9 184.6 42406.25 232.3 999999.9 163.5 42441.25 220.5 999999.9 999999.9 42476.25 241.3 999999.9 999999.9 42511.25 216.5 675.3 999999.9 42546.25 200.6 999999.9 999999.9 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