41, 1001 Brune, William; Thames, Alexander; Miller, David; Brosius, Alexandra Penn State University ATHOS - Airborne Tropospheric Hydrogen Oxides Sensor based on LIF ATom 1, 1 2016, 08, 06, 2017, 06, 06 0 Start_UTC, seconds, seconds since takeoff's midnight UTC 5 1, 1, 1, 1, 1 -9999.000, -9999.000, -9999.000, -9999.000, -9999.000 Stop_UTC, seconds, seconds since takeoff's midnight UTC Mid_UTC, seconds, seconds since takeoff's midnight UTC OH_pptv, pptv, OH mixing ratio in pptv HO2_pptv, pptv, HO2 mixing ratio in pptv OHR_Hz, Hz, OH reactivity in Hz 0 22 PI_CONTACT_INFO: Address: 503 Walker Building, University Park, PA 16802; email: whb2@psu.edu 814-865-3286 PLATFORM: NASA - DC-8 Aircraft - sampling underneath aircraft forward cargo bay LOCATION: ATom I: Science Flight #4 -- KOA - PPG ASSOCIATED_DATA: N/A INSTRUMENT_INFO: OH/HO2 with Laser Induced Fluorescence; OH reactivity with discharge flow DATA_INFO: Units are pptv for OH and HO2; Hz for OHR. UNCERTAINTY: Normaly HOx absolute accuracy is estimated to be +/- 32% at two sigma confidence. Please see comments below. ULOD_FLAG: -7777 ULOD_VALUE: N/A LLOD_FLAG: -8888 LLOD_VALUE: N/A DM_CONTACT_INFO: William H. Brune, Penn State, whb2@psu.edu; 814-865-3286 PROJECT_INFO: NSF/NASA ATom Mission. 2016 - 2018; Multiple Locations STIPULATIONS_ON_USE: No restrictions. Contact PI or DM with any questions. OTHER_COMMENTS: Semi-Final Data. Calibrating ATHOS with the new OH scavenging inlet is proving to be difficult. Until we complete more tests, OH uncertainty above 6 km estimated to be a factor of 2, 2 sigma confidence HO2 uncertainty for all altitudes estimated to be a factor of 1.6, 2 sigma confidence. OHR uncertainty estimated to be 15%, 2 sigma confidence, with 0.3 s^-1 zero uncertainty. OHR correction for NO appears to work for conditions with ambient NO<=~5 ppbv; OHR data are not reported for higher NO conditions. REVISION: R1 R1: Final Data Start_UTC, Stop_UTC, Mid_UTC, OH_pptv, HO2_pptv, OHR_Hz 65545, 65574, 65559, -9999.000, -9999.000, 2.186 65575, 65604, 65589, -9999.000, -9999.000, 2.852 65605, 65634, 65619, -9999.000, 10.486, 1.591 65635, 65664, 65649, -9999.000, 7.867, 2.586 65665, 65694, 65679, 0.086, 8.526, 2.201 65695, 65724, 65709, 0.106, 8.097, 2.588 65725, 65754, 65739, 0.106, 8.337, 1.890 65755, 65784, 65769, 0.279, 8.577, 1.832 65786, 65815, 65800, 0.279, 8.013, 1.676 65816, 65845, 65830, 0.190, 8.753, 1.693 65846, 65875, 65860, 0.190, 8.905, 1.668 65876, 65905, 65890, 0.152, 9.055, 1.843 65906, 65935, 65920, 0.152, 9.668, 2.111 65936, 65965, 65950, 0.197, 9.209, 1.684 65966, 65995, 65980, 0.197, 8.676, 2.236 65996, 66025, 66010, 0.101, 8.143, 0.894 66026, 66055, 66040, 0.101, 7.607, 2.097 66056, 66085, 66070, 0.233, 7.075, 1.231 66086, 66115, 66100, 0.233, 6.540, 2.038 66117, 66146, 66131, 0.201, 6.006, 1.952 66147, 66176, 66161, 0.201, 7.197, 0.867 66177, 66206, 66191, 0.178, 6.873, 1.457 66207, 66236, 66221, 0.178, 7.624, 1.205 66237, 66266, 66251, 0.205, 8.376, 1.912 66267, 66296, 66281, 0.205, 8.499, 1.526 66297, 66326, 66311, 0.210, 8.920, 1.533 66327, 66356, 66341, 0.210, 9.197, 0.648 66357, 66386, 66371, 0.155, 9.475, 1.061 66387, 66416, 66401, 0.155, 9.963, 1.608 66417, 66446, 66431, 0.107, 10.530, 0.815 66447, 66476, 66461, 0.107, 10.227, 1.500 66477, 66506, 66491, 0.142, 9.923, 1.174 66508, 66537, 66522, 0.142, 9.853, 1.150 66538, 66567, 66552, 0.176, 10.287, 0.927 66568, 66597, 66582, 0.176, 9.774, 0.908 66598, 66627, 66612, 0.183, 9.262, 1.260 66628, 66657, 66642, 0.183, 10.266, 1.049 66658, 66687, 66672, 0.157, 10.368, 0.535 66688, 66717, 66702, 0.157, 10.549, 1.191 66718, 66747, 66732, 0.120, 10.731, 0.629 66748, 66777, 66762, 0.120, 10.410, 0.421 66778, 66807, 66792, 0.120, 10.565, 1.397 66872, 66901, 66886, 0.168, 8.500, -9999.000 66903, 66932, 66917, 0.168, 7.832, 0.802 66933, 66962, 66947, 0.168, 10.747, 0.708 66963, 66992, 66977, 0.167, 11.023, 1.221 66993, 67022, 67007, 0.167, 11.014, 0.900 67023, 67052, 67037, 0.201, 11.005, 0.587 67053, 67082, 67067, 0.201, 10.676, 1.089 67083, 67112, 67097, 0.174, 11.133, 1.161 67113, 67142, 67127, 0.174, 10.540, 0.841 67143, 67172, 67157, 0.170, 9.943, 0.835 67173, 67202, 67187, 0.170, 11.644, 0.696 67203, 67232, 67217, 0.215, 11.399, 0.476 67233, 67262, 67247, 0.215, 10.713, 1.146 67263, 67292, 67277, 0.173, 10.030, 0.906 67293, 67322, 67307, 0.173, 11.331, -0.110 67324, 67353, 67338, 0.155, 10.016, 0.919 67354, 67383, 67368, 0.155, 9.433, -0.066 67384, 67413, 67398, 0.195, 8.846, 1.018 67414, 67443, 67428, 0.195, 9.768, 0.890 67444, 67473, 67458, 0.193, 10.397, 0.382 67474, 67503, 67488, 0.193, 10.489, 1.215 67504, 67533, 67518, 0.145, 10.581, 1.184 67534, 67563, 67548, 0.145, 11.497, 0.574 67564, 67593, 67578, 0.149, 11.848, 1.067 67594, 67623, 67608, 0.149, 10.660, 0.328 67624, 67653, 67638, 0.141, 9.464, 0.254 67654, 67683, 67668, 0.141, 10.528, 0.663 67684, 67713, 67698, 0.176, 11.424, 1.073 67715, 67744, 67729, 0.176, 10.978, 0.114 67745, 67774, 67759, 0.235, 10.533, 1.145 67775, 67804, 67789, 0.235, 11.339, 0.855 67805, 67834, 67819, 0.244, 11.026, 0.657 67835, 67864, 67849, 0.244, 10.837, 1.177 67865, 67894, 67879, 0.303, 10.645, 0.634 67895, 67924, 67909, 0.303, 10.507, 1.466 67925, 67954, 67939, 0.157, 10.127, 0.876 67955, 67984, 67969, 0.157, 9.221, 1.014 67985, 68014, 67999, 0.185, 8.319, 0.059 68015, 68044, 68029, 0.185, 9.833, 0.733 68045, 68074, 68059, 0.126, 9.174, 0.942 68075, 68104, 68089, 0.126, 8.301, 1.057 68106, 68135, 68120, 0.114, 7.423, 0.276 68136, 68165, 68150, 0.114, 6.583, 0.100 68166, 68195, 68180, 0.135, 7.386, 1.324 68196, 68225, 68210, 0.135, 7.549, 0.593 68226, 68255, 68240, 0.119, 7.713, 0.499 68256, 68285, 68270, 0.119, 7.875, -0.002 68286, 68315, 68300, 0.113, 8.581, 0.586 68316, 68345, 68330, 0.113, 9.589, -0.308 68346, 68375, 68360, 0.135, 10.604, 0.687 68376, 68405, 68390, 0.135, 11.343, 0.879 68406, 68435, 68420, 0.167, 12.152, 1.551 68436, 68465, 68450, 0.167, 11.646, 2.301 68466, 68495, 68480, 0.138, 11.142, 2.723 68496, 68525, 68510, 0.138, 11.764, 1.722 68527, 68556, 68541, 0.094, 13.071, 1.568 68557, 68586, 68571, 0.094, 14.027, 2.223 68587, 68616, 68601, 0.149, 14.987, 3.425 68617, 68646, 68631, 0.149, 18.671, 2.853 68647, 68676, 68661, 0.229, 23.305, 2.882 68677, 68706, 68691, 0.229, 22.085, 1.476 68707, 68736, 68721, 0.160, 20.874, 2.618 68737, 68766, 68751, 0.160, 23.928, 4.306 68767, 68796, 68781, 0.151, 23.320, 3.385 68797, 68826, 68811, 0.151, 23.534, 1.131 68827, 68856, 68841, 0.065, 23.748, 0.518 68857, 68886, 68871, 0.065, 36.440, -0.063 68887, 68916, 68901, 0.132, 36.336, -9999.000 68918, 68947, 68932, 0.132, 37.104, -0.621 68948, 68977, 68962, 0.132, 37.870, -9999.000 69045, 69074, 69059, 0.137, 32.838, -9999.000 69076, 69105, 69090, 0.137, 31.365, 1.017 69106, 69135, 69120, 0.137, 32.495, -0.400 69136, 69165, 69150, 0.135, 33.628, 1.517 69166, 69195, 69180, 0.135, 34.468, 1.781 69196, 69225, 69210, 0.126, 44.235, 2.403 69226, 69255, 69240, 0.126, 40.980, 1.433 69256, 69285, 69270, 0.249, 37.725, 1.929 69286, 69315, 69300, 0.249, 37.385, 1.833 69316, 69345, 69330, 0.265, 34.146, 3.930 69346, 69375, 69360, 0.265, 27.095, 2.168 69376, 69405, 69390, 0.131, 20.068, 1.953 69406, 69435, 69420, 0.131, 17.499, 1.708 69436, 69465, 69450, 0.146, 12.162, 2.332 69466, 69495, 69480, 0.146, 13.143, 0.980 69496, 69525, 69510, 0.161, 14.123, 0.801 69526, 69555, 69540, 0.161, 12.883, 0.945 69557, 69586, 69571, 0.200, 12.770, 1.260 69587, 69616, 69601, 0.200, 13.317, 0.365 69617, 69646, 69631, 0.237, 13.866, 0.755 69647, 69676, 69661, 0.237, 13.902, 1.378 69677, 69706, 69691, 0.196, 12.790, 1.505 69707, 69736, 69721, 0.196, 12.432, 0.532 69737, 69766, 69751, 0.202, 12.074, 1.897 69767, 69796, 69781, 0.202, 11.072, 1.160 69797, 69826, 69811, 0.178, 11.092, 0.706 69827, 69856, 69841, 0.178, 10.168, 0.024 69857, 69886, 69871, 0.180, 9.247, 0.503 69888, 69917, 69902, 0.180, 8.865, 1.011 69917, 69946, 69931, 0.158, 8.834, 0.537 69948, 69977, 69962, 0.158, 8.137, 1.073 69978, 70007, 69992, 0.158, 7.439, 0.801 70008, 70037, 70022, 0.158, 7.470, -0.209 70038, 70067, 70052, 0.171, 7.505, 1.107 70068, 70097, 70082, 0.171, 7.166, 1.318 70098, 70127, 70112, 0.095, 6.826, 0.300 70128, 70157, 70142, 0.095, 7.577, 0.650 70158, 70187, 70172, 0.128, 7.688, 0.662 70188, 70217, 70202, 0.128, 8.327, 0.659 70218, 70247, 70232, 0.157, 8.960, 0.931 70248, 70277, 70262, 0.157, 9.369, 0.671 70278, 70307, 70292, 0.131, 8.906, 1.016 70308, 70337, 70322, 0.131, 9.165, 0.286 70339, 70368, 70353, 0.168, 9.425, 0.714 70369, 70398, 70383, 0.168, 10.808, 1.075 70399, 70428, 70413, 0.243, 9.769, 0.812 70429, 70458, 70443, 0.243, 10.489, 0.745 70459, 70488, 70473, 0.269, 11.207, 0.357 70489, 70518, 70503, 0.269, 10.414, 0.308 70519, 70548, 70533, 0.235, 11.649, 0.293 70549, 70578, 70563, 0.235, 11.335, 0.351 70579, 70608, 70593, 0.208, 11.021, 0.734 70609, 70638, 70623, 0.208, 11.482, 0.682 70639, 70668, 70653, 0.251, 11.724, 0.517 70669, 70698, 70683, 0.251, 12.173, 0.934 70699, 70728, 70713, 0.159, 12.621, 0.327 70729, 70758, 70743, 0.159, 14.260, 0.623 70760, 70789, 70774, 0.205, 13.354, 0.953 70790, 70819, 70804, 0.205, 12.603, 0.687 70820, 70849, 70834, 0.266, 11.856, 0.405 70850, 70879, 70864, 0.266, 12.473, 0.977 70880, 70909, 70894, 0.245, 13.990, 0.741 70910, 70939, 70924, 0.245, 12.774, 0.475 70940, 70969, 70954, 0.304, 11.559, -0.082 70970, 70999, 70984, 0.304, 13.131, 0.426 71000, 71029, 71014, 0.294, 11.887, 0.596 71030, 71059, 71044, 0.294, 11.516, 0.494 71060, 71089, 71074, 0.234, 11.144, -0.273 71090, 71119, 71104, 0.234, 12.186, 0.721 71120, 71149, 71134, 0.245, 12.404, 0.177 71151, 71180, 71165, 0.245, 11.927, 1.522 71181, 71210, 71195, 0.220, 11.449, 0.413 71211, 71240, 71225, 0.220, 10.804, 0.701 71241, 71270, 71255, 0.321, 12.682, 1.505 71271, 71300, 71285, 0.321, 12.552, 0.791 71301, 71330, 71315, 0.270, 12.422, 0.878 71331, 71360, 71345, 0.270, 13.342, 1.156 71361, 71390, 71375, 0.344, 13.485, -0.216 71391, 71420, 71405, 0.344, 13.111, 0.620 71421, 71450, 71435, 0.219, 12.737, 0.053 71451, 71480, 71465, 0.219, 10.765, 0.538 71481, 71510, 71495, 0.095, 10.162, 0.547 71511, 71540, 71525, 0.095, 9.956, 0.537 71541, 71570, 71555, 0.129, 9.748, 0.404 71572, 71601, 71586, 0.129, 10.916, 0.338 71602, 71631, 71616, 0.168, 10.142, 0.475 71632, 71661, 71646, 0.168, 10.431, -0.039 71662, 71691, 71676, 0.154, 10.720, 0.841 71692, 71721, 71706, 0.154, 11.548, 0.018 71722, 71751, 71736, 0.188, 12.188, -0.098 71752, 71781, 71766, 0.188, 14.274, 0.836 71782, 71811, 71796, 0.277, 16.353, 0.283 71812, 71841, 71826, 0.277, 16.732, 1.107 71842, 71871, 71856, 0.265, 17.339, 2.297 71872, 71901, 71886, 0.265, 20.328, 1.065 71902, 71931, 71916, 0.367, 23.338, 1.565 71932, 71961, 71946, 0.367, 21.740, 1.242 71963, 71992, 71977, 0.220, 23.040, 1.490 71992, 72021, 72006, 0.220, 20.187, 2.805 72023, 72052, 72037, -9999.000, -9999.000, 1.830 72053, 72082, 72067, -9999.000, -9999.000, 3.210 72083, 72112, 72097, -9999.000, -9999.000, 3.406 72113, 72142, 72127, -9999.000, -9999.000, 1.503 72143, 72172, 72157, 0.168, 25.735, 2.255 72173, 72202, 72187, 0.168, 31.330, 2.166 72203, 72232, 72217, 0.124, 38.953, 3.518 72233, 72262, 72247, 0.124, 38.165, 0.731 72263, 72292, 72277, 0.105, 37.377, -9999.000 72293, 72322, 72307, 0.105, 32.115, 1.378 72323, 72352, 72337, 0.129, 40.613, -9999.000 72353, 72382, 72367, 0.129, 37.338, -0.655 72383, 72412, 72397, 0.122, 34.063, 1.571 72413, 72442, 72427, 0.122, 40.425, -9999.000 72444, 72473, 72458, 0.100, 41.520, -9999.000 72474, 72503, 72488, 0.100, 41.746, -0.677 72504, 72533, 72518, 0.085, 41.972, -0.213 72534, 72563, 72548, 0.085, 51.852, -0.656 72564, 72593, 72578, 0.120, 47.880, -0.912 72594, 72623, 72608, 0.120, 39.216, 0.650 72624, 72653, 72638, 0.066, 30.551, -9999.000 72654, 72683, 72668, 0.066, 30.029, 0.577 72684, 72713, 72698, 0.821, 43.798, 3.049 72714, 72743, 72728, 0.821, 36.690, 0.296 72744, 72773, 72758, 0.288, 29.606, 3.890 72775, 72804, 72789, 0.288, 35.679, 1.599 72805, 72834, 72819, 0.245, 34.846, 1.539 72835, 72864, 72849, 0.245, 28.465, -0.089 72865, 72894, 72879, 0.338, 22.084, 1.589 72895, 72924, 72909, 0.338, 19.093, 1.722 72925, 72954, 72939, 0.296, 19.018, 0.468 72955, 72984, 72969, 0.296, 17.418, 0.956 72985, 73014, 72999, 0.296, 15.824, 0.275 73015, 73044, 73029, 0.296, 17.193, 0.712 73045, 73074, 73059, 0.250, 15.896, 0.728 73075, 73104, 73089, 0.250, 13.102, 0.545 73105, 73134, 73119, 0.118, 10.307, 1.050 73135, 73164, 73149, 0.118, 10.068, -0.151 73165, 73194, 73179, 0.138, 8.299, 0.110 73195, 73224, 73209, 0.138, 9.026, 0.023 73226, 73255, 73240, 0.200, 9.753, 0.126 73256, 73285, 73270, 0.200, 11.041, 0.497 73286, 73315, 73300, 0.181, 10.106, 0.764 73316, 73345, 73330, 0.181, 9.283, 0.594 73346, 73375, 73360, 0.188, 8.459, -0.070 73376, 73405, 73390, 0.188, 10.834, 0.515 73406, 73435, 73420, 0.205, 9.945, 0.089 73436, 73465, 73450, 0.205, 9.362, 0.554 73466, 73495, 73480, 0.166, 8.781, 0.569 73496, 73525, 73510, 0.166, 10.713, 1.068 73526, 73555, 73540, 0.200, 11.332, 0.187 73556, 73585, 73570, 0.200, 10.946, 0.846 73587, 73616, 73601, 0.173, 10.557, 0.134 73617, 73646, 73631, 0.173, 11.735, 0.804 73647, 73676, 73661, 0.198, 13.634, 0.591 73677, 73706, 73691, 0.198, 12.282, 0.417 73707, 73736, 73721, 0.248, 10.935, 0.623 73737, 73766, 73751, 0.248, 12.777, -0.124 73767, 73796, 73781, 0.287, 13.855, 0.416 73797, 73826, 73811, 0.287, 12.945, 0.194 73827, 73856, 73841, 0.172, 12.030, 0.309 73857, 73886, 73871, 0.172, 12.224, 0.467 73887, 73916, 73901, 0.237, 12.254, 0.553 73917, 73946, 73931, 0.237, 11.798, 0.603 73947, 73976, 73961, 0.192, 11.344, -0.067 73978, 74007, 73992, 0.192, 13.007, 0.241 74008, 74037, 74022, 0.138, 12.987, 0.729 74038, 74067, 74052, 0.138, 13.565, 0.579 74068, 74097, 74082, 0.196, 14.146, 0.406 74098, 74127, 74112, 0.196, 13.715, 0.096 74128, 74157, 74142, 0.153, 14.595, 0.715 74158, 74187, 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