47, 1001 Brune, William; Thames, Alexander; Miller, David; Brosius, Alexandra Penn State University ATHOS - Airborne Tropospheric Hydrogen Oxides Sensor ATom 1, 1 2017, 02, 15, 2018, 10, 25 0 Start_UTC, seconds, seconds since UTC midnight on day of takeoff 4 1, 1, 1, 1 -9999.000, -9999.000, -9999.000, -9999.000 Stop_UTC, seconds, seconds since UTC midnight on day of takeoff Mid_UTC, seconds, seconds since UTC midnight on day of takeoff OH_ATHOS, pptv, OH mixing ratio in pptv HO2_ATHOS, pptv, HO2 mixing ratio in pptv 0 29 PI_CONTACT_INFO: Address: 503 Walker Building, University Park, PA 16802; email: whb2@psu.edu 814-865-3286 PLATFORM: NASA - DC-8 Aircraft - sampling underneath aircraft forward cargo bay LOCATION: ATom II: Science Flight #8 -- ASI - TER ASSOCIATED_DATA: N/A INSTRUMENT_INFO: OH/HO2 from Laser Induced Fluorescence. DATA_INFO: Units are pptv for OH and HO2. UNCERTAINTY: HOx absolute accuracy ~+/- 32% (actually a multiplicative factor of 1/1.32 to 1.32), 2 sigma confidence. ULOD_FLAG: -7777 ULOD_VALUE: N/A LLOD_FLAG: -8888 LLOD_VALUE: N/A DM_CONTACT_INFO: William H. Brune, Penn State, whb2@psu.edu; 814-865-3286 PROJECT_INFO: NSF/NASA ATom Mission. 2016 - 2018; Multiple Locations STIPULATIONS_ON_USE: No restrictions. Contact PI or DM with any questions. OTHER_COMMENTS: Final Data. Future modifications to the calibration are possible but unlikely. - Calibrating ATHOS with the new OH-removing inlet (OHSI) has been difficult, particularly for low pressure (high altitude). - The ATHOS HOx calibrations are pressure-dependent, changing a factor of 3-5 over the atmospheric pressure range. - The laboratory calibration uses different inlet hole sizes to simulate atmospheric pressure changes. - For 2 years, we tried various calibration approaches with the OHSI in place, but none gave repeatable results for high altitude measurements. - In the laboratory calibrations, it proved to be impossible to simulate the atmospheric airflow with the OHSI on and the smaller inlet sizes. - In the end, we found that our previous calibration method gave the most repeatable and reliable results. - In-flight diagnostics show that OH loss on the OHSI is negligible. - For details, please see Faloona et al., J. Atmos. Chem., 47, 139-167, 2004. REVISION: R3 R3: Final Data (see OTHER_COMMENTS) R2: Final Data (see OTHER_COMMENTS) R1: Final Data R0: No comments for this revision. Start_UTC, Stop_UTC, Mid_UTC, OH_ATHOS, HO2_ATHOS 31859, 31878, 31869, -9999.000, -9999.000 31879, 31898, 31889, -9999.000, -9999.000 31899, 31918, 31909, -9999.000, -9999.000 31919, 31938, 31929, -9999.000, -9999.000 31939, 31958, 31949, -9999.000, -9999.000 31959, 31978, 31969, -9999.000, -9999.000 31979, 31998, 31989, 0.120, 17.141 31999, 32018, 32009, 0.120, 18.196 32019, 32038, 32029, 0.122, 18.089 32039, 32058, 32049, 0.122, 17.981 32059, 32078, 32069, 0.122, 23.808 32079, 32098, 32089, 0.089, 31.315 32100, 32119, 32110, 0.143, 29.249 32120, 32139, 32130, 0.143, 27.193 32140, 32159, 32150, 0.143, 33.181 32160, 32179, 32170, 0.141, 30.224 32180, 32199, 32190, 0.141, 30.822 32200, 32219, 32210, 0.176, 31.426 32220, 32239, 32230, 0.176, 31.139 32240, 32259, 32250, 0.179, 34.490 32260, 32279, 32270, 0.179, 34.066 32280, 32299, 32290, 0.185, 33.636 32300, 32319, 32310, 0.185, 33.057 32320, 32339, 32330, 0.251, 32.185 32340, 32359, 32350, 0.251, 31.528 32360, 32379, 32370, 0.248, 30.871 32380, 32399, 32390, 0.248, 31.379 32400, 32419, 32410, 0.240, 28.450 32420, 32439, 32430, 0.240, 25.537 32440, 32459, 32450, 0.223, 22.623 32460, 32479, 32470, 0.223, 19.709 32480, 32499, 32490, 0.207, 16.795 32500, 32519, 32510, 0.207, 13.867 32520, 32539, 32530, 0.181, 10.939 32540, 32559, 32550, 0.239, 19.351 32560, 32579, 32570, 0.239, 21.083 32580, 32599, 32590, 0.239, 20.359 32600, 32619, 32610, 0.203, 19.632 32620, 32639, 32630, 0.136, 14.904 32640, 32659, 32650, 0.136, 13.888 32660, 32679, 32670, 0.136, 17.127 32680, 32699, 32690, 0.179, 20.367 32700, 32719, 32710, 0.179, 19.798 32721, 32740, 32731, 0.179, 15.914 32741, 32760, 32751, 0.184, 18.103 32761, 32780, 32771, 0.184, 20.292 32781, 32800, 32791, 0.255, 23.851 32801, 32820, 32811, 0.255, 24.425 32821, 32840, 32831, 0.255, 23.165 32841, 32860, 32851, 0.282, 21.897 32861, 32880, 32871, 0.220, 23.070 32881, 32900, 32891, 0.220, 20.028 32901, 32920, 32911, 0.220, 18.169 32921, 32940, 32931, 0.255, 16.310 32941, 32960, 32951, 0.257, 17.789 32961, 32980, 32971, 0.257, 16.476 32981, 33000, 32991, 0.230, 14.647 33001, 33020, 33011, 0.230, 12.817 33021, 33040, 33031, 0.230, 15.529 33041, 33060, 33051, 0.254, 12.954 33061, 33080, 33071, 0.254, 13.801 33081, 33100, 33091, 0.230, 14.648 33101, 33120, 33111, 0.230, 13.591 33121, 33140, 33131, 0.177, 14.607 33141, 33160, 33151, 0.191, 13.499 33161, 33180, 33171, 0.191, 12.403 33181, 33200, 33191, 0.173, 12.137 33201, 33220, 33211, 0.173, 13.006 33221, 33240, 33231, 0.173, 12.206 33242, 33261, 33252, 0.200, 11.399 33262, 33281, 33272, 0.222, 12.993 33282, 33301, 33292, 0.222, 11.828 33302, 33321, 33312, 0.229, 10.837 33322, 33341, 33332, 0.229, 9.847 33342, 33361, 33352, 0.213, 11.459 33362, 33381, 33372, 0.213, 11.975 33382, 33401, 33392, 0.200, 10.988 33402, 33421, 33412, 0.200, 10.007 33422, 33441, 33432, 0.200, 10.560 33442, 33461, 33452, 0.243, 10.900 33462, 33481, 33472, 0.245, 10.254 33482, 33501, 33492, 0.245, 9.608 33502, 33521, 33512, 0.294, 11.353 33522, 33541, 33532, 0.294, 10.838 33542, 33561, 33552, 0.294, 10.520 33562, 33581, 33572, 0.273, 10.201 33582, 33601, 33592, 0.306, 10.076 33602, 33621, 33612, 0.306, 10.409 33622, 33641, 33632, 0.306, 10.084 33642, 33661, 33652, 0.287, 9.758 33662, 33681, 33672, 0.287, 10.393 33682, 33701, 33692, 0.290, 10.308 33703, 33722, 33713, 0.280, 10.005 33723, 33742, 33733, 0.280, 9.704 33743, 33762, 33753, 0.325, 10.216 33763, 33782, 33773, 0.325, 9.714 33783, 33802, 33793, 0.325, 9.748 33803, 33822, 33813, 0.288, 9.782 33823, 33842, 33833, 0.331, 10.938 33843, 33862, 33853, 0.331, 11.664 33863, 33882, 33873, 0.351, 11.394 33883, 33902, 33893, 0.351, 11.124 33903, 33922, 33913, 0.351, 9.857 33923, 33942, 33933, 0.294, -9999.000 33943, 33962, 33953, 0.294, -9999.000 34076, 34095, 34086, 0.280, 8.709 34096, 34115, 34106, 0.277, 10.674 34116, 34135, 34126, 0.277, 10.438 34136, 34155, 34146, 0.277, 10.009 34156, 34175, 34166, 0.286, 9.577 34177, 34196, 34187, 0.295, 11.645 34197, 34216, 34207, 0.295, 10.678 34216, 34235, 34226, 0.295, 9.921 34236, 34255, 34246, 0.332, 9.159 34256, 34275, 34266, 0.332, 10.201 34276, 34295, 34286, 0.343, 9.865 34296, 34315, 34306, 0.297, 10.387 34317, 34336, 34327, 0.297, 10.909 34337, 34356, 34347, 0.297, 11.573 34357, 34376, 34367, 0.322, 11.450 34377, 34396, 34387, 0.322, 11.266 34397, 34416, 34407, 0.308, 11.083 34417, 34436, 34427, 0.308, 11.734 34437, 34456, 34447, 0.351, 10.025 34457, 34476, 34467, 0.351, 10.033 34477, 34496, 34487, 0.371, 10.040 34497, 34516, 34507, 0.314, 12.038 34517, 34536, 34527, 0.314, 10.496 34537, 34556, 34547, 0.314, 11.122 34557, 34576, 34567, 0.266, 11.749 34577, 34596, 34587, 0.266, 15.059 34597, 34616, 34607, 0.252, 14.917 34617, 34636, 34627, 0.250, 14.247 34637, 34656, 34647, 0.250, 13.577 34657, 34676, 34667, 0.250, 17.513 34677, 34696, 34687, 0.240, 17.194 34697, 34716, 34707, 0.240, 17.441 34717, 34736, 34727, 0.250, 17.687 34737, 34756, 34747, 0.250, 19.643 34757, 34776, 34767, 0.266, 20.646 34777, 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38.227 36027, 36046, 36037, 0.335, 40.431 36047, 36066, 36057, 0.335, 40.954 36067, 36086, 36077, 0.242, -9999.000 36087, 36106, 36097, 0.256, -9999.000 36107, 36126, 36117, 0.256, 24.187 36127, 36146, 36137, 0.256, 26.680 36147, 36166, 36157, 0.232, 26.169 36167, 36186, 36177, 0.232, 24.999 36187, 36206, 36197, 0.224, 23.817 36207, 36226, 36217, 0.287, 27.702 36227, 36246, 36237, 0.287, 29.303 36247, 36266, 36257, 0.308, 28.283 36267, 36286, 36277, 0.308, 27.264 36287, 36306, 36297, 0.308, 25.728 36307, 36326, 36317, 0.241, 23.553 36327, 36346, 36337, 0.269, 24.040 36347, 36366, 36357, 0.269, 24.524 36367, 36386, 36377, 0.269, 26.926 36387, 36406, 36397, 0.267, 28.181 36407, 36426, 36417, 0.236, 24.673 36428, 36447, 36438, 0.236, 21.165 36448, 36467, 36458, 0.315, 25.619 36468, 36487, 36478, 0.315, 24.380 36488, 36507, 36498, 0.290, 24.174 36508, 36527, 36518, 0.290, 23.968 36528, 36547, 36538, 0.290, 22.673 36548, 36567, 36558, 0.272, 23.228 36568, 36587, 36578, 0.300, 22.126 36588, 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