43, 1001 Brune, William; Thames, Alexander; Miller, David; Brosius, Alexandra Penn State University ATHOS - Airborne Tropospheric Hydrogen Oxides Sensor based on LIF ATom 1, 1 2017, 02, 15, 2018, 02, 16 0 Start_UTC, seconds, seconds since takeoff's midnight UTC 5 1, 1, 1, 1, 1 -9999.000, -9999.000, -9999.000, -9999.000, -9999.000 Stop_UTC, seconds, seconds since takeoff's midnight UTC Mid_UTC, seconds, seconds since takeoff's midnight UTC OH_pptv, pptv, OH mixing ratio in pptv HO2_pptv, pptv, HO2 mixing ratio in pptv OHR_Hz, Hz, OH reactivity in Hz 0 24 PI_CONTACT_INFO: Address: 503 Walker Building, University Park, PA 16802; email: whb2@psu.edu 814-865-3286 PLATFORM: NASA - DC-8 Aircraft - sampling underneath aircraft forward cargo bay LOCATION: ATom II: Science Flight #8 -- ASI - TER ASSOCIATED_DATA: N/A INSTRUMENT_INFO: OH/HO2 with Laser Induced Fluorescence; OH reactivity with discharge flow DATA_INFO: Units are pptv for OH and HO2; Hz for OHR. UNCERTAINTY: Normaly HOx absolute accuracy is estimated to be +/- 32% at two sigma confidence. Please see comments below. ULOD_FLAG: -7777 ULOD_VALUE: N/A LLOD_FLAG: -8888 LLOD_VALUE: N/A DM_CONTACT_INFO: William H. Brune, Penn State, whb2@psu.edu; 814-865-3286 PROJECT_INFO: NSF/NASA ATom Mission. 2016 - 2018; Multiple Locations STIPULATIONS_ON_USE: No restrictions. Contact PI or DM with any questions. OTHER_COMMENTS: Final Data. ATHOS is calibrated with the new OH scavenging inlet. Differences with previous version due to improved calibration methods. OH & HO2 uncertainty ~1.32, 2 sigma confidence. Data in dense clouds is noisy, and is removed. OHR uncertainty estimated to be 15%, 2 sigma confidence, with 0.3 s^-1 zero uncertainty. OHR correction for NO works for conditions up to ambient NO ~20 ppbv; data are not recoverd for some low altitudes. REVISION: R2 R2: Final Data (see OTHER_COMMENTS) R1: Final Data R0: No comments for this revision. Start_UTC, Stop_UTC, Mid_UTC, OH_pptv, HO2_pptv, OHR_Hz 31875, 31894, 31889, -9999.000, 6.303, -9999.000 31895, 31914, 31909, -9999.000, 7.593, 1.034 31915, 31934, 31929, 0.084, 6.788, -9999.000 31935, 31954, 31949, 0.084, 6.904, -9999.000 31955, 31974, 31969, 0.117, 7.020, 0.699 31975, 31994, 31989, 0.117, 7.794, -9999.000 31995, 32014, 32009, 0.039, 8.287, 3.269 32015, 32034, 32029, 0.039, 8.283, 3.044 32035, 32054, 32049, 0.146, 8.279, 2.962 32055, 32074, 32069, 0.146, 11.366, 3.322 32075, 32094, 32089, 0.084, -9999.000, 2.614 32096, 32115, 32110, 0.084, 14.124, 0.971 32116, 32135, 32130, 0.123, 13.298, 1.497 32136, 32155, 32150, 0.123, 15.970, 2.468 32156, 32175, 32170, 0.116, 14.707, 1.609 32176, 32195, 32190, 0.116, 14.961, 2.557 32196, 32215, 32210, 0.159, 15.217, 2.327 32216, 32235, 32230, 0.159, 15.034, 1.046 32236, 32255, 32250, 0.122, 16.693, 2.613 32256, 32275, 32270, 0.122, 16.527, 3.364 32276, 32295, 32290, 0.193, 16.359, 2.316 32296, 32315, 32310, 0.193, 16.225, 3.091 32316, 32335, 32330, 0.252, 15.798, 2.327 32336, 32355, 32350, 0.252, 15.490, 2.810 32356, 32375, 32370, 0.156, 15.182, 3.152 32376, 32395, 32390, 0.156, 15.508, 2.538 32396, 32415, 32410, 0.274, 14.081, 2.571 32416, 32435, 32430, 0.274, 12.662, 2.825 32436, 32455, 32450, 0.190, 11.242, 3.014 32456, 32475, 32470, 0.190, 9.822, 2.445 32476, 32495, 32490, 0.140, 8.402, 2.705 32496, 32515, 32510, 0.140, 6.976, 2.004 32516, 32535, 32530, 0.165, -9999.000, 1.945 32536, 32555, 32550, 0.165, 9.749, 2.010 32556, 32575, 32570, 0.251, 10.652, 1.986 32576, 32595, 32590, 0.251, 10.265, 2.731 32596, 32615, 32610, 0.163, 9.875, 1.326 32616, 32635, 32630, 0.163, 7.609, 2.201 32636, 32655, 32650, 0.134, 7.059, 0.971 32656, 32675, 32670, 0.134, 8.714, 2.072 32676, 32695, 32690, 0.204, 10.368, 1.776 32696, 32715, 32710, 0.204, 10.064, 1.754 32717, 32736, 32731, 0.132, 8.172, 1.810 32737, 32756, 32751, 0.132, 9.280, 1.145 32757, 32776, 32771, 0.273, 10.388, 1.774 32777, 32796, 32791, 0.273, 12.069, 2.044 32797, 32816, 32811, 0.237, 12.466, 0.880 32817, 32836, 32831, 0.237, 11.827, 1.313 32837, 32856, 32851, 0.290, 11.186, 2.338 32857, 32876, 32871, 0.290, 11.828, 1.223 32877, 32896, 32891, 0.198, 10.247, 0.822 32897, 32916, 32911, 0.198, 9.836, 1.128 32917, 32936, 32931, 0.346, 9.425, 1.236 32937, 32956, 32951, 0.346, 10.269, 1.229 32957, 32976, 32971, 0.269, 9.511, 1.286 32977, 32996, 32991, 0.269, 8.470, 1.532 32997, 33016, 33011, 0.252, 7.429, 1.626 33017, 33036, 33031, 0.252, 8.905, 0.975 33037, 33056, 33051, 0.300, 7.475, 0.793 33057, 33076, 33071, 0.300, 7.979, 0.584 33077, 33096, 33091, 0.229, 8.483, 1.259 33097, 33116, 33111, 0.229, 7.846, 0.932 33117, 33136, 33131, 0.206, 8.467, 1.557 33137, 33156, 33151, 0.206, 7.798, 0.665 33157, 33176, 33171, 0.228, 7.136, 0.343 33177, 33196, 33191, 0.228, 7.028, 0.494 33197, 33216, 33211, 0.205, 7.536, 0.799 33217, 33236, 33231, 0.205, 7.067, 0.902 33238, 33257, 33252, 0.271, 6.593, 1.011 33258, 33277, 33272, 0.271, 7.512, 0.860 33278, 33297, 33292, 0.239, 6.868, 0.466 33298, 33317, 33312, 0.239, 6.308, 0.628 33318, 33337, 33332, 0.269, 5.748, 0.821 33338, 33357, 33352, 0.269, 6.589, 0.305 33358, 33377, 33372, 0.238, 6.986, 0.293 33378, 33397, 33392, 0.238, 6.380, 0.205 33398, 33417, 33412, 0.258, 5.778, 0.609 33418, 33437, 33432, 0.258, 6.147, 0.648 33438, 33457, 33452, 0.261, 6.352, 0.641 33458, 33477, 33472, 0.261, 5.974, 0.558 33478, 33497, 33492, 0.342, 5.596, 0.244 33498, 33517, 33512, 0.342, 6.608, 0.664 33518, 33537, 33532, 0.352, 6.296, 0.487 33538, 33557, 33552, 0.352, 6.149, 0.576 33558, 33577, 33572, 0.303, 6.002, 0.244 33578, 33597, 33592, 0.303, 5.836, 0.753 33598, 33617, 33612, 0.377, 6.098, 0.245 33618, 33637, 33632, 0.377, 5.891, 0.530 33638, 33657, 33652, 0.310, 5.685, 0.965 33658, 33677, 33672, 0.310, 6.014, 0.659 33678, 33697, 33692, 0.347, 6.062, -0.104 33699, 33718, 33713, 0.347, 5.914, 0.933 33719, 33738, 33733, 0.354, 5.766, 0.661 33739, 33758, 33753, 0.354, 5.965, 0.259 33759, 33778, 33773, 0.398, 5.707, 0.422 33779, 33798, 33793, 0.398, 5.732, 0.856 33799, 33818, 33813, 0.331, 5.758, 0.606 33819, 33838, 33833, 0.331, 6.405, 0.665 33839, 33858, 33853, 0.407, 6.822, 0.207 33859, 33878, 33873, 0.407, 6.678, 0.970 33879, 33898, 33893, 0.439, 6.535, 0.650 33899, 33918, 33913, 0.439, -9999.000, 0.069 33919, 33938, 33933, 0.303, -9999.000, 0.443 33939, 33958, 33953, 0.303, -9999.000, 0.441 34072, 34091, 34086, 0.350, 5.156, -9999.000 34092, 34111, 34106, 0.350, 6.244, 0.321 34112, 34131, 34126, 0.314, 6.173, 0.786 34132, 34151, 34146, 0.314, 5.919, 0.389 34152, 34171, 34166, 0.365, 5.664, 0.325 34173, 34192, 34187, 0.365, 6.864, 0.868 34193, 34212, 34207, 0.368, 6.314, -0.247 34212, 34231, 34226, 0.368, 5.884, -9999.000 34232, 34251, 34246, 0.446, 5.451, 1.143 34252, 34271, 34266, 0.446, 5.958, 0.067 34272, 34291, 34286, 0.377, 5.889, 0.130 34292, 34311, 34306, 0.377, 6.207, 0.902 34313, 34332, 34327, 0.324, 6.525, 0.276 34333, 34352, 34347, 0.324, 6.731, 0.310 34353, 34372, 34367, 0.380, 6.755, 0.610 34373, 34392, 34387, 0.380, 6.642, 0.359 34393, 34412, 34407, 0.399, 6.529, 0.493 34413, 34432, 34427, 0.399, 6.875, 0.563 34433, 34452, 34447, 0.426, 5.901, 0.420 34453, 34472, 34467, 0.426, 5.910, 0.160 34473, 34492, 34487, 0.449, 5.920, 0.242 34493, 34512, 34507, 0.449, 7.038, 0.002 34513, 34532, 34527, 0.322, 6.191, 0.630 34533, 34552, 34547, 0.322, 6.572, 0.562 34553, 34572, 34567, 0.286, 6.953, 0.053 34573, 34592, 34587, 0.286, 8.777, 0.461 34593, 34612, 34607, 0.326, 8.798, 0.411 34613, 34632, 34627, 0.326, 8.393, 0.326 34633, 34652, 34647, 0.259, 7.987, 0.645 34653, 34672, 34667, 0.259, 10.149, 0.593 34673, 34692, 34687, 0.298, 10.035, 0.238 34693, 34712, 34707, 0.298, 10.169, 0.273 34713, 34732, 34727, 0.295, 10.302, 0.608 34733, 34752, 34747, 0.295, 11.446, 0.142 34753, 34772, 34767, 0.313, 11.994, 0.400 34773, 34792, 34787, 0.313, 11.843, 0.909 34793, 34812, 34807, 0.306, 11.691, 0.643 34813, 34832, 34827, 0.306, 13.673, -0.084 34833, 34852, 34847, 0.264, 16.259, -0.125 34853, 34872, 34867, 0.264, 14.129, 0.123 34874, 34893, 34888, 0.248, 11.978, 0.942 34894, 34913, 34908, 0.248, 12.962, 0.072 34914, 34933, 34928, 0.275, -9999.000, 0.273 34934, 34953, 34948, 0.275, -9999.000, 1.899 34954, 34973, 34968, -9999.000, -9999.000, 0.797 34974, 34993, 34988, -9999.000, 15.894, 0.820 34994, 35013, 35008, 0.326, 14.894, 1.858 35014, 35033, 35028, 0.326, 13.808, 2.185 35034, 35053, 35048, 0.275, 12.722, 0.706 35054, 35073, 35068, 0.275, 22.084, 2.223 35074, 35093, 35088, 0.258, 19.321, 2.336 35094, 35113, 35108, 0.258, 19.415, 1.332 35114, 35133, 35128, 0.279, 19.511, 3.046 35134, 35153, 35148, 0.279, 18.460, 2.004 35154, 35173, 35168, 0.196, 23.360, 2.553 35174, 35193, 35188, 0.196, 21.479, 2.511 35194, 35213, 35208, 0.177, 19.598, 3.515 35214, 35233, 35228, 0.177, 23.140, 4.175 35234, 35253, 35248, 0.089, 20.903, 4.564 35254, 35273, 35268, 0.089, 18.305, 2.136 35274, 35293, 35288, 0.130, 15.707, -9999.000 35294, 35313, 35308, 0.130, 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35897, 0.176, 15.527, 3.965 35903, 35922, 35917, 0.168, 12.944, 2.985 35923, 35942, 35937, 0.168, 15.523, 3.461 35943, 35962, 35957, 0.284, 18.115, 4.223 35963, 35982, 35977, 0.284, 22.464, 2.664 35983, 36002, 35997, 0.222, 20.839, 2.980 36003, 36022, 36017, 0.222, 22.102, 2.493 36023, 36042, 36037, 0.350, 23.365, 2.083 36043, 36062, 36057, 0.350, -9999.000, 1.696 36063, 36082, 36077, 0.222, -9999.000, 1.800 36083, 36102, 36097, 0.222, -9999.000, 0.801 36103, 36122, 36117, 0.273, 13.995, 1.177 36123, 36142, 36137, 0.273, 15.413, 2.028 36143, 36162, 36157, 0.245, 15.119, 1.474 36163, 36182, 36177, 0.245, 14.409, 0.911 36183, 36202, 36197, 0.231, 13.692, 1.265 36203, 36222, 36217, 0.231, 15.836, 1.105 36223, 36242, 36237, 0.385, 17.064, 0.767 36243, 36262, 36257, 0.385, 16.516, 1.625 36263, 36282, 36277, 0.291, 15.969, 1.545 36283, 36302, 36297, 0.291, 14.989, 1.056 36303, 36322, 36317, 0.264, 13.768, 1.499 36323, 36342, 36337, 0.264, 13.999, 0.327 36343, 36362, 36357, 0.322, 14.228, 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37324, 37319, 0.357, 11.122, 0.346 37325, 37344, 37339, 0.357, 9.715, 0.685 37345, 37364, 37359, 0.380, 9.216, 0.414 37365, 37384, 37379, 0.380, 8.421, 0.030 37385, 37404, 37399, 0.397, 7.630, 0.888 37405, 37424, 37419, 0.397, 8.492, 1.026 37425, 37444, 37439, 0.350, 8.831, 0.469 37445, 37464, 37459, 0.350, 8.824, -9999.000 37465, 37484, 37479, 0.350, 8.818, -9999.000 37576, 37595, 37590, 0.452, 8.198, -9999.000 37596, 37615, 37610, 0.452, 8.474, 0.349 37616, 37635, 37630, 0.452, 7.984, 0.531 37636, 37655, 37650, 0.441, 7.496, 0.308 37656, 37675, 37670, 0.441, 8.607, -9999.000 37676, 37695, 37690, 0.454, 7.746, -0.265 37696, 37715, 37710, 0.454, 7.856, 0.363 37716, 37735, 37730, 0.448, 7.966, 0.090 37736, 37755, 37750, 0.448, 8.577, 0.220 37756, 37775, 37770, 0.386, 7.916, -0.101 37776, 37795, 37790, 0.386, 8.268, 0.687 37796, 37815, 37810, 0.450, 8.620, 0.365 37816, 37835, 37830, 0.450, 9.242, 0.208 37836, 37855, 37850, 0.404, 8.941, 0.879 37856, 37875, 37870, 0.404, 9.488, 0.448 37876, 37895, 37890, 0.386, 10.032, 0.433 37896, 37915, 37910, 0.386, 10.236, 1.253 37916, 37935, 37930, 0.438, 9.765, 0.406 37937, 37956, 37951, 0.438, 9.090, -0.036 37957, 37976, 37971, 0.326, 8.414, 0.177 37977, 37996, 37991, 0.326, 9.343, 0.474 37997, 38016, 38011, 0.377, 9.329, 0.104 38017, 38036, 38031, 0.377, 9.787, 0.013 38037, 38056, 38051, 0.290, 10.246, 0.294 38057, 38076, 38071, 0.290, 10.777, 0.312 38077, 38096, 38091, 0.326, 9.849, 0.759 38097, 38116, 38111, 0.326, 9.736, 0.592 38117, 38136, 38131, 0.356, 9.623, 0.257 38137, 38156, 38151, 0.356, 10.771, 0.458 38157, 38176, 38171, 0.451, 9.765, 0.248 38177, 38196, 38191, 0.451, 11.528, 0.273 38197, 38216, 38211, 0.391, 13.291, 0.167 38217, 38236, 38231, 0.391, 12.639, 0.207 38237, 38256, 38251, 0.355, 13.598, -0.338 38257, 38276, 38271, 0.355, 13.045, 0.215 38277, 38296, 38291, 0.293, 12.492, -0.227 38297, 38316, 38311, 0.293, 15.319, -0.304 38317, 38336, 38331, 0.309, 13.922, 0.266 38337, 38356, 38351, 0.309, 15.092, 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