41, 1001 Brune, William; Thames, Alexander; Miller, David; Brosius, Alexandra Penn State University ATHOS - Airborne Tropospheric Hydrogen Oxides Sensor based on LIF ATom 1, 1 2016, 08, 03, 2017, 06, 06 0 Start_UTC, seconds, seconds since takeoff's midnight UTC 5 1, 1, 1, 1, 1 -9999.000, -9999.000, -9999.000, -9999.000, -9999.000 Stop_UTC, seconds, seconds since takeoff's midnight UTC Mid_UTC, seconds, seconds since takeoff's midnight UTC OH_pptv, pptv, OH mixing ratio in pptv HO2_pptv, pptv, HO2 mixing ratio in pptv OHR_Hz, Hz, OH reactivity in Hz 0 22 PI_CONTACT_INFO: Address: 503 Walker Building, University Park, PA 16802; email: whb2@psu.edu 814-865-3286 PLATFORM: NASA - DC-8 Aircraft - sampling underneath aircraft forward cargo bay LOCATION: ATom I: Science Flight #3 -- ANC - KOA ASSOCIATED_DATA: N/A INSTRUMENT_INFO: OH/HO2 with Laser Induced Fluorescence; OH reactivity with discharge flow DATA_INFO: Units are pptv for OH and HO2; Hz for OHR. UNCERTAINTY: Normaly HOx absolute accuracy is estimated to be +/- 32% at two sigma confidence. Please see comments below. ULOD_FLAG: -7777 ULOD_VALUE: N/A LLOD_FLAG: -8888 LLOD_VALUE: N/A DM_CONTACT_INFO: William H. Brune, Penn State, whb2@psu.edu; 814-865-3286 PROJECT_INFO: NSF/NASA ATom Mission. 2016 - 2018; Multiple Locations STIPULATIONS_ON_USE: No restrictions. Contact PI or DM with any questions. OTHER_COMMENTS: Semi-Final Data. Calibrating ATHOS with the new OH scavenging inlet is proving to be difficult. Until we complete more tests, OH uncertainty above 6 km estimated to be a factor of 2, 2 sigma confidence HO2 uncertainty for all altitudes estimated to be a factor of 1.6, 2 sigma confidence. OHR uncertainty estimated to be 15%, 2 sigma confidence, with 0.3 s^-1 zero uncertainty. OHR correction for NO appears to work for conditions with ambient NO<=~5 ppbv; OHR data are not reported for higher NO conditions. REVISION: R1 R1: Final Data Start_UTC, Stop_UTC, Mid_UTC, OH_pptv, HO2_pptv, OHR_Hz 68446, 68475, 68460, -9999.000, -9999.000, -1.642 68506, 68535, 68520, -9999.000, -9999.000, 4.203 68536, 68565, 68550, -9999.000, -9999.000, 3.921 68566, 68595, 68580, -9999.000, 43.739, 1.569 68596, 68625, 68610, -9999.000, 22.985, 1.738 68626, 68655, 68640, 0.075, 23.441, 3.008 68656, 68685, 68670, 0.096, 19.970, 2.141 68686, 68715, 68700, 0.096, 18.205, -0.220 68717, 68746, 68731, 0.009, 16.439, 0.867 68747, 68776, 68761, 0.009, 17.857, 1.033 68777, 68806, 68791, 0.079, 15.781, 0.671 68807, 68836, 68821, 0.079, 14.944, 1.008 68837, 68866, 68851, 0.076, 14.102, 1.369 68867, 68896, 68881, 0.076, 12.830, 1.658 68897, 68926, 68911, 0.119, 10.893, 0.793 68927, 68956, 68941, 0.119, 12.310, 2.163 68957, 68986, 68971, 0.113, 13.726, 1.755 68987, 69016, 69001, 0.113, 12.703, 2.413 69017, 69046, 69031, 0.040, 11.674, 2.513 69047, 69076, 69061, 0.040, 11.243, 2.430 69077, 69106, 69091, 0.161, 10.809, 1.591 69107, 69136, 69121, 0.161, 11.028, 1.756 69137, 69166, 69151, 0.111, 9.919, 1.522 69167, 69196, 69181, 0.111, 9.479, 2.340 69197, 69226, 69211, 0.016, 9.036, 1.708 69227, 69256, 69241, 0.016, 8.595, 2.350 69257, 69286, 69271, 0.101, 8.155, 1.593 69287, 69316, 69301, 0.101, 7.713, 1.463 69317, 69346, 69331, 0.098, 7.270, 1.624 69347, 69376, 69361, 0.098, 8.411, 1.742 69377, 69406, 69391, 0.027, 9.084, 1.443 69407, 69436, 69421, 0.027, 8.914, 1.675 69438, 69467, 69452, 0.051, 8.743, 1.221 69468, 69497, 69482, 0.051, 10.733, 1.678 69498, 69527, 69512, 0.045, 12.887, 2.180 69528, 69557, 69542, 0.045, 11.263, 0.995 69558, 69587, 69572, 0.055, 9.628, 1.878 69588, 69617, 69602, 0.055, 11.791, 1.508 69618, 69647, 69632, 0.094, 11.270, 1.331 69648, 69677, 69662, 0.094, 11.988, 1.650 69678, 69707, 69692, 0.048, 12.701, 1.643 69708, 69737, 69722, 0.048, 14.905, 0.622 69738, 69767, 69752, 0.088, 12.943, 1.485 69768, 69797, 69782, 0.088, 11.558, 1.936 69798, 69827, 69812, 0.132, 10.178, 1.022 69828, 69857, 69842, 0.132, 10.374, 0.879 69858, 69887, 69872, 0.132, 9.900, 0.818 69969, 69998, 69983, 0.127, 10.480, -9999.000 69999, 70028, 70013, 0.127, 10.636, 1.166 70029, 70058, 70043, 0.127, 12.299, 0.887 70059, 70088, 70073, 0.040, 12.084, 1.243 70089, 70118, 70103, 0.040, 12.317, 1.191 70119, 70148, 70133, 0.102, 12.551, 1.395 70149, 70178, 70163, 0.102, 13.174, 0.934 70180, 70209, 70194, 0.115, 12.652, 1.234 70210, 70239, 70224, 0.115, 12.355, 1.046 70240, 70269, 70254, 0.197, 12.058, 0.577 70270, 70299, 70284, 0.197, 10.975, 0.968 70300, 70329, 70314, 0.109, 11.811, 1.143 70330, 70359, 70344, 0.109, 12.380, 0.770 70360, 70389, 70374, 0.208, 12.949, 0.763 70390, 70419, 70404, 0.208, 13.024, 0.423 70420, 70449, 70434, 0.168, 14.040, 0.748 70450, 70479, 70464, 0.168, 13.301, 0.564 70480, 70509, 70494, 0.172, 12.559, 1.239 70510, 70539, 70524, 0.172, 13.977, 1.376 70540, 70569, 70554, 0.325, 13.384, 1.198 70570, 70599, 70584, 0.325, 13.286, 1.136 70600, 70629, 70614, 0.303, 13.188, -0.412 70630, 70659, 70644, 0.303, 13.149, 0.840 70660, 70689, 70674, 0.235, 14.853, 0.277 70691, 70720, 70705, 0.235, 13.795, 0.960 70721, 70750, 70735, 0.117, 12.741, 0.285 70751, 70780, 70765, 0.117, 13.106, 0.379 70781, 70810, 70795, 0.159, 12.589, 0.825 70811, 70840, 70825, 0.159, 12.495, 1.171 70841, 70870, 70855, 0.138, 12.401, 0.616 70871, 70900, 70885, 0.138, 12.613, 0.847 70901, 70930, 70915, 0.173, 13.475, 0.404 70931, 70960, 70945, 0.173, 13.214, 0.484 70961, 70990, 70975, 0.203, 12.954, 0.970 70991, 71020, 71005, 0.203, 14.175, 1.140 71021, 71050, 71035, 0.121, 13.464, 0.648 71051, 71080, 71065, 0.121, 12.457, 0.940 71081, 71110, 71095, 0.234, 11.450, 0.327 71111, 71140, 71125, 0.234, 12.304, 0.834 71141, 71170, 71155, 0.167, 13.332, 0.148 71171, 71200, 71185, 0.167, 12.683, 1.181 71201, 71230, 71215, 0.188, 12.029, 0.471 71231, 71260, 71245, 0.188, 13.456, 0.930 71262, 71291, 71276, 0.198, 13.737, 1.054 71292, 71321, 71306, 0.198, 13.269, 0.328 71322, 71351, 71336, 0.208, 12.800, 0.784 71352, 71381, 71366, 0.208, 13.801, 1.003 71382, 71411, 71396, 0.292, 14.379, 0.975 71412, 71441, 71426, 0.292, 13.852, 1.724 71442, 71471, 71456, 0.284, 13.326, 1.167 71472, 71501, 71486, 0.284, 15.724, 0.871 71502, 71531, 71516, 0.258, 14.754, 0.748 71532, 71561, 71546, 0.258, 13.332, 1.161 71562, 71591, 71576, 0.173, 11.910, 0.392 71592, 71621, 71606, -9999.000, -9999.000, 0.498 71622, 71651, 71636, 0.347, 13.208, -0.338 71652, 71681, 71666, 0.347, 13.119, 0.695 71682, 71711, 71696, 0.192, 13.031, 1.006 71712, 71741, 71726, 0.192, 13.288, 0.800 71742, 71771, 71756, 0.197, 12.766, 0.955 71772, 71801, 71786, 0.197, 12.309, 0.639 71802, 71831, 71816, 0.268, 11.852, 0.534 71832, 71861, 71846, 0.268, 12.545, 0.527 71863, 71892, 71877, 0.373, 13.174, 1.168 71893, 71922, 71907, 0.373, 12.873, 0.292 71923, 71952, 71937, 0.250, 12.574, 0.786 71953, 71982, 71967, 0.250, 11.744, 0.985 71983, 72012, 71997, 0.261, 12.972, 0.872 72013, 72042, 72027, 0.261, 11.921, 0.834 72043, 72072, 72057, 0.314, 10.866, 0.432 72073, 72102, 72087, 0.314, 11.591, 0.525 72103, 72132, 72117, 0.360, 13.623, 0.872 72133, 72162, 72147, 0.360, 12.004, 0.831 72163, 72192, 72177, 0.323, 10.373, 0.857 72193, 72222, 72207, 0.323, 11.250, 0.317 72223, 72252, 72237, 0.367, 12.491, 0.332 72253, 72282, 72267, 0.367, 10.969, 0.244 72283, 72312, 72297, 0.230, 9.457, 1.242 72313, 72342, 72327, 0.230, 10.663, 0.579 72343, 72372, 72357, 0.210, 11.719, 0.618 72374, 72403, 72388, 0.210, 11.315, 0.952 72404, 72433, 72418, 0.371, 10.914, 0.899 72434, 72463, 72448, 0.371, 10.372, 0.360 72464, 72493, 72478, 0.281, 9.525, 0.329 72494, 72523, 72508, 0.281, 8.419, 0.754 72524, 72553, 72538, 0.194, 7.321, 1.569 72554, 72583, 72568, 0.194, 9.368, 0.559 72584, 72613, 72598, 0.310, 13.787, 0.965 72614, 72643, 72628, 0.310, 13.257, 1.185 72644, 72673, 72658, 0.280, 12.726, 0.385 72674, 72703, 72688, 0.280, 12.860, 0.180 72704, 72733, 72718, 0.180, 12.723, -9999.000 72734, 72763, 72748, 0.180, 12.348, 0.731 72764, 72793, 72778, 0.112, 11.971, -0.006 72794, 72823, 72808, 0.112, 11.548, -9999.000 72824, 72853, 72838, 0.208, 11.749, 0.701 72854, 72883, 72868, 0.208, 11.693, 0.754 72884, 72913, 72898, 0.270, 11.637, -0.055 72914, 72943, 72928, 0.270, 11.381, 0.407 72944, 72973, 72958, 0.213, 11.091, 0.238 72975, 73004, 72989, 0.213, 11.170, 0.018 73005, 73034, 73019, 0.277, 11.250, 0.369 73035, 73064, 73049, 0.277, 10.528, 0.779 73065, 73094, 73079, 0.197, 11.115, 0.793 73095, 73124, 73109, 0.197, 9.275, 0.984 73125, 73154, 73139, 0.087, 7.435, 2.262 73155, 73184, 73169, 0.087, 5.810, 1.437 73185, 73214, 73199, 0.197, 8.467, 0.530 73215, 73244, 73229, 0.197, 7.283, 1.856 73245, 73274, 73259, -0.025, 6.103, 3.098 73275, 73304, 73289, -0.025, 9.923, -0.130 73305, 73334, 73319, 0.034, 7.562, 0.519 73335, 73364, 73349, 0.034, 6.938, 1.655 73365, 73394, 73379, 0.054, 6.312, 1.363 73395, 73424, 73409, 0.054, 7.589, 1.286 73425, 73454, 73439, 0.072, 5.723, -9999.000 73455, 73484, 73469, 0.072, 5.624, -0.697 73485, 73514, 73499, -9999.000, -9999.000, -1.219 73515, 73544, 73529, 0.105, 5.307, -0.871 73546, 73575, 73560, 0.123, 4.992, -9999.000 73576, 73605, 73590, 0.123, 5.507, -9999.000 73606, 73635, 73620, 0.113, 6.022, -9999.000 73636, 73665, 73650, 0.113, 3.468, -9999.000 73666, 73695, 73680, 0.015, 3.229, -9999.000 73696, 73725, 73710, 0.015, 2.763, -0.124 73726, 73755, 73740, 0.087, 2.296, -9999.000 73756, 73785, 73770, 0.087, 3.544, -9999.000 73786, 73815, 73800, -0.009, 5.580, 0.431 73816, 73845, 73830, -0.009, 7.767, -0.694 73846, 73875, 73860, -0.020, 9.954, 1.108 73876, 73905, 73890, -0.020, 9.525, 2.169 73906, 73935, 73920, 0.039, 8.398, 1.475 73936, 73965, 73950, 0.039, 6.808, 0.634 73966, 73995, 73980, -0.004, 5.223, 1.246 73996, 74025, 74010, -0.004, 5.390, 0.974 74027, 74056, 74041, 0.138, 11.379, 1.374 74057, 74086, 74071, 0.138, 10.694, 0.987 74087, 74116, 74101, 0.169, 10.009, 1.966 74117, 74146, 74131, 0.169, 11.069, 1.004 74147, 74176, 74161, 0.173, 7.990, 0.298 74177, 74206, 74191, 0.173, 10.153, 1.864 74207, 74236, 74221, 0.195, 12.331, -0.324 74237, 74266, 74251, 0.195, 12.599, 0.493 74267, 74296, 74281, 0.212, 10.857, 2.203 74297, 74326, 74311, 0.212, 11.773, -0.706 74327, 74356, 74341, 0.245, 12.688, 1.036 74357, 74386, 74371, 0.245, 13.416, 0.762 74387, 74416, 74401, 0.262, 11.793, 1.383 74417, 74446, 74431, 0.262, 9.827, 0.193 74447, 74476, 74461, 0.282, 7.861, 0.289 74477, 74506, 74491, 0.282, 11.474, 0.379 74507, 74536, 74521, 0.398, 11.982, 1.002 74537, 74566, 74551, 0.398, 11.909, 0.575 74567, 74596, 74581, 0.340, 11.835, -0.381 74597, 74626, 74611, 0.340, 14.218, 0.340 74628, 74657, 74642, 0.396, 14.309, 1.059 74658, 74687, 74672, 0.396, 13.460, 0.571 74688, 74717, 74702, 0.345, 12.614, 0.936 74718, 74747, 74732, 0.345, 11.414, 0.867 74748, 74777, 74762, 0.314, 11.017, -0.313 74778, 74807, 74792, 0.314, 11.599, 1.136 74808, 74837, 74822, 0.232, 12.184, -0.007 74838, 74867, 74852, 0.232, 13.957, 0.305 74868, 74897, 74882, 0.307, 13.524, 0.828 74898, 74927, 74912, 0.307, 11.799, 0.349 74928, 74957, 74942, 0.293, 10.075, 0.300 74958, 74987, 74972, 0.293, 11.036, 0.926 74988, 75017, 75002, 0.280, 11.128, -0.013 75018, 75047, 75032, 0.280, 11.118, 0.381 75048, 75077, 75062, 0.319, 11.107, 0.593 75078, 75107, 75092, 0.319, 11.560, 0.258 75108, 75137, 75122, 0.232, 10.171, -0.042 75139, 75168, 75153, 0.232, 10.655, -9999.000 75169, 75198, 75183, 0.230, 11.141, -0.032 75199, 75228, 75213, 0.230, 11.620, 0.219 75229, 75258, 75243, 0.238, 11.896, 0.556 75259, 75288, 75273, 0.238, 11.402, 0.592 75289, 75318, 75303, 0.341, 10.909, 0.955 75319, 75348, 75333, 0.341, 11.164, 1.099 75349, 75378, 75363, 0.270, 12.786, 0.672 75379, 75408, 75393, 0.270, 11.706, 0.807 75409, 75438, 75423, 0.391, 10.625, 0.900 75439, 75468, 75453, 0.391, 9.672, 0.350 75469, 75498, 75483, 0.430, 14.822, 0.909 75499, 75528, 75513, 0.430, 12.882, -9999.000 75529, 75558, 75543, 0.253, 10.949, 0.424 75559, 75588, 75573, 0.253, 9.920, -0.112 75589, 75618, 75603, 0.272, 11.797, 1.264 75619, 75648, 75633, 0.272, 10.877, 0.446 75649, 75678, 75663, 0.327, 9.956, 0.727 75680, 75709, 75694, 0.327, 11.859, 0.398 75710, 75739, 75724, 0.263, 11.183, 0.446 75740, 75769, 75754, 0.263, 9.918, 0.239 75770, 75799, 75784, 0.473, 8.654, 0.629 75800, 75829, 75814, 0.473, 11.076, 0.824 75830, 75859, 75844, 0.343, 9.688, 0.283 75860, 75889, 75874, 0.343, 9.591, 1.129 75890, 75919, 75904, 0.419, 9.494, 0.279 75920, 75949, 75934, 0.419, 10.936, 0.995 75950, 75979, 75964, 0.360, 8.821, 0.672 75980, 76009, 75994, 0.360, 9.174, -0.265 76010, 76039, 76024, 0.406, 9.527, 0.758 76040, 76069, 76054, 0.406, 9.329, 1.047 76070, 76099, 76084, 0.430, 9.165, 1.496 76100, 76129, 76114, 0.430, 8.342, 0.562 76130, 76159, 76144, 0.355, 7.519, 0.615 76160, 76189, 76174, 0.355, 8.138, 0.944 76191, 76220, 76205, 0.514, 9.506, 0.893 76221, 76250, 76235, 0.514, 9.005, 0.248 76251, 76280, 76265, 0.384, 8.507, 0.460 76281, 76310, 76295, 0.384, 7.269, 0.656 76311, 76340, 76325, 0.385, 8.659, 0.615 76341, 76370, 76355, 0.385, 8.346, 1.258 76371, 76400, 76385, 0.399, 8.034, 0.410 76401, 76430, 76415, 0.399, 7.504, 0.356 76431, 76460, 76445, 0.324, 9.830, 0.725 76461, 76490, 76475, 0.324, 9.279, 0.031 76491, 76520, 76505, 0.322, 8.727, 0.421 76521, 76550, 76535, 0.322, 8.381, 1.392 76551, 76580, 76565, 0.225, 10.375, 0.229 76581, 76610, 76595, 0.225, 9.029, 1.217 76611, 76640, 76625, 0.116, 7.684, -0.020 76641, 76670, 76655, 0.116, 8.165, 0.011 76671, 76700, 76685, 0.149, 7.442, -9999.000 76701, 76730, 76715, 0.149, 7.387, -0.147 76731, 76760, 76745, 0.109, 7.332, 0.283 76761, 76790, 76775, 0.109, 8.290, -0.127 76791, 76820, 76805, 0.108, 7.960, 0.012 76822, 76851, 76836, 0.108, 7.266, 0.050 76852, 76881, 76866, 0.181, 6.575, 0.991 76882, 76911, 76896, 0.181, 7.650, -0.072 76912, 76941, 76926, 0.178, 5.979, -0.258 76942, 76971, 76956, 0.178, 6.156, 0.394 76972, 77001, 76986, 0.097, 6.334, -0.774 77002, 77031, 77016, 0.097, 6.841, 0.838 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