42, 1001 Brune, William; Thames, Alexander; Miller, David; Brosius, Alexandra Penn State University ATHOS - Airborne Tropospheric Hydrogen Oxides Sensor based on LIF ATom 1, 1 2017, 02, 03, 2017, 12, 07 0 Start_UTC, seconds, seconds since takeoff's midnight UTC 5 1, 1, 1, 1, 1 -9999.000, -9999.000, -9999.000, -9999.000, -9999.000 Stop_UTC, seconds, seconds since takeoff's midnight UTC Mid_UTC, seconds, seconds since takeoff's midnight UTC OH_pptv, pptv, OH mixing ratio in pptv HO2_pptv, pptv, HO2 mixing ratio in pptv OHR_Hz, Hz, OH reactivity in Hz 0 23 PI_CONTACT_INFO: Address: 503 Walker Building, University Park, PA 16802; email: whb2@psu.edu 814-865-3286 PLATFORM: NASA - DC-8 Aircraft - sampling underneath aircraft forward cargo bay LOCATION: ATom II: Science Flight #4 -- KOA - NAN ASSOCIATED_DATA: N/A INSTRUMENT_INFO: OH/HO2 with Laser Induced Fluorescence; OH reactivity with discharge flow DATA_INFO: Units are pptv for OH and HO2; Hz for OHR. UNCERTAINTY: Normaly HOx absolute accuracy is estimated to be +/- 32% at two sigma confidence. Please see comments below. ULOD_FLAG: -7777 ULOD_VALUE: N/A LLOD_FLAG: -8888 LLOD_VALUE: N/A DM_CONTACT_INFO: William H. Brune, Penn State, whb2@psu.edu; 814-865-3286 PROJECT_INFO: NSF/NASA ATom Mission. 2016 - 2018; Multiple Locations STIPULATIONS_ON_USE: No restrictions. Contact PI or DM with any questions. OTHER_COMMENTS: Semi-Final Data. Calibrating ATHOS with the new OH scavenging inlet is proving to be difficult. Until we complete more tests, OH uncertainty above 6 km estimated to be a factor of 2, 2 sigma confidence HO2 uncertainty for all altitudes estimated to be a factor of 1.6, 2 sigma confidence. OHR uncertainty estimated to be 15%, 2 sigma confidence, with 0.3 s^-1 zero uncertainty. OHR correction for NO appears to work for conditions with ambient NO<=~5 ppbv; OHR data are not reported for higher NO conditions. REVISION: R1 R1: Final Data R0: No comments for this revision. Start_UTC, Stop_UTC, Mid_UTC, OH_pptv, HO2_pptv, OHR_Hz 68395, 68414, 68404, -9999.000, 15.167, -1.695 68415, 68434, 68424, 0.132, 30.824, 7.304 68435, 68454, 68444, 0.132, 34.061, 1.168 68455, 68474, 68464, 0.026, 37.332, 1.501 68475, 68494, 68484, 0.026, 36.699, 1.487 68495, 68514, 68504, 0.026, 34.362, 1.823 68515, 68534, 68524, 0.026, 29.491, 1.214 68535, 68554, 68544, 0.122, 24.619, 2.408 68555, 68574, 68564, 0.122, 22.535, 2.593 68575, 68595, 68585, 0.087, 23.480, 1.823 68596, 68615, 68605, 0.087, 23.008, 1.861 68616, 68635, 68625, 0.074, 22.535, 1.429 68636, 68655, 68645, 0.074, 18.755, 1.899 68656, 68675, 68665, 0.031, -9999.000, 0.539 68676, 68695, 68685, 0.031, -9999.000, 0.050 68696, 68715, 68705, -9999.000, -9999.000, 1.340 68716, 68735, 68725, -9999.000, 15.358, 0.500 68736, 68755, 68745, 0.145, 9.446, 0.009 68756, 68775, 68765, 0.145, 3.535, 1.037 68776, 68795, 68785, 0.104, 4.261, 1.060 68796, 68815, 68805, 0.104, 4.988, 3.031 68816, 68835, 68825, 0.116, 5.714, 1.835 68836, 68855, 68845, 0.116, 6.440, 3.040 68856, 68875, 68865, 0.162, 7.170, 2.644 68876, 68895, 68885, 0.162, 12.821, 2.873 68896, 68915, 68905, 0.144, 12.714, 1.608 68916, 68935, 68925, 0.144, 11.859, 1.239 68936, 68955, 68945, 0.122, 11.004, 2.097 68956, 68975, 68965, 0.122, 10.642, 1.095 68976, 68995, 68985, 0.167, 11.461, 1.383 68996, 69015, 69005, 0.167, 9.963, 1.549 69016, 69035, 69025, 0.136, 8.449, 2.496 69036, 69055, 69045, 0.136, 9.919, 0.603 69056, 69075, 69065, 0.151, 10.458, 1.363 69076, 69095, 69085, 0.151, 9.524, 1.112 69096, 69115, 69105, 0.168, 8.589, 1.536 69116, 69135, 69125, 0.168, 9.684, 1.518 69136, 69155, 69145, 0.155, 9.558, 3.062 69156, 69175, 69165, 0.155, 8.863, 1.282 69176, 69195, 69185, 0.193, 8.172, 2.269 69196, 69215, 69205, 0.193, 8.750, 0.518 69216, 69235, 69225, 0.194, 9.977, 0.630 69236, 69255, 69245, 0.194, 9.727, 0.472 69256, 69275, 69265, 0.173, 9.477, 1.454 69276, 69296, 69286, 0.173, 10.765, 0.639 69297, 69316, 69306, 0.194, 8.436, 1.456 69317, 69336, 69326, 0.194, 8.737, 0.761 69337, 69356, 69346, 0.284, 9.038, 1.031 69357, 69376, 69366, 0.284, 9.298, 1.010 69377, 69396, 69386, 0.264, 9.839, 1.144 69397, 69416, 69406, 0.264, 8.849, 0.717 69417, 69436, 69426, 0.189, 7.860, 0.479 69437, 69456, 69446, 0.189, 6.711, 0.299 69457, 69476, 69466, 0.255, 6.407, 0.773 69477, 69496, 69486, 0.255, 5.774, 0.549 69497, 69516, 69506, 0.283, 5.142, 0.510 69517, 69536, 69526, 0.283, 4.961, 0.215 69537, 69556, 69546, 0.200, 5.288, 0.260 69557, 69576, 69566, 0.200, 5.717, 0.214 69577, 69596, 69586, 0.229, 6.146, 0.287 69597, 69616, 69606, 0.229, 6.547, 0.348 69617, 69636, 69626, 0.216, 7.904, 0.608 69637, 69656, 69646, 0.216, 7.596, 0.762 69657, 69676, 69666, 0.305, 7.285, 0.892 69677, 69696, 69686, 0.305, 6.567, 0.751 69697, 69716, 69706, 0.362, 6.983, 0.148 69717, 69736, 69726, 0.362, 7.154, 0.960 69737, 69756, 69746, 0.395, 7.325, -0.143 69757, 69776, 69766, 0.395, -9999.000, 0.508 69777, 69796, 69786, -9999.000, -9999.000, 0.802 69797, 69816, 69806, -9999.000, -9999.000, 0.829 69817, 69836, 69826, 0.441, 5.443, 0.639 69837, 69856, 69846, 0.441, 7.049, 0.519 69857, 69876, 69866, 0.394, 7.168, 1.138 69877, 69896, 69886, 0.394, 7.717, 0.376 69897, 69916, 69906, 0.400, 8.266, 0.681 69917, 69936, 69926, 0.400, 7.167, 1.134 69937, 69956, 69946, 0.356, 7.749, 0.221 69957, 69976, 69966, 0.356, 7.560, 0.352 69977, 70002, 69987, 0.356, 7.371, 0.612 70107, 70131, 70121, 0.265, 8.791, -9999.000 70132, 70151, 70141, 0.265, 8.211, 0.611 70152, 70171, 70161, 0.265, 8.128, 0.260 70172, 70191, 70181, 0.312, 8.045, 0.346 70192, 70211, 70201, 0.312, 8.552, -0.550 70212, 70231, 70221, 0.344, 9.450, 0.323 70232, 70251, 70241, 0.344, 8.396, 0.544 70252, 70272, 70262, 0.293, 7.342, 0.225 70273, 70292, 70282, 0.293, 9.310, 0.151 70293, 70312, 70302, 0.274, 8.315, 0.460 70313, 70332, 70322, 0.274, 8.914, -0.045 70333, 70352, 70342, 0.309, 9.513, 0.731 70353, 70372, 70362, 0.309, 8.572, 0.439 70373, 70392, 70382, 0.325, 8.114, 0.320 70393, 70412, 70402, 0.325, 7.635, 0.874 70413, 70432, 70422, 0.333, 7.156, 0.330 70433, 70452, 70442, 0.333, 8.114, -0.031 70453, 70472, 70462, 0.404, 8.403, -0.043 70473, 70492, 70482, 0.404, 8.323, 0.626 70493, 70512, 70502, 0.391, 8.243, 0.281 70513, 70532, 70522, 0.391, 7.919, 0.225 70533, 70552, 70542, 0.423, 8.462, 0.217 70553, 70572, 70562, 0.423, 7.675, -0.097 70573, 70592, 70582, 0.397, 6.888, 1.039 70593, 70612, 70602, 0.397, 7.987, 0.762 70613, 70632, 70622, 0.360, 8.169, 0.778 70633, 70652, 70642, 0.360, 7.748, -0.010 70653, 70672, 70662, 0.392, 7.324, 0.220 70673, 70692, 70682, 0.392, 8.554, 0.531 70693, 70712, 70702, 0.314, 8.360, 0.209 70713, 70732, 70722, 0.314, 8.486, 0.948 70733, 70752, 70742, 0.326, 8.613, 0.250 70753, 70772, 70762, 0.326, 8.346, 0.157 70773, 70792, 70782, 0.375, 8.399, 0.237 70793, 70812, 70802, 0.375, 8.831, 0.436 70813, 70832, 70822, 0.349, 9.260, 0.985 70833, 70852, 70842, 0.349, 8.773, 0.676 70853, 70872, 70862, 0.344, 8.375, -0.336 70873, 70892, 70882, 0.344, 7.802, -0.180 70893, 70912, 70902, 0.444, 7.229, 0.471 70913, 70932, 70922, 0.444, 8.715, 0.208 70933, 70952, 70942, 0.436, 8.662, -0.179 70953, 70972, 70962, 0.436, 8.581, -0.684 70973, 70992, 70982, 0.406, 8.500, 0.176 70993, 71013, 71003, 0.406, 7.953, -0.076 71014, 71033, 71023, 0.404, 7.715, -0.115 71034, 71053, 71043, 0.404, 7.298, -0.135 71054, 71073, 71063, 0.318, 6.882, -0.540 71074, 71093, 71083, 0.318, 7.746, -0.158 71094, 71113, 71103, 0.251, 7.854, -0.835 71114, 71133, 71123, 0.251, 7.942, -0.445 71134, 71153, 71143, 0.212, 8.031, 0.611 71154, 71173, 71163, 0.212, 7.741, -0.073 71174, 71193, 71183, 0.256, 7.903, -0.551 71194, 71213, 71203, 0.256, 8.815, 0.421 71214, 71233, 71223, 0.261, 9.728, -0.141 71234, 71253, 71243, 0.261, 11.240, -0.835 71254, 71273, 71263, 0.127, 11.754, -0.185 71274, 71293, 71283, 0.127, 10.695, -0.043 71294, 71313, 71303, 0.135, 9.642, 0.047 71314, 71333, 71323, 0.135, 13.000, 0.788 71334, 71353, 71343, 0.187, 11.144, -0.130 71354, 71373, 71363, 0.187, 12.454, 0.335 71374, 71393, 71383, 0.095, 13.770, 1.182 71394, 71413, 71403, 0.095, 15.109, 0.311 71414, 71433, 71423, 0.170, 14.557, 2.770 71434, 71453, 71443, 0.170, 14.260, 2.196 71454, 71473, 71463, 0.104, 13.963, 0.665 71474, 71493, 71483, 0.104, 13.320, 0.067 71494, 71513, 71503, 0.130, 16.652, 1.174 71514, 71533, 71523, 0.130, 19.016, -0.315 71534, 71553, 71543, 0.177, 21.391, 1.723 71554, 71573, 71563, 0.177, 25.327, 2.011 71574, 71593, 71583, 0.188, 24.512, 3.132 71594, 71613, 71603, 0.188, 23.986, 1.687 71614, 71633, 71623, 0.146, 23.465, 1.994 71634, 71653, 71643, 0.146, 24.584, 1.682 71654, 71674, 71664, 0.163, 25.094, 1.357 71675, 71694, 71684, 0.163, 27.022, 2.115 71695, 71714, 71704, 0.129, 28.950, 3.057 71715, 71734, 71724, 0.129, 31.070, 2.938 71735, 71754, 71744, 0.131, 38.204, 2.945 71755, 71774, 71764, 0.131, 41.657, -9999.000 71775, 71794, 71784, 0.158, 45.111, 4.003 71795, 71814, 71804, 0.158, 47.354, 0.896 71815, 71834, 71824, 0.111, 42.789, 2.304 71835, 71854, 71844, 0.111, 39.459, 0.524 71855, 71874, 71864, 0.209, 36.130, 1.183 71875, 71899, 71884, 0.209, 46.615, 3.194 71985, 72009, 71999, 0.119, 47.884, -9999.000 72010, 72029, 72019, 0.119, 49.054, 1.918 72030, 72049, 72039, 0.158, 50.211, 1.131 72050, 72069, 72059, 0.158, 50.164, -9999.000 72070, 72089, 72079, 0.207, 56.221, 2.889 72090, 72109, 72099, 0.207, 55.351, 1.465 72110, 72129, 72119, 0.060, 54.480, 1.966 72130, 72149, 72139, 0.060, 55.061, 1.058 72150, 72169, 72159, 0.178, 42.351, 3.167 72170, 72189, 72179, 0.178, 37.500, 2.191 72190, 72209, 72199, 0.163, 32.648, 0.525 72210, 72229, 72219, 0.163, 31.834, 1.760 72230, 72249, 72239, 0.247, 30.184, 1.554 72250, 72269, 72259, 0.247, 25.630, 2.294 72270, 72289, 72279, 0.199, 21.076, 1.206 72290, 72309, 72299, 0.199, 25.050, 1.500 72310, 72329, 72319, 0.177, 19.238, 0.534 72330, 72349, 72339, 0.177, 18.320, 1.480 72350, 72369, 72359, 0.119, 17.397, 1.421 72370, 72390, 72380, 0.119, 16.433, 0.947 72391, 72410, 72400, 0.170, 13.559, 0.039 72411, 72430, 72420, 0.170, 12.074, 0.797 72431, 72450, 72440, 0.185, 10.588, 0.905 72451, 72470, 72460, 0.185, 10.623, 0.690 72471, 72490, 72480, 0.147, 13.675, 0.303 72491, 72510, 72500, 0.147, 12.978, 0.603 72511, 72530, 72520, 0.126, 12.275, 1.404 72531, 72550, 72540, 0.126, 10.114, 0.091 72551, 72570, 72560, 0.120, 11.564, 0.532 72571, 72590, 72580, 0.120, 10.671, 0.509 72591, 72610, 72600, 0.177, 9.777, 0.432 72611, 72630, 72620, 0.177, 9.754, 0.975 72631, 72650, 72640, 0.245, 12.269, 0.035 72651, 72670, 72660, 0.245, 12.395, 0.795 72671, 72690, 72680, 0.285, 12.521, 0.410 72691, 72710, 72700, 0.285, 11.348, -0.466 72711, 72730, 72720, 0.210, 9.479, -0.059 72731, 72750, 72740, 0.210, 8.114, 0.391 72751, 72770, 72760, 0.276, 6.749, 0.326 72771, 72790, 72780, 0.276, 10.246, 0.884 72791, 72810, 72800, 0.301, 9.842, 0.384 72811, 72830, 72820, 0.301, 9.488, 0.241 72831, 72850, 72840, 0.302, 9.134, 0.583 72851, 72870, 72860, 0.302, 10.688, 0.191 72871, 72890, 72880, 0.280, 9.892, 0.229 72891, 72910, 72900, 0.280, 9.066, 0.544 72911, 72930, 72920, 0.346, 8.241, 0.148 72931, 72950, 72940, 0.346, 9.430, -0.175 72951, 72970, 72960, 0.302, 9.184, 0.131 72971, 72990, 72980, 0.302, 9.856, -0.337 72991, 73010, 73000, 0.317, 10.527, -0.297 73011, 73030, 73020, 0.317, 8.614, 0.278 73031, 73050, 73040, 0.384, 7.753, 0.421 73051, 73070, 73060, 0.384, 6.726, 0.710 73071, 73090, 73080, 0.472, 5.698, -0.051 73091, 73110, 73100, 0.472, 6.998, 0.212 73111, 73130, 73120, 0.504, 7.397, 0.042 73131, 73150, 73140, 0.504, 7.088, 0.044 73151, 73170, 73160, 0.470, 6.778, -0.068 73171, 73191, 73180, 0.470, 6.725, 0.344 73192, 73211, 73201, 0.516, 6.715, 0.388 73212, 73230, 73220, 0.516, 6.834, -0.341 73231, 73251, 73240, 0.471, 6.953, 0.114 73252, 73271, 73261, 0.471, 8.920, -0.271 73272, 73291, 73280, 0.426, 8.165, 0.502 73292, 73311, 73301, 0.426, 8.287, 0.113 73312, 73331, 73321, 0.370, 8.409, 0.603 73332, 73351, 73341, 0.370, 9.340, -0.186 73352, 73371, 73361, 0.429, 8.631, 0.300 73372, 73391, 73381, 0.429, 8.841, 0.255 73392, 73411, 73401, 0.335, 9.051, 0.342 73412, 73431, 73421, 0.335, 8.834, 0.319 73432, 73451, 73441, 0.416, 8.092, -0.070 73452, 73471, 73461, 0.416, 9.166, 0.018 73472, 73491, 73481, 0.485, 10.245, -0.157 73492, 73511, 73501, 0.485, 8.922, -0.024 73512, 73531, 73521, 0.442, 8.971, 0.288 73532, 73551, 73541, 0.442, 8.576, 0.089 73552, 73571, 73561, 0.427, 8.178, 0.278 73572, 73591, 73581, 0.427, 9.078, 0.428 73592, 73611, 73601, 0.439, 9.777, 0.230 73612, 73631, 73621, 0.439, 9.183, 0.051 73632, 73651, 73641, 0.467, 8.589, 0.491 73652, 73671, 73661, 0.467, 10.620, 0.640 73672, 73691, 73681, 0.396, 9.178, 0.228 73692, 73711, 73701, 0.396, 8.870, -0.082 73712, 73731, 73721, 0.504, 8.560, 0.206 73732, 73751, 73741, 0.504, 8.889, 0.375 73752, 73771, 73761, 0.458, 8.397, 0.528 73772, 73791, 73781, 0.458, 8.922, 0.096 73792, 73811, 73801, 0.331, 9.447, 0.072 73812, 73831, 73821, 0.331, 10.532, 0.063 73832, 73851, 73841, 0.439, 9.709, 0.103 73852, 73871, 73861, 0.439, 9.393, -0.078 73872, 73891, 73881, 0.480, 9.077, -0.277 73892, 73911, 73901, 0.480, 9.577, 0.229 73912, 73931, 73921, 0.472, 9.368, 0.169 73932, 73951, 73941, 0.472, 9.459, -0.316 73952, 73971, 73961, 0.364, 9.551, 0.010 73972, 73992, 73981, 0.364, 8.923, -0.104 73993, 74012, 74002, 0.350, 10.699, -0.562 74013, 74032, 74022, 0.350, 10.438, 0.018 74033, 74052, 74042, 0.434, 10.176, 0.670 74053, 74072, 74062, 0.434, 11.132, -0.128 74073, 74092, 74082, 0.398, 9.993, 0.459 74093, 74112, 74102, 0.398, 9.696, -0.133 74113, 74132, 74122, 0.350, 9.400, -0.373 74133, 74152, 74142, 0.350, 9.532, 0.471 74153, 74172, 74162, 0.387, 10.101, -0.390 74173, 74192, 74182, 0.387, 9.307, -0.146 74193, 74212, 74202, 0.373, 8.512, -0.425 74213, 74232, 74222, 0.373, 9.817, 1.104 74233, 74252, 74242, 0.380, 9.639, 0.628 74253, 74272, 74262, 0.380, 10.669, 0.203 74273, 74292, 74282, 0.350, 11.704, 0.376 74293, 74312, 74302, 0.350, 10.713, -9999.000 74313, 74332, 74322, 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